Towards Terawatt Sub-Cycle Long-Wave Infrared Pulses via Chirped Optical Parametric Amplification and Indirect Pulse Shaping

We present an approach for both efficient generation and amplification of 4–12  μ m pulses by tailoring the phase matching of the nonlinear crystal Zinc Germanium Phosphide (ZGP) in a narrowband-pumped optical parametric chirped pulse amplifier (OPCPA) and a broadband-pumped dual-chirped optical par...

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Veröffentlicht in:Scientific reports 2017-04, Vol.7 (1), p.45794-45794, Article 45794
Hauptverfasser: Yin, Yanchun, Chew, Andrew, Ren, Xiaoming, Li, Jie, Wang, Yang, Wu, Yi, Chang, Zenghu
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Chew, Andrew
Ren, Xiaoming
Li, Jie
Wang, Yang
Wu, Yi
Chang, Zenghu
description We present an approach for both efficient generation and amplification of 4–12  μ m pulses by tailoring the phase matching of the nonlinear crystal Zinc Germanium Phosphide (ZGP) in a narrowband-pumped optical parametric chirped pulse amplifier (OPCPA) and a broadband-pumped dual-chirped optical parametric amplifier (DC-OPA), respectively. Preliminary experimental results are obtained for generating 1.8–4.2  μ m super broadband spectra, which can be used to seed both the signal of the OPCPA and the pump of the DC-OPA. The theoretical pump-to-idler conversion efficiency reaches 27% in the DC-OPA pumped by a chirped broadband Cr 2+ :ZnSe/ZnS laser, enabling the generation of Terawatt-level 4–12  μ m pulses with an available large-aperture ZGP. Furthermore, the 4–12  μ m idler pulses can be compressed to sub-cycle pulses by compensating the tailored positive chirp of the idler pulses using the bulk compressor NaCl, and by indirectly controlling the higher-order idler phase through tuning the signal (2.4–4.0  μ m) phase with a commercially available acousto-optic programmable dispersive filter (AOPDF). A similar approach is also described for generating high-energy 4–12  μ m sub-cycle pulses via OPCPA pumped by a 2  μ m Ho:YLF laser.
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Preliminary experimental results are obtained for generating 1.8–4.2  μ m super broadband spectra, which can be used to seed both the signal of the OPCPA and the pump of the DC-OPA. The theoretical pump-to-idler conversion efficiency reaches 27% in the DC-OPA pumped by a chirped broadband Cr 2+ :ZnSe/ZnS laser, enabling the generation of Terawatt-level 4–12  μ m pulses with an available large-aperture ZGP. Furthermore, the 4–12  μ m idler pulses can be compressed to sub-cycle pulses by compensating the tailored positive chirp of the idler pulses using the bulk compressor NaCl, and by indirectly controlling the higher-order idler phase through tuning the signal (2.4–4.0  μ m) phase with a commercially available acousto-optic programmable dispersive filter (AOPDF). A similar approach is also described for generating high-energy 4–12  μ m sub-cycle pulses via OPCPA pumped by a 2  μ m Ho:YLF laser.</description><identifier>ISSN: 2045-2322</identifier><identifier>EISSN: 2045-2322</identifier><identifier>DOI: 10.1038/srep45794</identifier><identifier>PMID: 28367966</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>639/624/1020/1095 ; 639/624/400/385 ; Bandwidths ; Energy ; Germanium ; Humanities and Social Sciences ; Lasers ; multidisciplinary ; Optics ; Science ; Sodium chloride ; Spectrum allocation</subject><ispartof>Scientific reports, 2017-04, Vol.7 (1), p.45794-45794, Article 45794</ispartof><rights>The Author(s) 2017</rights><rights>Copyright Nature Publishing Group Apr 2017</rights><rights>Copyright © 2017, The Author(s) 2017 The Author(s)</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c504t-c33f200ac008be12cd18bd65b3f68dec4a7ce7241e7489b3d7ee87641169eb933</citedby><cites>FETCH-LOGICAL-c504t-c33f200ac008be12cd18bd65b3f68dec4a7ce7241e7489b3d7ee87641169eb933</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC5377938/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC5377938/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,314,727,780,784,864,885,27924,27925,41120,42189,51576,53791,53793</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/28367966$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Yin, Yanchun</creatorcontrib><creatorcontrib>Chew, Andrew</creatorcontrib><creatorcontrib>Ren, Xiaoming</creatorcontrib><creatorcontrib>Li, Jie</creatorcontrib><creatorcontrib>Wang, Yang</creatorcontrib><creatorcontrib>Wu, Yi</creatorcontrib><creatorcontrib>Chang, Zenghu</creatorcontrib><title>Towards Terawatt Sub-Cycle Long-Wave Infrared Pulses via Chirped Optical Parametric Amplification and Indirect Pulse Shaping</title><title>Scientific reports</title><addtitle>Sci Rep</addtitle><addtitle>Sci Rep</addtitle><description>We present an approach for both efficient generation and amplification of 4–12  μ m pulses by tailoring the phase matching of the nonlinear crystal Zinc Germanium Phosphide (ZGP) in a narrowband-pumped optical parametric chirped pulse amplifier (OPCPA) and a broadband-pumped dual-chirped optical parametric amplifier (DC-OPA), respectively. 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Preliminary experimental results are obtained for generating 1.8–4.2  μ m super broadband spectra, which can be used to seed both the signal of the OPCPA and the pump of the DC-OPA. The theoretical pump-to-idler conversion efficiency reaches 27% in the DC-OPA pumped by a chirped broadband Cr 2+ :ZnSe/ZnS laser, enabling the generation of Terawatt-level 4–12  μ m pulses with an available large-aperture ZGP. Furthermore, the 4–12  μ m idler pulses can be compressed to sub-cycle pulses by compensating the tailored positive chirp of the idler pulses using the bulk compressor NaCl, and by indirectly controlling the higher-order idler phase through tuning the signal (2.4–4.0  μ m) phase with a commercially available acousto-optic programmable dispersive filter (AOPDF). 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subjects 639/624/1020/1095
639/624/400/385
Bandwidths
Energy
Germanium
Humanities and Social Sciences
Lasers
multidisciplinary
Optics
Science
Sodium chloride
Spectrum allocation
title Towards Terawatt Sub-Cycle Long-Wave Infrared Pulses via Chirped Optical Parametric Amplification and Indirect Pulse Shaping
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