Origin of magnetic properties in carbon implanted ZnO nanowires
Various synchrotron radiation-based spectroscopic and microscopic techniques are used to elucidate the room-temperature ferromagnetism of carbon-doped ZnO-nanowires (ZnO-C:NW) via a mild C + ion implantation method. The photoluminescence and magnetic hysteresis loops reveal that the implantation of...
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| creator | Wang, Y. F. Shao, Y. C. Hsieh, S. H. Chang, Y. K. Yeh, P. H. Hsueh, H. C. Chiou, J. W. Wang, H. T. Ray, S. C. Tsai, H. M. Pao, C. W. Chen, C. H. Lin, H. J. Lee, J. F. Wu, C. T. Wu, J. J. Chang, Y. M. Asokan, K. Chae, K. H. Ohigashi, T. Takagi, Y. Yokoyama, T. Kosugi, N. Pong, W. F. |
| description | Various synchrotron radiation-based spectroscopic and microscopic techniques are used to elucidate the room-temperature ferromagnetism of carbon-doped ZnO-nanowires (ZnO-C:NW) via a mild C
+
ion implantation method. The photoluminescence and magnetic hysteresis loops reveal that the implantation of C reduces the number of intrinsic surface defects and increases the saturated magnetization of ZnO-NW. The interstitial implanted C ions constitute the majority of defects in ZnO-C:NW as confirmed by the X-ray absorption spectroscopic studies. The X-ray magnetic circular dichroism spectra of O and C
K
-edge respectively indicate there is a reduction in the number of unpaired/dangling O 2
p
bonds in the surface region of ZnO-C:NW and the C 2
p
-derived states of the implanted C ions strongly affect the net spin polarization in the surface and bulk regions of ZnO-C:NW. Furthermore, these findings corroborate well with the first-principles calculations of C-implanted ZnO in surface and bulk regions, which highlight the stability of implanted C for the suppression and enhancement of the ferromagnetism of the ZnO-C:NW in the surface region and bulk phase, respectively. |
| doi_str_mv | 10.1038/s41598-018-25948-x |
| format | Article |
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+
ion implantation method. The photoluminescence and magnetic hysteresis loops reveal that the implantation of C reduces the number of intrinsic surface defects and increases the saturated magnetization of ZnO-NW. The interstitial implanted C ions constitute the majority of defects in ZnO-C:NW as confirmed by the X-ray absorption spectroscopic studies. The X-ray magnetic circular dichroism spectra of O and C
K
-edge respectively indicate there is a reduction in the number of unpaired/dangling O 2
p
bonds in the surface region of ZnO-C:NW and the C 2
p
-derived states of the implanted C ions strongly affect the net spin polarization in the surface and bulk regions of ZnO-C:NW. Furthermore, these findings corroborate well with the first-principles calculations of C-implanted ZnO in surface and bulk regions, which highlight the stability of implanted C for the suppression and enhancement of the ferromagnetism of the ZnO-C:NW in the surface region and bulk phase, respectively.</description><identifier>ISSN: 2045-2322</identifier><identifier>EISSN: 2045-2322</identifier><identifier>DOI: 10.1038/s41598-018-25948-x</identifier><identifier>PMID: 29773822</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>140/146 ; 639/301 ; 639/925/357 ; Circular dichroism ; Humanities and Social Sciences ; Magnetic properties ; Microscopes ; multidisciplinary ; Nanotechnology ; Photons ; Science ; Science (multidisciplinary)</subject><ispartof>Scientific reports, 2018-05, Vol.8 (1), p.7758-13, Article 7758</ispartof><rights>The Author(s) 2018</rights><rights>2018. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c540t-ef5b2cf756838d28f6738e2b1fe2885d2810d0d9cb8811b04f5eaf3472c856d23</citedby><cites>FETCH-LOGICAL-c540t-ef5b2cf756838d28f6738e2b1fe2885d2810d0d9cb8811b04f5eaf3472c856d23</cites><orcidid>0000-0003-3894-670X ; 0000-0001-5535-5878 ; 0000-0002-1602-765X ; 0000-0002-8475-7486</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC5958067/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC5958067/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,314,723,776,780,860,881,27901,27902,41096,42165,51551,53766,53768</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/29773822$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Wang, Y. F.</creatorcontrib><creatorcontrib>Shao, Y. C.</creatorcontrib><creatorcontrib>Hsieh, S. H.</creatorcontrib><creatorcontrib>Chang, Y. K.</creatorcontrib><creatorcontrib>Yeh, P. H.</creatorcontrib><creatorcontrib>Hsueh, H. C.</creatorcontrib><creatorcontrib>Chiou, J. W.</creatorcontrib><creatorcontrib>Wang, H. T.</creatorcontrib><creatorcontrib>Ray, S. C.</creatorcontrib><creatorcontrib>Tsai, H. M.</creatorcontrib><creatorcontrib>Pao, C. W.</creatorcontrib><creatorcontrib>Chen, C. H.</creatorcontrib><creatorcontrib>Lin, H. J.</creatorcontrib><creatorcontrib>Lee, J. F.</creatorcontrib><creatorcontrib>Wu, C. T.</creatorcontrib><creatorcontrib>Wu, J. J.</creatorcontrib><creatorcontrib>Chang, Y. M.</creatorcontrib><creatorcontrib>Asokan, K.</creatorcontrib><creatorcontrib>Chae, K. H.</creatorcontrib><creatorcontrib>Ohigashi, T.</creatorcontrib><creatorcontrib>Takagi, Y.</creatorcontrib><creatorcontrib>Yokoyama, T.</creatorcontrib><creatorcontrib>Kosugi, N.</creatorcontrib><creatorcontrib>Pong, W. F.</creatorcontrib><title>Origin of magnetic properties in carbon implanted ZnO nanowires</title><title>Scientific reports</title><addtitle>Sci Rep</addtitle><addtitle>Sci Rep</addtitle><description>Various synchrotron radiation-based spectroscopic and microscopic techniques are used to elucidate the room-temperature ferromagnetism of carbon-doped ZnO-nanowires (ZnO-C:NW) via a mild C
+
ion implantation method. The photoluminescence and magnetic hysteresis loops reveal that the implantation of C reduces the number of intrinsic surface defects and increases the saturated magnetization of ZnO-NW. The interstitial implanted C ions constitute the majority of defects in ZnO-C:NW as confirmed by the X-ray absorption spectroscopic studies. The X-ray magnetic circular dichroism spectra of O and C
K
-edge respectively indicate there is a reduction in the number of unpaired/dangling O 2
p
bonds in the surface region of ZnO-C:NW and the C 2
p
-derived states of the implanted C ions strongly affect the net spin polarization in the surface and bulk regions of ZnO-C:NW. Furthermore, these findings corroborate well with the first-principles calculations of C-implanted ZnO in surface and bulk regions, which highlight the stability of implanted C for the suppression and enhancement of the ferromagnetism of the ZnO-C:NW in the surface region and bulk phase, respectively.</description><subject>140/146</subject><subject>639/301</subject><subject>639/925/357</subject><subject>Circular dichroism</subject><subject>Humanities and Social Sciences</subject><subject>Magnetic properties</subject><subject>Microscopes</subject><subject>multidisciplinary</subject><subject>Nanotechnology</subject><subject>Photons</subject><subject>Science</subject><subject>Science (multidisciplinary)</subject><issn>2045-2322</issn><issn>2045-2322</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><sourceid>C6C</sourceid><sourceid>BENPR</sourceid><recordid>eNp9kTtPBCEUhYnRqFn9AxZmEhubUR7DDjQas_GVmGyjjQ1hmMuK2YERZn38e9H1XUgD4Xz3XC4HoR2CDwhm4jBVhEtRYiJKymUlyucVtElxxUvKKF39cd5A2ynd47w4lRWR62iDyrpmgtJNdDyNbuZ8EWzR6ZmHwZmij6GHODhIRVaMjk3whev6ufYDtMWtnxZe-_DkIqQttGb1PMH2xz5CN2en15OL8mp6fjk5uSoNr_BQguUNNbbmY8FES4Ud5_5AG2KBCsHzDcEtbqVphCCkwZXloC2ramoEH7eUjdDR0rdfNB20BvwQ9Vz10XU6vqignfqteHenZuFRcckFzt1GaP_DIIaHBaRBdS4ZmOehICySyt9FxoxILDO69we9D4vo83hvFK4rhqXIFF1SJoaUItivxxCs3iJSy4hUjki9R6Sec9HuzzG-Sj4DyQBbAilLfgbxu_c_tq_woZzG</recordid><startdate>20180517</startdate><enddate>20180517</enddate><creator>Wang, Y. F.</creator><creator>Shao, Y. C.</creator><creator>Hsieh, S. H.</creator><creator>Chang, Y. K.</creator><creator>Yeh, P. H.</creator><creator>Hsueh, H. C.</creator><creator>Chiou, J. W.</creator><creator>Wang, H. T.</creator><creator>Ray, S. C.</creator><creator>Tsai, H. M.</creator><creator>Pao, C. W.</creator><creator>Chen, C. H.</creator><creator>Lin, H. J.</creator><creator>Lee, J. F.</creator><creator>Wu, C. T.</creator><creator>Wu, J. J.</creator><creator>Chang, Y. M.</creator><creator>Asokan, K.</creator><creator>Chae, K. H.</creator><creator>Ohigashi, T.</creator><creator>Takagi, Y.</creator><creator>Yokoyama, T.</creator><creator>Kosugi, N.</creator><creator>Pong, W. 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F. ; Shao, Y. C. ; Hsieh, S. H. ; Chang, Y. K. ; Yeh, P. H. ; Hsueh, H. C. ; Chiou, J. W. ; Wang, H. T. ; Ray, S. C. ; Tsai, H. M. ; Pao, C. W. ; Chen, C. H. ; Lin, H. J. ; Lee, J. F. ; Wu, C. T. ; Wu, J. J. ; Chang, Y. M. ; Asokan, K. ; Chae, K. H. ; Ohigashi, T. ; Takagi, Y. ; Yokoyama, T. ; Kosugi, N. ; Pong, W. 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F.</au><au>Shao, Y. C.</au><au>Hsieh, S. H.</au><au>Chang, Y. K.</au><au>Yeh, P. H.</au><au>Hsueh, H. C.</au><au>Chiou, J. W.</au><au>Wang, H. T.</au><au>Ray, S. C.</au><au>Tsai, H. M.</au><au>Pao, C. W.</au><au>Chen, C. H.</au><au>Lin, H. J.</au><au>Lee, J. F.</au><au>Wu, C. T.</au><au>Wu, J. J.</au><au>Chang, Y. M.</au><au>Asokan, K.</au><au>Chae, K. H.</au><au>Ohigashi, T.</au><au>Takagi, Y.</au><au>Yokoyama, T.</au><au>Kosugi, N.</au><au>Pong, W. F.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Origin of magnetic properties in carbon implanted ZnO nanowires</atitle><jtitle>Scientific reports</jtitle><stitle>Sci Rep</stitle><addtitle>Sci Rep</addtitle><date>2018-05-17</date><risdate>2018</risdate><volume>8</volume><issue>1</issue><spage>7758</spage><epage>13</epage><pages>7758-13</pages><artnum>7758</artnum><issn>2045-2322</issn><eissn>2045-2322</eissn><abstract>Various synchrotron radiation-based spectroscopic and microscopic techniques are used to elucidate the room-temperature ferromagnetism of carbon-doped ZnO-nanowires (ZnO-C:NW) via a mild C
+
ion implantation method. The photoluminescence and magnetic hysteresis loops reveal that the implantation of C reduces the number of intrinsic surface defects and increases the saturated magnetization of ZnO-NW. The interstitial implanted C ions constitute the majority of defects in ZnO-C:NW as confirmed by the X-ray absorption spectroscopic studies. The X-ray magnetic circular dichroism spectra of O and C
K
-edge respectively indicate there is a reduction in the number of unpaired/dangling O 2
p
bonds in the surface region of ZnO-C:NW and the C 2
p
-derived states of the implanted C ions strongly affect the net spin polarization in the surface and bulk regions of ZnO-C:NW. Furthermore, these findings corroborate well with the first-principles calculations of C-implanted ZnO in surface and bulk regions, which highlight the stability of implanted C for the suppression and enhancement of the ferromagnetism of the ZnO-C:NW in the surface region and bulk phase, respectively.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>29773822</pmid><doi>10.1038/s41598-018-25948-x</doi><tpages>13</tpages><orcidid>https://orcid.org/0000-0003-3894-670X</orcidid><orcidid>https://orcid.org/0000-0001-5535-5878</orcidid><orcidid>https://orcid.org/0000-0002-1602-765X</orcidid><orcidid>https://orcid.org/0000-0002-8475-7486</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | 140/146 639/301 639/925/357 Circular dichroism Humanities and Social Sciences Magnetic properties Microscopes multidisciplinary Nanotechnology Photons Science Science (multidisciplinary) |
| title | Origin of magnetic properties in carbon implanted ZnO nanowires |
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