(Bio)Degradable Polymeric Materials for Sustainable Future-Part 3: Degradation Studies of the PHA/Wood Flour-Based Composites and Preliminary Tests of Antimicrobial Activity
The need for a cost reduction of the materials derived from (bio)degradable polymers forces research development into the formation of biocomposites with cheaper fillers. As additives can be made using the post-consumer wood, generated during wood products processing, re-use of recycled waste materi...
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| Veröffentlicht in: | Materials 2020-05, Vol.13 (9), p.2200 |
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| creator | Musioł, Marta Jurczyk, Sebastian Sobota, Michał Klim, Magdalena Sikorska, Wanda Zięba, Magdalena Janeczek, Henryk Rydz, Joanna Kurcok, Piotr Johnston, Brian Radecka, Izabela |
| description | The need for a cost reduction of the materials derived from (bio)degradable polymers forces research development into the formation of biocomposites with cheaper fillers. As additives can be made using the post-consumer wood, generated during wood products processing, re-use of recycled waste materials in the production of biocomposites can be an environmentally friendly way to minimalize and/or utilize the amount of the solid waste. Also, bioactive materials, which possess small amounts of antimicrobial additives belong to a very attractive packaging industry solution. This paper presents a study into the biodegradation, under laboratory composting conditions, of the composites that consist of poly[(
)-3-hydroxybutyrate-
-4-hydroxybutyrate)] and wood flour as a polymer matrix and natural filler, respectively. Thermogravimetric analysis, differential scanning calorimetry and scanning electron microscopy were used to evaluate the degradation progress of the obtained composites with different amounts of wood flour. The degradation products were characterized by multistage electrospray ionization mass spectrometry. Also, preliminary tests of the antimicrobial activity of selected materials with the addition of nisin were performed. The obtained results suggest that the different amount of filler has a significant influence on the degradation profile. |
| doi_str_mv | 10.3390/ma13092200 |
| format | Article |
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)-3-hydroxybutyrate-
-4-hydroxybutyrate)] and wood flour as a polymer matrix and natural filler, respectively. Thermogravimetric analysis, differential scanning calorimetry and scanning electron microscopy were used to evaluate the degradation progress of the obtained composites with different amounts of wood flour. The degradation products were characterized by multistage electrospray ionization mass spectrometry. Also, preliminary tests of the antimicrobial activity of selected materials with the addition of nisin were performed. The obtained results suggest that the different amount of filler has a significant influence on the degradation profile.</description><identifier>ISSN: 1996-1944</identifier><identifier>EISSN: 1996-1944</identifier><identifier>DOI: 10.3390/ma13092200</identifier><identifier>PMID: 32403315</identifier><language>eng</language><publisher>Switzerland: MDPI AG</publisher><subject>Additives ; Antiinfectives and antibacterials ; Antimicrobial agents ; Biocompatibility ; Biodegradable materials ; Biodegradation ; Biomedical materials ; Cellulose ; Composite materials ; Composting ; Differential scanning calorimetry ; Experiments ; Fillers ; Flour ; Laboratories ; Mass spectrometry ; Materials selection ; Mechanical properties ; Nisin ; Plastics ; Polymers ; Recycled materials ; Thermogravimetric analysis ; Wood products</subject><ispartof>Materials, 2020-05, Vol.13 (9), p.2200</ispartof><rights>2020. This work is licensed under http://creativecommons.org/licenses/by/3.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><rights>2020 by the authors. 2020</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c406t-d5c207440a14923a2c46f3a534f5aadbaacc133198d77ae40c500896b2d6fa843</citedby><cites>FETCH-LOGICAL-c406t-d5c207440a14923a2c46f3a534f5aadbaacc133198d77ae40c500896b2d6fa843</cites><orcidid>0000-0003-3257-8803 ; 0000-0003-1177-985X ; 0000-0002-5015-4337 ; 0000-0002-8748-1649 ; 0000-0003-3972-7074</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC7254317/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC7254317/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,314,725,778,782,883,27911,27912,53778,53780</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/32403315$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Musioł, Marta</creatorcontrib><creatorcontrib>Jurczyk, Sebastian</creatorcontrib><creatorcontrib>Sobota, Michał</creatorcontrib><creatorcontrib>Klim, Magdalena</creatorcontrib><creatorcontrib>Sikorska, Wanda</creatorcontrib><creatorcontrib>Zięba, Magdalena</creatorcontrib><creatorcontrib>Janeczek, Henryk</creatorcontrib><creatorcontrib>Rydz, Joanna</creatorcontrib><creatorcontrib>Kurcok, Piotr</creatorcontrib><creatorcontrib>Johnston, Brian</creatorcontrib><creatorcontrib>Radecka, Izabela</creatorcontrib><title>(Bio)Degradable Polymeric Materials for Sustainable Future-Part 3: Degradation Studies of the PHA/Wood Flour-Based Composites and Preliminary Tests of Antimicrobial Activity</title><title>Materials</title><addtitle>Materials (Basel)</addtitle><description>The need for a cost reduction of the materials derived from (bio)degradable polymers forces research development into the formation of biocomposites with cheaper fillers. As additives can be made using the post-consumer wood, generated during wood products processing, re-use of recycled waste materials in the production of biocomposites can be an environmentally friendly way to minimalize and/or utilize the amount of the solid waste. Also, bioactive materials, which possess small amounts of antimicrobial additives belong to a very attractive packaging industry solution. This paper presents a study into the biodegradation, under laboratory composting conditions, of the composites that consist of poly[(
)-3-hydroxybutyrate-
-4-hydroxybutyrate)] and wood flour as a polymer matrix and natural filler, respectively. Thermogravimetric analysis, differential scanning calorimetry and scanning electron microscopy were used to evaluate the degradation progress of the obtained composites with different amounts of wood flour. The degradation products were characterized by multistage electrospray ionization mass spectrometry. Also, preliminary tests of the antimicrobial activity of selected materials with the addition of nisin were performed. The obtained results suggest that the different amount of filler has a significant influence on the degradation profile.</description><subject>Additives</subject><subject>Antiinfectives and antibacterials</subject><subject>Antimicrobial agents</subject><subject>Biocompatibility</subject><subject>Biodegradable materials</subject><subject>Biodegradation</subject><subject>Biomedical materials</subject><subject>Cellulose</subject><subject>Composite materials</subject><subject>Composting</subject><subject>Differential scanning calorimetry</subject><subject>Experiments</subject><subject>Fillers</subject><subject>Flour</subject><subject>Laboratories</subject><subject>Mass spectrometry</subject><subject>Materials selection</subject><subject>Mechanical properties</subject><subject>Nisin</subject><subject>Plastics</subject><subject>Polymers</subject><subject>Recycled materials</subject><subject>Thermogravimetric analysis</subject><subject>Wood products</subject><issn>1996-1944</issn><issn>1996-1944</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNpdkltrFDEUx4MottS--AEk4EtbGJvbXOKDsF1dK1RcaMXHcCbJtCkzkzXJFPZD-R3NbrcXzcvJ5Xf-_M85QegtJR84l-R0AMqJZIyQF2ifSlkVVArx8tl-Dx3GeEvy4pw2TL5Ge5yJzaHcR3-Ozpw__myvAxhoe4uXvl8PNjiNv0PKEfqIOx_w5RQTuHHLLKY0BVssISTMP-JddnJ-xJdpMs5G7DucbrLa-ez0l_cGL3o_heIMojV47oeVjy5lDEaDl8H2bsjSYY2vbEzb5NmY8p0Ovs0O8Ewnd-fS-g161WVD9nAXD9DPxZer-Xlx8ePrt_nsotCCVKkwpWakFoIAFZJxYFpUHYeSi64EMC2A1jTXLxtT12AF0SUhjaxaZqoOGsEP0Kd73dXUDtZoO6YAvVoFN2SXyoNT_76M7kZd-ztVs1JwWmeBo51A8L-nXJQaXNS272G0fopq03_C67rZoO__Q29zq8Zc3pZq8sgalqmTeyq3JMZgu0czlKjNR1BPHyHD757bf0Qfxs7_Ap4Ar9I</recordid><startdate>20200511</startdate><enddate>20200511</enddate><creator>Musioł, Marta</creator><creator>Jurczyk, Sebastian</creator><creator>Sobota, Michał</creator><creator>Klim, Magdalena</creator><creator>Sikorska, Wanda</creator><creator>Zięba, Magdalena</creator><creator>Janeczek, Henryk</creator><creator>Rydz, Joanna</creator><creator>Kurcok, Piotr</creator><creator>Johnston, Brian</creator><creator>Radecka, Izabela</creator><general>MDPI AG</general><general>MDPI</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>7X8</scope><scope>5PM</scope><orcidid>https://orcid.org/0000-0003-3257-8803</orcidid><orcidid>https://orcid.org/0000-0003-1177-985X</orcidid><orcidid>https://orcid.org/0000-0002-5015-4337</orcidid><orcidid>https://orcid.org/0000-0002-8748-1649</orcidid><orcidid>https://orcid.org/0000-0003-3972-7074</orcidid></search><sort><creationdate>20200511</creationdate><title>(Bio)Degradable Polymeric Materials for Sustainable Future-Part 3: Degradation Studies of the PHA/Wood Flour-Based Composites and Preliminary Tests of Antimicrobial Activity</title><author>Musioł, Marta ; 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As additives can be made using the post-consumer wood, generated during wood products processing, re-use of recycled waste materials in the production of biocomposites can be an environmentally friendly way to minimalize and/or utilize the amount of the solid waste. Also, bioactive materials, which possess small amounts of antimicrobial additives belong to a very attractive packaging industry solution. This paper presents a study into the biodegradation, under laboratory composting conditions, of the composites that consist of poly[(
)-3-hydroxybutyrate-
-4-hydroxybutyrate)] and wood flour as a polymer matrix and natural filler, respectively. Thermogravimetric analysis, differential scanning calorimetry and scanning electron microscopy were used to evaluate the degradation progress of the obtained composites with different amounts of wood flour. The degradation products were characterized by multistage electrospray ionization mass spectrometry. Also, preliminary tests of the antimicrobial activity of selected materials with the addition of nisin were performed. The obtained results suggest that the different amount of filler has a significant influence on the degradation profile.</abstract><cop>Switzerland</cop><pub>MDPI AG</pub><pmid>32403315</pmid><doi>10.3390/ma13092200</doi><orcidid>https://orcid.org/0000-0003-3257-8803</orcidid><orcidid>https://orcid.org/0000-0003-1177-985X</orcidid><orcidid>https://orcid.org/0000-0002-5015-4337</orcidid><orcidid>https://orcid.org/0000-0002-8748-1649</orcidid><orcidid>https://orcid.org/0000-0003-3972-7074</orcidid><oa>free_for_read</oa></addata></record> |
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| source | Elektronische Zeitschriftenbibliothek - Frei zugängliche E-Journals; PubMed Central Open Access; MDPI - Multidisciplinary Digital Publishing Institute; PubMed Central; Free Full-Text Journals in Chemistry |
| subjects | Additives Antiinfectives and antibacterials Antimicrobial agents Biocompatibility Biodegradable materials Biodegradation Biomedical materials Cellulose Composite materials Composting Differential scanning calorimetry Experiments Fillers Flour Laboratories Mass spectrometry Materials selection Mechanical properties Nisin Plastics Polymers Recycled materials Thermogravimetric analysis Wood products |
| title | (Bio)Degradable Polymeric Materials for Sustainable Future-Part 3: Degradation Studies of the PHA/Wood Flour-Based Composites and Preliminary Tests of Antimicrobial Activity |
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