Beyond fossil fuel-driven nitrogen transformations
Nitrogen is fundamental to all of life and many industrial processes. The interchange of nitrogen oxidation states in the industrial production of ammonia, nitric acid, and other commodity chemicals is largely powered by fossil fuels. A key goal of contemporary research in the field of nitrogen chem...
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| Veröffentlicht in: | Science (American Association for the Advancement of Science) 2018-05, Vol.360 (6391) |
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| creator | Chen, Jingguang G Crooks, Richard M Seefeldt, Lance C Bren, Kara L Bullock, R Morris Darensbourg, Marcetta Y Holland, Patrick L Hoffman, Brian Janik, Michael J Jones, Anne K Kanatzidis, Mercouri G King, Paul Lancaster, Kyle M Lymar, Sergei V Pfromm, Peter Schneider, William F Schrock, Richard R |
| description | Nitrogen is fundamental to all of life and many industrial processes. The interchange of nitrogen oxidation states in the industrial production of ammonia, nitric acid, and other commodity chemicals is largely powered by fossil fuels. A key goal of contemporary research in the field of nitrogen chemistry is to minimize the use of fossil fuels by developing more efficient heterogeneous, homogeneous, photo-, and electrocatalytic processes or by adapting the enzymatic processes underlying the natural nitrogen cycle. These approaches, as well as the challenges involved, are discussed in this Review. |
| doi_str_mv | 10.1126/science.aar6611 |
| format | Article |
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The interchange of nitrogen oxidation states in the industrial production of ammonia, nitric acid, and other commodity chemicals is largely powered by fossil fuels. A key goal of contemporary research in the field of nitrogen chemistry is to minimize the use of fossil fuels by developing more efficient heterogeneous, homogeneous, photo-, and electrocatalytic processes or by adapting the enzymatic processes underlying the natural nitrogen cycle. These approaches, as well as the challenges involved, are discussed in this Review.</description><identifier>ISSN: 0036-8075</identifier><identifier>EISSN: 1095-9203</identifier><identifier>DOI: 10.1126/science.aar6611</identifier><identifier>PMID: 29798857</identifier><language>eng</language><publisher>United States: The American Association for the Advancement of Science</publisher><subject>09 BIOMASS FUELS ; Acids ; Ammonia ; Atmospheric chemistry ; Automotive parts ; Benign ; Carbon ; Carbon dioxide ; Carbon dioxide emissions ; Catalysis ; Catalysts ; Catalytic converters ; Chemical industry ; Chemicals ; Chemistry ; Commodities ; Denitrification ; Efficiency ; Electrocatalysts ; Electrochemistry ; Emission control equipment ; Emissions ; Emissions control ; Energy consumption ; Energy conversion efficiency ; Energy efficiency ; Environmental changes ; Environmental degradation ; Environmental protection ; Enzymes ; Exhaust systems ; Fertilizers ; Fluidized bed combustion ; Fossil fuels ; Fuels ; Greenhouse effect ; Greenhouse gases ; Heavy metals ; Hydrocarbons ; Hydrogen ; Methane ; Molecular chains ; Nitric acid ; Nitrogen ; Nitrogen cycle ; Nitrogenase ; Organic Chemistry ; Ostwald ripening ; Oxidation ; Oxides ; Photochemicals ; Pollutants ; Polymers ; Steam ; Transformations</subject><ispartof>Science (American Association for the Advancement of Science), 2018-05, Vol.360 (6391)</ispartof><rights>Copyright © 2018 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works.</rights><rights>Copyright © 2018 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c514t-50a3f9078430eebb7d5d939cc28fcfc318837319a9c5af42c12c44fc2287c6783</citedby><cites>FETCH-LOGICAL-c514t-50a3f9078430eebb7d5d939cc28fcfc318837319a9c5af42c12c44fc2287c6783</cites><orcidid>0000-0001-7296-128X ; 0000-0001-6306-4851 ; 0000-0002-2883-2031 ; 0000-0003-2037-4168 ; 0000-0001-5827-3552 ; 0000-0001-5039-654X ; 0000-0003-2663-6157 ; 0000-0002-9592-2635 ; 0000-0002-6457-9504 ; 0000-0003-4025-4809 ; 0000-0002-3100-0746 ; 0000-0003-4869-9503 ; 0000-0001-5186-4878 ; 0000-0002-8082-3634 ; 0000-0003-0664-2138 ; 0000000228832031 ; 0000000340254809 ; 000000015039654X ; 0000000158273552 ; 0000000264579504 ; 000000017296128X ; 0000000231000746 ; 0000000320374168 ; 0000000306642138 ; 0000000163064851 ; 0000000326636157 ; 0000000295922635 ; 0000000280823634 ; 0000000151864878 ; 0000000348699503</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,776,780,881,2871,2872,27901,27902</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/29798857$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/servlets/purl/1440394$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Chen, Jingguang G</creatorcontrib><creatorcontrib>Crooks, Richard M</creatorcontrib><creatorcontrib>Seefeldt, Lance C</creatorcontrib><creatorcontrib>Bren, Kara L</creatorcontrib><creatorcontrib>Bullock, R Morris</creatorcontrib><creatorcontrib>Darensbourg, Marcetta Y</creatorcontrib><creatorcontrib>Holland, Patrick L</creatorcontrib><creatorcontrib>Hoffman, Brian</creatorcontrib><creatorcontrib>Janik, Michael J</creatorcontrib><creatorcontrib>Jones, Anne K</creatorcontrib><creatorcontrib>Kanatzidis, Mercouri G</creatorcontrib><creatorcontrib>King, Paul</creatorcontrib><creatorcontrib>Lancaster, Kyle M</creatorcontrib><creatorcontrib>Lymar, Sergei V</creatorcontrib><creatorcontrib>Pfromm, Peter</creatorcontrib><creatorcontrib>Schneider, William F</creatorcontrib><creatorcontrib>Schrock, Richard R</creatorcontrib><creatorcontrib>National Renewable Energy Laboratory (NREL), Golden, CO (United States)</creatorcontrib><title>Beyond fossil fuel-driven nitrogen transformations</title><title>Science (American Association for the Advancement of Science)</title><addtitle>Science</addtitle><description>Nitrogen is fundamental to all of life and many industrial processes. The interchange of nitrogen oxidation states in the industrial production of ammonia, nitric acid, and other commodity chemicals is largely powered by fossil fuels. A key goal of contemporary research in the field of nitrogen chemistry is to minimize the use of fossil fuels by developing more efficient heterogeneous, homogeneous, photo-, and electrocatalytic processes or by adapting the enzymatic processes underlying the natural nitrogen cycle. These approaches, as well as the challenges involved, are discussed in this Review.</description><subject>09 BIOMASS FUELS</subject><subject>Acids</subject><subject>Ammonia</subject><subject>Atmospheric chemistry</subject><subject>Automotive parts</subject><subject>Benign</subject><subject>Carbon</subject><subject>Carbon dioxide</subject><subject>Carbon dioxide emissions</subject><subject>Catalysis</subject><subject>Catalysts</subject><subject>Catalytic converters</subject><subject>Chemical industry</subject><subject>Chemicals</subject><subject>Chemistry</subject><subject>Commodities</subject><subject>Denitrification</subject><subject>Efficiency</subject><subject>Electrocatalysts</subject><subject>Electrochemistry</subject><subject>Emission control equipment</subject><subject>Emissions</subject><subject>Emissions control</subject><subject>Energy consumption</subject><subject>Energy conversion efficiency</subject><subject>Energy efficiency</subject><subject>Environmental changes</subject><subject>Environmental degradation</subject><subject>Environmental protection</subject><subject>Enzymes</subject><subject>Exhaust systems</subject><subject>Fertilizers</subject><subject>Fluidized bed combustion</subject><subject>Fossil fuels</subject><subject>Fuels</subject><subject>Greenhouse effect</subject><subject>Greenhouse gases</subject><subject>Heavy metals</subject><subject>Hydrocarbons</subject><subject>Hydrogen</subject><subject>Methane</subject><subject>Molecular chains</subject><subject>Nitric acid</subject><subject>Nitrogen</subject><subject>Nitrogen cycle</subject><subject>Nitrogenase</subject><subject>Organic Chemistry</subject><subject>Ostwald ripening</subject><subject>Oxidation</subject><subject>Oxides</subject><subject>Photochemicals</subject><subject>Pollutants</subject><subject>Polymers</subject><subject>Steam</subject><subject>Transformations</subject><issn>0036-8075</issn><issn>1095-9203</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNpdkc9rVDEQx4Modq2evcmiFy-vnfxOLkItagsFL-05ZOclbcrbpCbvFfrfm2XXop4yMJ_5Zub7JeQ9hRNKmTptmELGcOJ9VYrSF2RFwcrBMuAvyQqAq8GAlkfkTWv3AL1n-WtyxKy2xki9IuxreCp5XMfSWprWcQnTMNb0GPI6p7mW217M1ecWS936OZXc3pJX0U8tvDu8x-Tm-7fr84vh6uePy_OzqwElFfMgwfNoQRvBIYTNRo9ytNwiMhMxIqfGcM2p9Ralj4IhZShERMaMRqUNPyZf9roPy2YbRgy5LzK5h5q2vj654pP7t5PTnbstj06BMdqqLvBxL1DanFy3ag54hyXngLOjQgC3okOfD7_U8msJbXbb1DBMk8-hLM0xEJKDoiA7-uk_9L4sNXcPdhTXWmnYCZ7uKazd0xri88YU3C40dwjNHULrEx_-PvSZ_5MS_w0ozZTw</recordid><startdate>20180525</startdate><enddate>20180525</enddate><creator>Chen, Jingguang G</creator><creator>Crooks, Richard 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| fulltext | fulltext |
| identifier | ISSN: 0036-8075 |
| ispartof | Science (American Association for the Advancement of Science), 2018-05, Vol.360 (6391) |
| issn | 0036-8075 1095-9203 |
| language | eng |
| recordid | cdi_pubmedcentral_primary_oai_pubmedcentral_nih_gov_6088796 |
| source | American Association for the Advancement of Science; Jstor Complete Legacy |
| subjects | 09 BIOMASS FUELS Acids Ammonia Atmospheric chemistry Automotive parts Benign Carbon Carbon dioxide Carbon dioxide emissions Catalysis Catalysts Catalytic converters Chemical industry Chemicals Chemistry Commodities Denitrification Efficiency Electrocatalysts Electrochemistry Emission control equipment Emissions Emissions control Energy consumption Energy conversion efficiency Energy efficiency Environmental changes Environmental degradation Environmental protection Enzymes Exhaust systems Fertilizers Fluidized bed combustion Fossil fuels Fuels Greenhouse effect Greenhouse gases Heavy metals Hydrocarbons Hydrogen Methane Molecular chains Nitric acid Nitrogen Nitrogen cycle Nitrogenase Organic Chemistry Ostwald ripening Oxidation Oxides Photochemicals Pollutants Polymers Steam Transformations |
| title | Beyond fossil fuel-driven nitrogen transformations |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-08T12%3A47%3A14IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_pubme&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Beyond%20fossil%20fuel-driven%20nitrogen%20transformations&rft.jtitle=Science%20(American%20Association%20for%20the%20Advancement%20of%20Science)&rft.au=Chen,%20Jingguang%20G&rft.aucorp=National%20Renewable%20Energy%20Laboratory%20(NREL),%20Golden,%20CO%20(United%20States)&rft.date=2018-05-25&rft.volume=360&rft.issue=6391&rft.issn=0036-8075&rft.eissn=1095-9203&rft_id=info:doi/10.1126/science.aar6611&rft_dat=%3Cproquest_pubme%3E2045306105%3C/proquest_pubme%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2043776704&rft_id=info:pmid/29798857&rfr_iscdi=true |