Ultrafast Vibrational Energy Transfer between Protein and Cofactor in a Flavoenzyme

Protein motions and enzyme catalysis are often linked. It is hypothesized that ultrafast vibrations (femtosecond–picosecond) enhance the rate of hydride transfer catalyzed by members of the old yellow enzyme (OYE) family of ene-reductases. Here, we use time-resolved infrared (TRIR) spectroscopy in c...

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Veröffentlicht in:	The journal of physical chemistry. B 2020-06, Vol.124 (25), p.5163-5168
Hauptverfasser:	Hardman, Samantha J. O, Iorgu, Andreea I, Heyes, Derren J, Scrutton, Nigel S, Sazanovich, Igor V, Hay, Sam
Format:	Artikel
Sprache:	eng
Schlagworte:	B: Biophysics Physical Chemistry of Biological Systems and Biomolecules Catalysis Energy Transfer Flavin Mononucleotide Flavins Vibration
Online-Zugang:	Volltext
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