Verification measurements of the IRMM-1027 and the IAEA large-sized dried (LSD) spikes
In the frame of the accountancy measurements of the fissile materials, reliable determinations of the plutonium and uranium content in spent nuclear fuel are required to comply with international safeguards agreements. Large-sized dried (LSD) spikes of enriched 235 U and 239 Pu for isotope dilution...
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| Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2017-03, Vol.311 (3), p.1781-1791 |
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| container_title | Journal of radioanalytical and nuclear chemistry |
| container_volume | 311 |
| creator | Jakopič, R. Aregbe, Y. Richter, S. Zuleger, E. Mialle, S. Balsley, S. D. Repinc, U. Hiess, J. |
| description | In the frame of the accountancy measurements of the fissile materials, reliable determinations of the plutonium and uranium content in spent nuclear fuel are required to comply with international safeguards agreements. Large-sized dried (LSD) spikes of enriched
235
U and
239
Pu for isotope dilution mass spectrometry (IDMS) analysis are routinely applied in reprocessing plants for this purpose. A correct characterisation of these elements is a pre-requirement for achieving high accuracy in IDMS analyses. This paper will present the results of external verification measurements of such LSD spikes performed by the European Commission and the International Atomic Energy Agency. |
| doi_str_mv | 10.1007/s10967-016-5123-8 |
| format | Article |
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235
U and
239
Pu for isotope dilution mass spectrometry (IDMS) analysis are routinely applied in reprocessing plants for this purpose. A correct characterisation of these elements is a pre-requirement for achieving high accuracy in IDMS analyses. This paper will present the results of external verification measurements of such LSD spikes performed by the European Commission and the International Atomic Energy Agency.</description><identifier>ISSN: 0236-5731</identifier><identifier>EISSN: 1588-2780</identifier><identifier>DOI: 10.1007/s10967-016-5123-8</identifier><identifier>PMID: 28344376</identifier><language>eng</language><publisher>Dordrecht: Springer Netherlands</publisher><subject>Analysis ; Analytical chemistry ; Chemical Sciences ; Chemistry ; Chemistry and Materials Science ; Diagnostic Radiology ; Dilution ; Fissionable materials ; Hadrons ; Heavy Ions ; Inorganic Chemistry ; Mass spectrometry ; Measurement ; Nuclear Chemistry ; Nuclear electric power generation ; Nuclear energy ; Nuclear fuel reprocessing ; Nuclear fuels ; Nuclear industry ; Nuclear Physics ; Nuclear reactors ; Nuclear weapons ; Physical Chemistry ; Plutonium ; Spent nuclear fuels ; Spent reactor fuels ; Spikes ; Uranium</subject><ispartof>Journal of radioanalytical and nuclear chemistry, 2017-03, Vol.311 (3), p.1781-1791</ispartof><rights>The Author(s) 2016</rights><rights>COPYRIGHT 2017 Springer</rights><rights>Copyright Springer Science & Business Media 2017</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c642t-3fe391ac528cb68445913db943559682347979590ffbcb4cc71e0bab631c28183</citedby><cites>FETCH-LOGICAL-c642t-3fe391ac528cb68445913db943559682347979590ffbcb4cc71e0bab631c28183</cites><orcidid>0000-0002-6117-3955</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10967-016-5123-8$$EPDF$$P50$$Gspringer$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10967-016-5123-8$$EHTML$$P50$$Gspringer$$Hfree_for_read</linktohtml><link.rule.ids>230,314,776,780,881,27903,27904,41467,42536,51298</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/28344376$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://cea.hal.science/cea-04453342$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Jakopič, R.</creatorcontrib><creatorcontrib>Aregbe, Y.</creatorcontrib><creatorcontrib>Richter, S.</creatorcontrib><creatorcontrib>Zuleger, E.</creatorcontrib><creatorcontrib>Mialle, S.</creatorcontrib><creatorcontrib>Balsley, S. D.</creatorcontrib><creatorcontrib>Repinc, U.</creatorcontrib><creatorcontrib>Hiess, J.</creatorcontrib><title>Verification measurements of the IRMM-1027 and the IAEA large-sized dried (LSD) spikes</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><addtitle>J Radioanal Nucl Chem</addtitle><description>In the frame of the accountancy measurements of the fissile materials, reliable determinations of the plutonium and uranium content in spent nuclear fuel are required to comply with international safeguards agreements. Large-sized dried (LSD) spikes of enriched
235
U and
239
Pu for isotope dilution mass spectrometry (IDMS) analysis are routinely applied in reprocessing plants for this purpose. A correct characterisation of these elements is a pre-requirement for achieving high accuracy in IDMS analyses. This paper will present the results of external verification measurements of such LSD spikes performed by the European Commission and the International Atomic Energy Agency.</description><subject>Analysis</subject><subject>Analytical chemistry</subject><subject>Chemical Sciences</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Diagnostic Radiology</subject><subject>Dilution</subject><subject>Fissionable materials</subject><subject>Hadrons</subject><subject>Heavy Ions</subject><subject>Inorganic Chemistry</subject><subject>Mass spectrometry</subject><subject>Measurement</subject><subject>Nuclear Chemistry</subject><subject>Nuclear electric power generation</subject><subject>Nuclear energy</subject><subject>Nuclear fuel reprocessing</subject><subject>Nuclear fuels</subject><subject>Nuclear industry</subject><subject>Nuclear Physics</subject><subject>Nuclear reactors</subject><subject>Nuclear weapons</subject><subject>Physical Chemistry</subject><subject>Plutonium</subject><subject>Spent nuclear fuels</subject><subject>Spent reactor fuels</subject><subject>Spikes</subject><subject>Uranium</subject><issn>0236-5731</issn><issn>1588-2780</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><sourceid>C6C</sourceid><recordid>eNqNkl1rFTEQhhdR7LH6A7yRBW_ai62ZfGySG2Gp1RZOEfzobchmZ89J3Y_T5GxBf71ZtpZaECSQwMwzb2aGN8teAzkBQuS7CESXsiBQFgIoK9STbAVCqYJKRZ5mK0JZykgGB9mLGK8JIVop9jw7oIpxzmS5yq6uMPjWO7v345D3aOMUsMdhH_OxzfdbzC--XF4WQKjM7dAskeqsyjsbNlhE_wubvAk-3Ufrrx-O87jzPzC-zJ61tov46u49zL5_PPt2el6sP3-6OK3WhSs53ResRabBOkGVq0vFudDAmlpzJoQuFWVcaqmFJm1bu5o7JwFJbeuSgaMKFDvM3i-6u6nusXGp8WA7swu-t-GnGa03f2cGvzWb8dYIxkvgs8DxIrB9VHZerY1Da0hqijFObyGxR3efhfFmwrg3vY8Ou84OOE7RgNKgSg1S_geqgPM0MUvo20fo9TiFIW1tpogUjBKSqJOF2tgOjR_aMY3j0mmw924csPUpXglBNNec8FQAS4ELY4wB2_vpgJjZPWZxj0nuMbN7zLyMNw-3eV_xxy4JoAsQU2rYYHjQ6z9VfwOCeMrK</recordid><startdate>20170301</startdate><enddate>20170301</enddate><creator>Jakopič, R.</creator><creator>Aregbe, Y.</creator><creator>Richter, S.</creator><creator>Zuleger, E.</creator><creator>Mialle, S.</creator><creator>Balsley, S. D.</creator><creator>Repinc, U.</creator><creator>Hiess, J.</creator><general>Springer Netherlands</general><general>Springer</general><general>Springer Nature B.V</general><general>Springer Verlag</general><scope>C6C</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7ST</scope><scope>C1K</scope><scope>SOI</scope><scope>1XC</scope><scope>5PM</scope><orcidid>https://orcid.org/0000-0002-6117-3955</orcidid></search><sort><creationdate>20170301</creationdate><title>Verification measurements of the IRMM-1027 and the IAEA large-sized dried (LSD) spikes</title><author>Jakopič, R. ; Aregbe, Y. ; Richter, S. ; Zuleger, E. ; Mialle, S. ; Balsley, S. D. ; Repinc, U. ; Hiess, J.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c642t-3fe391ac528cb68445913db943559682347979590ffbcb4cc71e0bab631c28183</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><topic>Analysis</topic><topic>Analytical chemistry</topic><topic>Chemical Sciences</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Diagnostic Radiology</topic><topic>Dilution</topic><topic>Fissionable materials</topic><topic>Hadrons</topic><topic>Heavy Ions</topic><topic>Inorganic Chemistry</topic><topic>Mass spectrometry</topic><topic>Measurement</topic><topic>Nuclear Chemistry</topic><topic>Nuclear electric power generation</topic><topic>Nuclear energy</topic><topic>Nuclear fuel reprocessing</topic><topic>Nuclear fuels</topic><topic>Nuclear industry</topic><topic>Nuclear Physics</topic><topic>Nuclear reactors</topic><topic>Nuclear weapons</topic><topic>Physical Chemistry</topic><topic>Plutonium</topic><topic>Spent nuclear fuels</topic><topic>Spent reactor fuels</topic><topic>Spikes</topic><topic>Uranium</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Jakopič, R.</creatorcontrib><creatorcontrib>Aregbe, Y.</creatorcontrib><creatorcontrib>Richter, S.</creatorcontrib><creatorcontrib>Zuleger, E.</creatorcontrib><creatorcontrib>Mialle, S.</creatorcontrib><creatorcontrib>Balsley, S. 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235
U and
239
Pu for isotope dilution mass spectrometry (IDMS) analysis are routinely applied in reprocessing plants for this purpose. A correct characterisation of these elements is a pre-requirement for achieving high accuracy in IDMS analyses. This paper will present the results of external verification measurements of such LSD spikes performed by the European Commission and the International Atomic Energy Agency.</abstract><cop>Dordrecht</cop><pub>Springer Netherlands</pub><pmid>28344376</pmid><doi>10.1007/s10967-016-5123-8</doi><tpages>11</tpages><orcidid>https://orcid.org/0000-0002-6117-3955</orcidid><oa>free_for_read</oa></addata></record> |
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| source | Springer Nature - Complete Springer Journals |
| subjects | Analysis Analytical chemistry Chemical Sciences Chemistry Chemistry and Materials Science Diagnostic Radiology Dilution Fissionable materials Hadrons Heavy Ions Inorganic Chemistry Mass spectrometry Measurement Nuclear Chemistry Nuclear electric power generation Nuclear energy Nuclear fuel reprocessing Nuclear fuels Nuclear industry Nuclear Physics Nuclear reactors Nuclear weapons Physical Chemistry Plutonium Spent nuclear fuels Spent reactor fuels Spikes Uranium |
| title | Verification measurements of the IRMM-1027 and the IAEA large-sized dried (LSD) spikes |
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