Tip-enhanced strong coupling spectroscopy, imaging, and control of a single quantum emitter

Optical cavities can enhance and control light-matter interactions. This level of control has recently been extended to the nanoscale with single emitter strong coupling even at room temperature using plasmonic nanostructures. However, emitters in static geometries, limit the ability to tune the cou...

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Veröffentlicht in:Science advances 2019-07, Vol.5 (7), p.eaav5931
Hauptverfasser: Park, Kyoung-Duck, May, Molly A, Leng, Haixu, Wang, Jiarong, Kropp, Jaron A, Gougousi, Theodosia, Pelton, Matthew, Raschke, Markus B
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container_issue 7
container_start_page eaav5931
container_title Science advances
container_volume 5
creator Park, Kyoung-Duck
May, Molly A
Leng, Haixu
Wang, Jiarong
Kropp, Jaron A
Gougousi, Theodosia
Pelton, Matthew
Raschke, Markus B
description Optical cavities can enhance and control light-matter interactions. This level of control has recently been extended to the nanoscale with single emitter strong coupling even at room temperature using plasmonic nanostructures. However, emitters in static geometries, limit the ability to tune the coupling strength or to couple different emitters to the same cavity. Here, we present tip-enhanced strong coupling (TESC) with a nanocavity formed between a scanning plasmonic antenna tip and the substrate. By reversibly and dynamically addressing single quantum dots, we observe mode splitting up to 160 meV and anticrossing over a detuning range of ~100 meV, and with subnanometer precision over the deep subdiffraction-limited mode volume. Thus, TESC enables previously inaccessible control over emitter-nanocavity coupling and mode volume based on near-field microscopy. This opens pathways to induce, probe, and control single-emitter plasmon hybrid quantum states for applications from optoelectronics to quantum information science at room temperature.
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subjects Optics
SciAdv r-articles
title Tip-enhanced strong coupling spectroscopy, imaging, and control of a single quantum emitter
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