Effect of Hybrid mono/bimetallic Nanocomposites for an enhancement of Catalytic and Antimicrobial Activities
Exploring the new catalytic systems for the reduction of organic and inorganic pollutants from an indispensable process in chemical, petrochemical, pharmaceutical and food industries, etc. Hence, in the present work, authors motivated to synthesize bare reduced graphene oxide (rGO), polyaniline (PAN...
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| Veröffentlicht in: | Scientific reports 2020-02, Vol.10 (1), p.2586, Article 2586 |
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| description | Exploring the new catalytic systems for the reduction of organic and inorganic pollutants from an indispensable process in chemical, petrochemical, pharmaceutical and food industries, etc. Hence, in the present work, authors motivated to synthesize bare reduced graphene oxide (rGO), polyaniline (PANI), three different ratios of rGO-PANI
(80:20,
50:50, 10:90)
composites and rGO-PANI
(80:20,
50:50, 10:90)
supported mono (Pd) & bimetallic [Pd: Au
(1:1,
1:2, 2:1)
] nanocomposite by a facile chemical reduction method. Also, it investigated their catalytic performances for the reduction of organic/inorganic pollutants and antimicrobial activities. All the freshly prepared bare rGO, PANI, three different ratios of rGO-PANI
(80:20, 50:50,
10:90)
composites and rGO-PANI
(80:20, 50:50,
10:90)
/Pd & Pd: Au
(1:1, 1:2,
2:1)
nanocomposite hybrid catalysts were characterized using UV-Vis, FT-IR, SEM, FE-SEM, EDAX, HR-TEM, XRD, XPS and Raman spectroscopy analysis. Among them, an optimized best composition of rGO-PANI
(80:20)
/Pd: Au
(1:1)
bimetallic nanocomposite hybrid catalyst exhibits better catalytic reduction and antimicrobial activities than other composites, as a result of strong electrostatic interactions between rGO, PANI and bimetal (Pd: Au) NPs through a synergistic effect. Hence, an optimized rGO-PANI
(80:20)
/Pd:Au
(1:1)
bimetallic nanocomposite catalyst would be considered as a suitable catalyst for the reduction of different nitroarenes, organic dyes, heavy metal ions and also significantly inhibit the growth of S. aureus, S. Typhi as well as Candida albicans and Candida kruesi in wastewater. |
| doi_str_mv | 10.1038/s41598-020-59491-5 |
| format | Article |
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(80:20,
50:50, 10:90)
composites and rGO-PANI
(80:20,
50:50, 10:90)
supported mono (Pd) & bimetallic [Pd: Au
(1:1,
1:2, 2:1)
] nanocomposite by a facile chemical reduction method. Also, it investigated their catalytic performances for the reduction of organic/inorganic pollutants and antimicrobial activities. All the freshly prepared bare rGO, PANI, three different ratios of rGO-PANI
(80:20, 50:50,
10:90)
composites and rGO-PANI
(80:20, 50:50,
10:90)
/Pd & Pd: Au
(1:1, 1:2,
2:1)
nanocomposite hybrid catalysts were characterized using UV-Vis, FT-IR, SEM, FE-SEM, EDAX, HR-TEM, XRD, XPS and Raman spectroscopy analysis. Among them, an optimized best composition of rGO-PANI
(80:20)
/Pd: Au
(1:1)
bimetallic nanocomposite hybrid catalyst exhibits better catalytic reduction and antimicrobial activities than other composites, as a result of strong electrostatic interactions between rGO, PANI and bimetal (Pd: Au) NPs through a synergistic effect. Hence, an optimized rGO-PANI
(80:20)
/Pd:Au
(1:1)
bimetallic nanocomposite catalyst would be considered as a suitable catalyst for the reduction of different nitroarenes, organic dyes, heavy metal ions and also significantly inhibit the growth of S. aureus, S. Typhi as well as Candida albicans and Candida kruesi in wastewater.</description><identifier>ISSN: 2045-2322</identifier><identifier>EISSN: 2045-2322</identifier><identifier>DOI: 10.1038/s41598-020-59491-5</identifier><identifier>PMID: 32054936</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>140/133 ; 140/146 ; 631/45/603 ; 639/925/918/1055 ; Aniline Compounds - chemistry ; Aniline Compounds - pharmacology ; Antimicrobial agents ; Bacteria - drug effects ; Catalysis ; Catalysts ; Chemical reduction ; Coloring Agents - isolation & purification ; Electrostatic properties ; Environmental Pollutants - isolation & purification ; Food industry ; Fungi - drug effects ; Gold - chemistry ; Gold - pharmacology ; Graphite - chemistry ; Graphite - pharmacology ; Heavy metals ; Humanities and Social Sciences ; Metal ions ; multidisciplinary ; Nanocomposites ; Nanocomposites - chemistry ; Nanocomposites - ultrastructure ; Nitro Compounds - isolation & purification ; Oxidation-Reduction ; Palladium - chemistry ; Palladium - pharmacology ; Petrochemicals ; Pollutants ; Raman spectroscopy ; Science ; Science (multidisciplinary) ; Synergistic effect ; Wastewater</subject><ispartof>Scientific reports, 2020-02, Vol.10 (1), p.2586, Article 2586</ispartof><rights>The Author(s) 2020</rights><rights>This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c511t-534f9065ac337a887e57a4b7c1fbbdd8ae57bcb1aa28202b8155747f464e1eb43</citedby><cites>FETCH-LOGICAL-c511t-534f9065ac337a887e57a4b7c1fbbdd8ae57bcb1aa28202b8155747f464e1eb43</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC7018773/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC7018773/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,314,727,780,784,864,885,27923,27924,41119,42188,51575,53790,53792</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/32054936$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Sivaranjan, Kuppan</creatorcontrib><creatorcontrib>Padmaraj, Osaimany</creatorcontrib><creatorcontrib>Santhanalakshmi, Jayadevan</creatorcontrib><creatorcontrib>Sathuvan, Malairaj</creatorcontrib><creatorcontrib>Sathiyaseelan, Anbazhagan</creatorcontrib><creatorcontrib>Sagadevan, Suresh</creatorcontrib><title>Effect of Hybrid mono/bimetallic Nanocomposites for an enhancement of Catalytic and Antimicrobial Activities</title><title>Scientific reports</title><addtitle>Sci Rep</addtitle><addtitle>Sci Rep</addtitle><description>Exploring the new catalytic systems for the reduction of organic and inorganic pollutants from an indispensable process in chemical, petrochemical, pharmaceutical and food industries, etc. Hence, in the present work, authors motivated to synthesize bare reduced graphene oxide (rGO), polyaniline (PANI), three different ratios of rGO-PANI
(80:20,
50:50, 10:90)
composites and rGO-PANI
(80:20,
50:50, 10:90)
supported mono (Pd) & bimetallic [Pd: Au
(1:1,
1:2, 2:1)
] nanocomposite by a facile chemical reduction method. Also, it investigated their catalytic performances for the reduction of organic/inorganic pollutants and antimicrobial activities. All the freshly prepared bare rGO, PANI, three different ratios of rGO-PANI
(80:20, 50:50,
10:90)
composites and rGO-PANI
(80:20, 50:50,
10:90)
/Pd & Pd: Au
(1:1, 1:2,
2:1)
nanocomposite hybrid catalysts were characterized using UV-Vis, FT-IR, SEM, FE-SEM, EDAX, HR-TEM, XRD, XPS and Raman spectroscopy analysis. Among them, an optimized best composition of rGO-PANI
(80:20)
/Pd: Au
(1:1)
bimetallic nanocomposite hybrid catalyst exhibits better catalytic reduction and antimicrobial activities than other composites, as a result of strong electrostatic interactions between rGO, PANI and bimetal (Pd: Au) NPs through a synergistic effect. Hence, an optimized rGO-PANI
(80:20)
/Pd:Au
(1:1)
bimetallic nanocomposite catalyst would be considered as a suitable catalyst for the reduction of different nitroarenes, organic dyes, heavy metal ions and also significantly inhibit the growth of S. aureus, S. Typhi as well as Candida albicans and Candida kruesi in wastewater.</description><subject>140/133</subject><subject>140/146</subject><subject>631/45/603</subject><subject>639/925/918/1055</subject><subject>Aniline Compounds - chemistry</subject><subject>Aniline Compounds - pharmacology</subject><subject>Antimicrobial agents</subject><subject>Bacteria - drug effects</subject><subject>Catalysis</subject><subject>Catalysts</subject><subject>Chemical reduction</subject><subject>Coloring Agents - isolation & purification</subject><subject>Electrostatic properties</subject><subject>Environmental Pollutants - isolation & purification</subject><subject>Food industry</subject><subject>Fungi - drug effects</subject><subject>Gold - chemistry</subject><subject>Gold - pharmacology</subject><subject>Graphite - chemistry</subject><subject>Graphite - pharmacology</subject><subject>Heavy metals</subject><subject>Humanities and Social Sciences</subject><subject>Metal ions</subject><subject>multidisciplinary</subject><subject>Nanocomposites</subject><subject>Nanocomposites - chemistry</subject><subject>Nanocomposites - ultrastructure</subject><subject>Nitro Compounds - isolation & purification</subject><subject>Oxidation-Reduction</subject><subject>Palladium - chemistry</subject><subject>Palladium - pharmacology</subject><subject>Petrochemicals</subject><subject>Pollutants</subject><subject>Raman spectroscopy</subject><subject>Science</subject><subject>Science (multidisciplinary)</subject><subject>Synergistic 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Catalytic and Antimicrobial Activities</title><author>Sivaranjan, Kuppan ; Padmaraj, Osaimany ; Santhanalakshmi, Jayadevan ; Sathuvan, Malairaj ; Sathiyaseelan, Anbazhagan ; Sagadevan, Suresh</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c511t-534f9065ac337a887e57a4b7c1fbbdd8ae57bcb1aa28202b8155747f464e1eb43</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>140/133</topic><topic>140/146</topic><topic>631/45/603</topic><topic>639/925/918/1055</topic><topic>Aniline Compounds - chemistry</topic><topic>Aniline Compounds - pharmacology</topic><topic>Antimicrobial agents</topic><topic>Bacteria - drug effects</topic><topic>Catalysis</topic><topic>Catalysts</topic><topic>Chemical reduction</topic><topic>Coloring Agents - isolation & purification</topic><topic>Electrostatic properties</topic><topic>Environmental Pollutants - isolation & purification</topic><topic>Food industry</topic><topic>Fungi - drug effects</topic><topic>Gold - chemistry</topic><topic>Gold - pharmacology</topic><topic>Graphite - chemistry</topic><topic>Graphite - pharmacology</topic><topic>Heavy metals</topic><topic>Humanities and Social Sciences</topic><topic>Metal ions</topic><topic>multidisciplinary</topic><topic>Nanocomposites</topic><topic>Nanocomposites - chemistry</topic><topic>Nanocomposites - ultrastructure</topic><topic>Nitro Compounds - isolation & purification</topic><topic>Oxidation-Reduction</topic><topic>Palladium - chemistry</topic><topic>Palladium - pharmacology</topic><topic>Petrochemicals</topic><topic>Pollutants</topic><topic>Raman spectroscopy</topic><topic>Science</topic><topic>Science (multidisciplinary)</topic><topic>Synergistic effect</topic><topic>Wastewater</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Sivaranjan, Kuppan</creatorcontrib><creatorcontrib>Padmaraj, Osaimany</creatorcontrib><creatorcontrib>Santhanalakshmi, Jayadevan</creatorcontrib><creatorcontrib>Sathuvan, Malairaj</creatorcontrib><creatorcontrib>Sathiyaseelan, Anbazhagan</creatorcontrib><creatorcontrib>Sagadevan, Suresh</creatorcontrib><collection>Springer Nature OA Free Journals</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Health & Medical Collection</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>Biology Database (Alumni Edition)</collection><collection>Medical Database (Alumni Edition)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Natural Science 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Suresh</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effect of Hybrid mono/bimetallic Nanocomposites for an enhancement of Catalytic and Antimicrobial Activities</atitle><jtitle>Scientific reports</jtitle><stitle>Sci Rep</stitle><addtitle>Sci Rep</addtitle><date>2020-02-13</date><risdate>2020</risdate><volume>10</volume><issue>1</issue><spage>2586</spage><pages>2586-</pages><artnum>2586</artnum><issn>2045-2322</issn><eissn>2045-2322</eissn><abstract>Exploring the new catalytic systems for the reduction of organic and inorganic pollutants from an indispensable process in chemical, petrochemical, pharmaceutical and food industries, etc. Hence, in the present work, authors motivated to synthesize bare reduced graphene oxide (rGO), polyaniline (PANI), three different ratios of rGO-PANI
(80:20,
50:50, 10:90)
composites and rGO-PANI
(80:20,
50:50, 10:90)
supported mono (Pd) & bimetallic [Pd: Au
(1:1,
1:2, 2:1)
] nanocomposite by a facile chemical reduction method. Also, it investigated their catalytic performances for the reduction of organic/inorganic pollutants and antimicrobial activities. All the freshly prepared bare rGO, PANI, three different ratios of rGO-PANI
(80:20, 50:50,
10:90)
composites and rGO-PANI
(80:20, 50:50,
10:90)
/Pd & Pd: Au
(1:1, 1:2,
2:1)
nanocomposite hybrid catalysts were characterized using UV-Vis, FT-IR, SEM, FE-SEM, EDAX, HR-TEM, XRD, XPS and Raman spectroscopy analysis. Among them, an optimized best composition of rGO-PANI
(80:20)
/Pd: Au
(1:1)
bimetallic nanocomposite hybrid catalyst exhibits better catalytic reduction and antimicrobial activities than other composites, as a result of strong electrostatic interactions between rGO, PANI and bimetal (Pd: Au) NPs through a synergistic effect. Hence, an optimized rGO-PANI
(80:20)
/Pd:Au
(1:1)
bimetallic nanocomposite catalyst would be considered as a suitable catalyst for the reduction of different nitroarenes, organic dyes, heavy metal ions and also significantly inhibit the growth of S. aureus, S. Typhi as well as Candida albicans and Candida kruesi in wastewater.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>32054936</pmid><doi>10.1038/s41598-020-59491-5</doi><oa>free_for_read</oa></addata></record> |
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| source | MEDLINE; DOAJ Directory of Open Access Journals; Springer Nature OA Free Journals; Nature Free; EZB-FREE-00999 freely available EZB journals; PubMed Central; Alma/SFX Local Collection; Free Full-Text Journals in Chemistry |
| subjects | 140/133 140/146 631/45/603 639/925/918/1055 Aniline Compounds - chemistry Aniline Compounds - pharmacology Antimicrobial agents Bacteria - drug effects Catalysis Catalysts Chemical reduction Coloring Agents - isolation & purification Electrostatic properties Environmental Pollutants - isolation & purification Food industry Fungi - drug effects Gold - chemistry Gold - pharmacology Graphite - chemistry Graphite - pharmacology Heavy metals Humanities and Social Sciences Metal ions multidisciplinary Nanocomposites Nanocomposites - chemistry Nanocomposites - ultrastructure Nitro Compounds - isolation & purification Oxidation-Reduction Palladium - chemistry Palladium - pharmacology Petrochemicals Pollutants Raman spectroscopy Science Science (multidisciplinary) Synergistic effect Wastewater |
| title | Effect of Hybrid mono/bimetallic Nanocomposites for an enhancement of Catalytic and Antimicrobial Activities |
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