Vertical Interface Induced Dielectric Relaxation in Nanocomposite (BaTiO3)1-x:(Sm2O3)x Thin Films

Vertical interfaces in vertically aligned nanocomposite thin films have been approved to be an effective method to manipulate functionalities. However, several challenges with regard to the understanding on the physical process underlying the manipulation still remain. In this work, because of the o...

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Veröffentlicht in:Scientific reports 2015-06, Vol.5 (1), p.11335-11335, Article 11335
Hauptverfasser: Li, Weiwei, Zhang, Wei, Wang, Le, Gu, Junxing, Chen, Aiping, Zhao, Run, Liang, Yan, Guo, Haizhong, Tang, Rujun, Wang, Chunchang, Jin, Kuijuan, Wang, Haiyan, Yang, Hao
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container_issue 1
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container_title Scientific reports
container_volume 5
creator Li, Weiwei
Zhang, Wei
Wang, Le
Gu, Junxing
Chen, Aiping
Zhao, Run
Liang, Yan
Guo, Haizhong
Tang, Rujun
Wang, Chunchang
Jin, Kuijuan
Wang, Haiyan
Yang, Hao
description Vertical interfaces in vertically aligned nanocomposite thin films have been approved to be an effective method to manipulate functionalities. However, several challenges with regard to the understanding on the physical process underlying the manipulation still remain. In this work, because of the ordered interfaces and large interfacial area, heteroepitaxial (BaTiO 3 ) 1-x :(Sm 2 O 3 ) x thin films have been fabricated and used as a model system to investigate the relationship between vertical interfaces and dielectric properties. Due to a relatively large strain generated at the interfaces, vertical interfaces between BaTiO 3 and Sm 2 O 3 are revealed to become the sinks to attract oxygen vacancies. The movement of oxygen vacancies is confined at the interfaces and hampered by the misfit dislocations, which contributed to a relaxation behavior in (BaTiO 3 ) 1-x :(Sm 2 O 3 ) x thin films. This work represents an approach to further understand that how interfaces influence on dielectric properties in oxide thin films.
doi_str_mv 10.1038/srep11335
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However, several challenges with regard to the understanding on the physical process underlying the manipulation still remain. In this work, because of the ordered interfaces and large interfacial area, heteroepitaxial (BaTiO 3 ) 1-x :(Sm 2 O 3 ) x thin films have been fabricated and used as a model system to investigate the relationship between vertical interfaces and dielectric properties. Due to a relatively large strain generated at the interfaces, vertical interfaces between BaTiO 3 and Sm 2 O 3 are revealed to become the sinks to attract oxygen vacancies. The movement of oxygen vacancies is confined at the interfaces and hampered by the misfit dislocations, which contributed to a relaxation behavior in (BaTiO 3 ) 1-x :(Sm 2 O 3 ) x thin films. 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subjects 639/301/119/996
639/766/119/996
Dielectric properties
Electrical properties
Humanities and Social Sciences
Interfaces
multidisciplinary
Nanocomposites
Oxygen
Science
Thin films
title Vertical Interface Induced Dielectric Relaxation in Nanocomposite (BaTiO3)1-x:(Sm2O3)x Thin Films
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