Friction, Abrasion and Crack Growth Behavior of In-Situ and Ex-Situ Silica Filled Rubber Composites
The article focuses on comparing the friction, abrasion, and crack growth behavior of two different kinds of silica-filled tire tread compounds loaded with (a) in-situ generated alkoxide silica and (b) commercial precipitated silica-filled compounds. The rubber matrix consists of solution styrene bu...
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| Veröffentlicht in: | Materials 2020-01, Vol.13 (2), p.270 |
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| creator | Vaikuntam, Sankar Raman Bhagavatheswaran, Eshwaran Subramani Xiang, Fei Wießner, Sven Heinrich, Gert Das, Amit Stöckelhuber, Klaus Werner |
| description | The article focuses on comparing the friction, abrasion, and crack growth behavior of two different kinds of silica-filled tire tread compounds loaded with (a) in-situ generated alkoxide silica and (b) commercial precipitated silica-filled compounds. The rubber matrix consists of solution styrene butadiene rubber polymers (SSBR). The in-situ generated particles are entirely different in filler morphology, i.e., in terms of size and physical structure, when compared to the precipitated silica. However, both types of the silicas were identified as amorphous in nature. Influence of filler morphology and surface modification of silica on the end performances of the rubbers like dynamic friction, abrasion index, and fatigue crack propagation were investigated. Compared to precipitated silica composites, in-situ derived silica composites offer better abrasion behavior and improved crack propagation with and without admixture of silane coupling agents. Silane modification, particle morphology, and crosslink density were identified as further vital parameters influencing the investigated rubber properties. |
| doi_str_mv | 10.3390/ma13020270 |
| format | Article |
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The rubber matrix consists of solution styrene butadiene rubber polymers (SSBR). The in-situ generated particles are entirely different in filler morphology, i.e., in terms of size and physical structure, when compared to the precipitated silica. However, both types of the silicas were identified as amorphous in nature. Influence of filler morphology and surface modification of silica on the end performances of the rubbers like dynamic friction, abrasion index, and fatigue crack propagation were investigated. Compared to precipitated silica composites, in-situ derived silica composites offer better abrasion behavior and improved crack propagation with and without admixture of silane coupling agents. Silane modification, particle morphology, and crosslink density were identified as further vital parameters influencing the investigated rubber properties.</description><identifier>ISSN: 1996-1944</identifier><identifier>EISSN: 1996-1944</identifier><identifier>DOI: 10.3390/ma13020270</identifier><identifier>PMID: 31936164</identifier><language>eng</language><publisher>Switzerland: MDPI AG</publisher><subject>Abrasion ; Butadiene ; Carbon black ; Coupling agents ; Crack propagation ; Fatigue failure ; Fillers ; Friction ; Morphology ; Nanocomposites ; Parameter identification ; Particulate composites ; Polymers ; Rubber ; Rubber products ; Silanes ; Silicon dioxide ; Sulfur ; Working conditions ; Zinc oxides</subject><ispartof>Materials, 2020-01, Vol.13 (2), p.270</ispartof><rights>2020 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/). 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Silane modification, particle morphology, and crosslink density were identified as further vital parameters influencing the investigated rubber properties.</description><subject>Abrasion</subject><subject>Butadiene</subject><subject>Carbon black</subject><subject>Coupling agents</subject><subject>Crack propagation</subject><subject>Fatigue failure</subject><subject>Fillers</subject><subject>Friction</subject><subject>Morphology</subject><subject>Nanocomposites</subject><subject>Parameter identification</subject><subject>Particulate composites</subject><subject>Polymers</subject><subject>Rubber</subject><subject>Rubber products</subject><subject>Silanes</subject><subject>Silicon dioxide</subject><subject>Sulfur</subject><subject>Working conditions</subject><subject>Zinc oxides</subject><issn>1996-1944</issn><issn>1996-1944</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNpdkd1L5DAUxYO4qMz64h8gAV9E7G6-mqYvwjg4riAs-PEc0vTWibbNmLR-_PdGx3XV-3IP3B-HczkI7VDyi_OS_O4M5YQRVpA1tEXLUma0FGL9k95E2zHekjScU8XKDbTJackllWIL2XlwdnC-P8TTKpiYFDZ9jWfB2Dt8GvzjsMDHsDAPzgfsG3zWZ5duGN-gk6eVvnStswbPXdtCjS_GqoKAZ75b-ugGiD_Rj8a0Ebbf9wRdz0-uZn-y87-nZ7PpeWYFkUPGKlCSq5JVzKhG0aaidQWQKyisUlbavChyyWyu6hKY4JyBNY2oGYGak5zzCTpa-S7HqoPaQj8E0-plcJ0Jz9obp79eerfQN_5BF4QmuyIZ7L8bBH8_Qhx056KFtjU9-DFqxlM8VchCJHTvG3rrx9Cn9zTLhZIiZynSBB2sKBt8jAGajzCU6Nf69P_6Erz7Of4H-q8s_gIroZSD</recordid><startdate>20200107</startdate><enddate>20200107</enddate><creator>Vaikuntam, Sankar Raman</creator><creator>Bhagavatheswaran, Eshwaran Subramani</creator><creator>Xiang, Fei</creator><creator>Wießner, Sven</creator><creator>Heinrich, Gert</creator><creator>Das, Amit</creator><creator>Stöckelhuber, Klaus Werner</creator><general>MDPI AG</general><general>MDPI</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>7X8</scope><scope>5PM</scope><orcidid>https://orcid.org/0000-0002-1881-5799</orcidid><orcidid>https://orcid.org/0000-0002-2579-1369</orcidid><orcidid>https://orcid.org/0000-0003-4237-3617</orcidid><orcidid>https://orcid.org/0000-0003-0967-4557</orcidid></search><sort><creationdate>20200107</creationdate><title>Friction, Abrasion and Crack Growth Behavior of In-Situ and Ex-Situ Silica Filled Rubber Composites</title><author>Vaikuntam, Sankar Raman ; 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| source | Elektronische Zeitschriftenbibliothek - Frei zugängliche E-Journals; PubMed Central Open Access; MDPI - Multidisciplinary Digital Publishing Institute; PubMed Central; Free Full-Text Journals in Chemistry |
| subjects | Abrasion Butadiene Carbon black Coupling agents Crack propagation Fatigue failure Fillers Friction Morphology Nanocomposites Parameter identification Particulate composites Polymers Rubber Rubber products Silanes Silicon dioxide Sulfur Working conditions Zinc oxides |
| title | Friction, Abrasion and Crack Growth Behavior of In-Situ and Ex-Situ Silica Filled Rubber Composites |
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