Ultra‐small‐angle X‐ray photon correlation spectroscopy using the Eiger detector
Successful implementation of the single‐photon‐counting Eiger 500k pixel array detector for sub‐millisecond X‐ray photon correlation spectroscopy (XPCS) measurements in the ultra‐small‐angle scattering region is reported. The performance is demonstrated by measuring the dynamics of dilute silica col...
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| Veröffentlicht in: | Journal of synchrotron radiation 2018-11, Vol.25 (6), p.1753-1759 |
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| container_title | Journal of synchrotron radiation |
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| creator | Zinn, T. Homs, A. Sharpnack, L. Tinti, G Fröjdh, E Douissard, P.-A. Kocsis, M. Möller, J. Chushkin, Y. Narayanan, T. |
| description | Successful implementation of the single‐photon‐counting Eiger 500k pixel array detector for sub‐millisecond X‐ray photon correlation spectroscopy (XPCS) measurements in the ultra‐small‐angle scattering region is reported. The performance is demonstrated by measuring the dynamics of dilute silica colloids in aqueous solvents when the detector is operated at different counter depths, 4, 8 and 12 bit. In the fastest mode involving 4 bit parallel readout, a stable frame rate of 22 kHz is obtained that enabled measurement of intensity–intensity autocorrelation functions with good statistics down to the 50 µs range for a sample with sufficient scattering power. The high frame rate and spatial resolution together with large number of pixels of the detector facilitate the investigation of sub‐millisecond dynamics over a broad length scale by multispeckle XPCS. This is illustrated by an example involving phoretic motion of colloids during the phase separation of the solvent.
The performance of the high‐resolution fast‐photon‐counting Eiger 500k detector for sub‐millisecond X‐ray photon correlation spectroscopy measurement is demonstrated. |
| doi_str_mv | 10.1107/S1600577518013899 |
| format | Article |
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The performance of the high‐resolution fast‐photon‐counting Eiger 500k detector for sub‐millisecond X‐ray photon correlation spectroscopy measurement is demonstrated.</description><identifier>ISSN: 1600-5775</identifier><identifier>ISSN: 0909-0495</identifier><identifier>EISSN: 1600-5775</identifier><identifier>DOI: 10.1107/S1600577518013899</identifier><identifier>PMID: 30407186</identifier><language>eng</language><publisher>5 Abbey Square, Chester, Cheshire CH1 2HU, England: International Union of Crystallography</publisher><subject>Autocorrelation functions ; coherent X‐ray scattering ; colloid dynamics ; Colloids ; Correlation analysis ; Phase separation ; Photon correlation spectroscopy ; Physics ; Pixels ; Research Papers ; Scattering ; Sensors ; Silica ; Silicon dioxide ; Solvents ; Spatial resolution ; Spectrum analysis ; USAXS ; X ray spectra ; XPCS</subject><ispartof>Journal of synchrotron radiation, 2018-11, Vol.25 (6), p.1753-1759</ispartof><rights>T. Zinn et al. 2018</rights><rights>open access.</rights><rights>Copyright Wiley Subscription Services, Inc. Nov 2018</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><rights>T. Zinn et al. 2018 2018</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c5597-773571c090a0e4ac708fc12d4941165cadd246e13f7c746afbc21276e7af314d3</citedby><cites>FETCH-LOGICAL-c5597-773571c090a0e4ac708fc12d4941165cadd246e13f7c746afbc21276e7af314d3</cites><orcidid>0000-0003-1957-1041 ; 0000-0003-2478-6063</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC6225738/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC6225738/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,314,723,776,780,881,1411,11541,27901,27902,45550,45551,46027,46451,53766,53768</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/30407186$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://hal.science/hal-02976415$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Zinn, T.</creatorcontrib><creatorcontrib>Homs, A.</creatorcontrib><creatorcontrib>Sharpnack, L.</creatorcontrib><creatorcontrib>Tinti, G</creatorcontrib><creatorcontrib>Fröjdh, E</creatorcontrib><creatorcontrib>Douissard, P.-A.</creatorcontrib><creatorcontrib>Kocsis, M.</creatorcontrib><creatorcontrib>Möller, J.</creatorcontrib><creatorcontrib>Chushkin, Y.</creatorcontrib><creatorcontrib>Narayanan, T.</creatorcontrib><title>Ultra‐small‐angle X‐ray photon correlation spectroscopy using the Eiger detector</title><title>Journal of synchrotron radiation</title><addtitle>J Synchrotron Radiat</addtitle><description>Successful implementation of the single‐photon‐counting Eiger 500k pixel array detector for sub‐millisecond X‐ray photon correlation spectroscopy (XPCS) measurements in the ultra‐small‐angle scattering region is reported. The performance is demonstrated by measuring the dynamics of dilute silica colloids in aqueous solvents when the detector is operated at different counter depths, 4, 8 and 12 bit. In the fastest mode involving 4 bit parallel readout, a stable frame rate of 22 kHz is obtained that enabled measurement of intensity–intensity autocorrelation functions with good statistics down to the 50 µs range for a sample with sufficient scattering power. The high frame rate and spatial resolution together with large number of pixels of the detector facilitate the investigation of sub‐millisecond dynamics over a broad length scale by multispeckle XPCS. This is illustrated by an example involving phoretic motion of colloids during the phase separation of the solvent.
The performance of the high‐resolution fast‐photon‐counting Eiger 500k detector for sub‐millisecond X‐ray photon correlation spectroscopy measurement is demonstrated.</description><subject>Autocorrelation functions</subject><subject>coherent X‐ray scattering</subject><subject>colloid dynamics</subject><subject>Colloids</subject><subject>Correlation analysis</subject><subject>Phase separation</subject><subject>Photon correlation spectroscopy</subject><subject>Physics</subject><subject>Pixels</subject><subject>Research Papers</subject><subject>Scattering</subject><subject>Sensors</subject><subject>Silica</subject><subject>Silicon dioxide</subject><subject>Solvents</subject><subject>Spatial resolution</subject><subject>Spectrum analysis</subject><subject>USAXS</subject><subject>X ray spectra</subject><subject>XPCS</subject><issn>1600-5775</issn><issn>0909-0495</issn><issn>1600-5775</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><sourceid>24P</sourceid><recordid>eNqFkc9O3DAQxq2qFf8foJcqUi_0sO2MHdvJpRIgCkUr9QBU7ckyjrMb5I2DnVDtjUfoM_IkOF1AFA6cPJr5zTee-Qh5j_AZEeSXUxQAXEqOBSAryvIN2RhTkzH39km8TjZjvARAISlbI-sMcpBYiA3y89z1Qd_e_I0L7Vx6dTtzNvuVoqCXWTf3vW8z40OwTvdNimNnTR98NL5bZkNs2lnWz2122MxsyCrbp6oP2-RdrV20O_fvFjn_dnh2cDyZ_jj6frA3nRjOSzmRknGJBkrQYHNtJBS1QVrlZY4ouNFVRXNhkdXSyFzo-sJQpFJYqWuGecW2yNeVbjdcLGxlbJu2caoLzUKHpfK6Uf9X2mauZv5aCUq5ZEUS-LQSmD9rO96bqjEHtJQiR36Nid29Hxb81WBjrxZNNNY53Vo_REWRIWUFAiT04zP00g-hTaf4R2EpCjEOxxVl0j1jsPXjDxDU6LB64XDq-fB048eOB0sTUK6AP42zy9cV1cnpb3q0zyGZcQc-2bPS</recordid><startdate>201811</startdate><enddate>201811</enddate><creator>Zinn, T.</creator><creator>Homs, A.</creator><creator>Sharpnack, L.</creator><creator>Tinti, G</creator><creator>Fröjdh, E</creator><creator>Douissard, P.-A.</creator><creator>Kocsis, M.</creator><creator>Möller, J.</creator><creator>Chushkin, Y.</creator><creator>Narayanan, T.</creator><general>International Union of Crystallography</general><general>John Wiley & Sons, Inc</general><scope>24P</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7U5</scope><scope>8FD</scope><scope>JQ2</scope><scope>L7M</scope><scope>7X8</scope><scope>1XC</scope><scope>VOOES</scope><scope>5PM</scope><orcidid>https://orcid.org/0000-0003-1957-1041</orcidid><orcidid>https://orcid.org/0000-0003-2478-6063</orcidid></search><sort><creationdate>201811</creationdate><title>Ultra‐small‐angle X‐ray photon correlation spectroscopy using the Eiger detector</title><author>Zinn, T. ; Homs, A. ; Sharpnack, L. ; Tinti, G ; Fröjdh, E ; Douissard, P.-A. ; Kocsis, M. ; Möller, J. ; Chushkin, Y. ; Narayanan, T.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c5597-773571c090a0e4ac708fc12d4941165cadd246e13f7c746afbc21276e7af314d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Autocorrelation functions</topic><topic>coherent X‐ray scattering</topic><topic>colloid dynamics</topic><topic>Colloids</topic><topic>Correlation analysis</topic><topic>Phase separation</topic><topic>Photon correlation spectroscopy</topic><topic>Physics</topic><topic>Pixels</topic><topic>Research Papers</topic><topic>Scattering</topic><topic>Sensors</topic><topic>Silica</topic><topic>Silicon dioxide</topic><topic>Solvents</topic><topic>Spatial resolution</topic><topic>Spectrum analysis</topic><topic>USAXS</topic><topic>X ray spectra</topic><topic>XPCS</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zinn, T.</creatorcontrib><creatorcontrib>Homs, A.</creatorcontrib><creatorcontrib>Sharpnack, L.</creatorcontrib><creatorcontrib>Tinti, G</creatorcontrib><creatorcontrib>Fröjdh, E</creatorcontrib><creatorcontrib>Douissard, P.-A.</creatorcontrib><creatorcontrib>Kocsis, M.</creatorcontrib><creatorcontrib>Möller, J.</creatorcontrib><creatorcontrib>Chushkin, Y.</creatorcontrib><creatorcontrib>Narayanan, T.</creatorcontrib><collection>Wiley Online Library Open Access</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>ProQuest Computer Science Collection</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><collection>Hyper Article en Ligne (HAL)</collection><collection>Hyper Article en Ligne (HAL) (Open Access)</collection><collection>PubMed Central (Full Participant titles)</collection><jtitle>Journal of synchrotron radiation</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zinn, T.</au><au>Homs, A.</au><au>Sharpnack, L.</au><au>Tinti, G</au><au>Fröjdh, E</au><au>Douissard, P.-A.</au><au>Kocsis, M.</au><au>Möller, J.</au><au>Chushkin, Y.</au><au>Narayanan, T.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Ultra‐small‐angle X‐ray photon correlation spectroscopy using the Eiger detector</atitle><jtitle>Journal of synchrotron radiation</jtitle><addtitle>J Synchrotron Radiat</addtitle><date>2018-11</date><risdate>2018</risdate><volume>25</volume><issue>6</issue><spage>1753</spage><epage>1759</epage><pages>1753-1759</pages><issn>1600-5775</issn><issn>0909-0495</issn><eissn>1600-5775</eissn><abstract>Successful implementation of the single‐photon‐counting Eiger 500k pixel array detector for sub‐millisecond X‐ray photon correlation spectroscopy (XPCS) measurements in the ultra‐small‐angle scattering region is reported. The performance is demonstrated by measuring the dynamics of dilute silica colloids in aqueous solvents when the detector is operated at different counter depths, 4, 8 and 12 bit. In the fastest mode involving 4 bit parallel readout, a stable frame rate of 22 kHz is obtained that enabled measurement of intensity–intensity autocorrelation functions with good statistics down to the 50 µs range for a sample with sufficient scattering power. The high frame rate and spatial resolution together with large number of pixels of the detector facilitate the investigation of sub‐millisecond dynamics over a broad length scale by multispeckle XPCS. This is illustrated by an example involving phoretic motion of colloids during the phase separation of the solvent.
The performance of the high‐resolution fast‐photon‐counting Eiger 500k detector for sub‐millisecond X‐ray photon correlation spectroscopy measurement is demonstrated.</abstract><cop>5 Abbey Square, Chester, Cheshire CH1 2HU, England</cop><pub>International Union of Crystallography</pub><pmid>30407186</pmid><doi>10.1107/S1600577518013899</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0003-1957-1041</orcidid><orcidid>https://orcid.org/0000-0003-2478-6063</orcidid><oa>free_for_read</oa></addata></record> |
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| source | Wiley Online Library Open Access; Wiley Online Library Journals Frontfile Complete; PubMed Central; Free Full-Text Journals in Chemistry |
| subjects | Autocorrelation functions coherent X‐ray scattering colloid dynamics Colloids Correlation analysis Phase separation Photon correlation spectroscopy Physics Pixels Research Papers Scattering Sensors Silica Silicon dioxide Solvents Spatial resolution Spectrum analysis USAXS X ray spectra XPCS |
| title | Ultra‐small‐angle X‐ray photon correlation spectroscopy using the Eiger detector |
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