Engineering opposite electronic polarization of singlet and triplet states increases the yield of high-energy photoproducts

Efficient photosynthetic energy conversion requires quantitative, light-driven formation of high-energy, charge-separated states. However, energies of high-lying excited states are rarely extracted, in part because the congested density of states in the excited-state manifold leads to rapid deactiva...

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Veröffentlicht in:Proceedings of the National Academy of Sciences - PNAS 2019-07, Vol.116 (29), p.14465-14470
Hauptverfasser: Polizzi, Nicholas F., Jiang, Ting, Beratan, David N., Therien, Michael J.
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Sprache:eng
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