Quantification of strain and charge co-mediated magnetoelectric coupling on ultra-thin Permalloy/PMN-PT interface
Strain and charge co-mediated magnetoelectric coupling are expected in ultra-thin ferromagnetic/ferroelectric multiferroic heterostructures, which could lead to significantly enhanced magnetoelectric coupling. It is however challenging to observe the combined strain charge mediated magnetoelectric c...
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creator | Nan, Tianxiang Zhou, Ziyao Liu, Ming Yang, Xi Gao, Yuan Assaf, Badih A. Lin, Hwaider Velu, Siddharth Wang, Xinjun Luo, Haosu Chen, Jimmy Akhtar, Saad Hu, Edward Rajiv, Rohit Krishnan, Kavin Sreedhar, Shalini Heiman, Don Howe, Brandon M. Brown, Gail J. Sun, Nian X. |
description | Strain and charge co-mediated magnetoelectric coupling are expected in ultra-thin ferromagnetic/ferroelectric multiferroic heterostructures, which could lead to significantly enhanced magnetoelectric coupling. It is however challenging to observe the combined strain charge mediated magnetoelectric coupling and difficult in quantitatively distinguish these two magnetoelectric coupling mechanisms. We demonstrated in this work, the quantification of the coexistence of strain and surface charge mediated magnetoelectric coupling on ultra-thin Ni
0.79
Fe
0.21
/PMN-PT interface by using a Ni
0.79
Fe
0.21
/Cu/PMN-PT heterostructure with only strain-mediated magnetoelectric coupling as a control. The NiFe/PMN-PT heterostructure exhibited a high voltage induced effective magnetic field change of 375 Oe enhanced by the surface charge at the PMN-PT interface. Without the enhancement of the charge-mediated magnetoelectric effect by inserting a Cu layer at the PMN-PT interface, the electric field modification of effective magnetic field was 202 Oe. By distinguishing the magnetoelectric coupling mechanisms, a pure surface charge modification of magnetism shows a strong correlation to polarization of PMN-PT. A non-volatile effective magnetic field change of 104 Oe was observed at zero electric field originates from the different remnant polarization state of PMN-PT. The strain and charge co-mediated magnetoelectric coupling in ultra-thin magnetic/ferroelectric heterostructures could lead to power efficient and non-volatile magnetoelectric devices with enhanced magnetoelectric coupling. |
doi_str_mv | 10.1038/srep03688 |
format | Article |
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0.79
Fe
0.21
/PMN-PT interface by using a Ni
0.79
Fe
0.21
/Cu/PMN-PT heterostructure with only strain-mediated magnetoelectric coupling as a control. The NiFe/PMN-PT heterostructure exhibited a high voltage induced effective magnetic field change of 375 Oe enhanced by the surface charge at the PMN-PT interface. Without the enhancement of the charge-mediated magnetoelectric effect by inserting a Cu layer at the PMN-PT interface, the electric field modification of effective magnetic field was 202 Oe. By distinguishing the magnetoelectric coupling mechanisms, a pure surface charge modification of magnetism shows a strong correlation to polarization of PMN-PT. A non-volatile effective magnetic field change of 104 Oe was observed at zero electric field originates from the different remnant polarization state of PMN-PT. The strain and charge co-mediated magnetoelectric coupling in ultra-thin magnetic/ferroelectric heterostructures could lead to power efficient and non-volatile magnetoelectric devices with enhanced magnetoelectric coupling.</description><identifier>ISSN: 2045-2322</identifier><identifier>EISSN: 2045-2322</identifier><identifier>DOI: 10.1038/srep03688</identifier><identifier>PMID: 24418911</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>639/301/119/996 ; 639/301/119/997 ; Coexistence ; Electric fields ; High voltage ; Humanities and Social Sciences ; Magnetic fields ; Magnetism ; multidisciplinary ; Polarization ; Science ; Surface charge</subject><ispartof>Scientific reports, 2014-01, Vol.4 (1), p.3688-3688, Article 3688</ispartof><rights>The Author(s) 2014</rights><rights>Copyright Nature Publishing Group Jan 2014</rights><rights>Copyright © 2014, Macmillan Publishers Limited. All rights reserved 2014 Macmillan Publishers Limited. All rights reserved</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c504t-10dc13c9ae34d3eb8e4d6d4d8905c66015a71c15d67e95f78a1da6c5e0b8e9cb3</citedby><cites>FETCH-LOGICAL-c504t-10dc13c9ae34d3eb8e4d6d4d8905c66015a71c15d67e95f78a1da6c5e0b8e9cb3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC3891213/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC3891213/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,314,723,776,780,860,881,27903,27904,41099,42168,51554,53769,53771</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/24418911$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Nan, Tianxiang</creatorcontrib><creatorcontrib>Zhou, Ziyao</creatorcontrib><creatorcontrib>Liu, Ming</creatorcontrib><creatorcontrib>Yang, Xi</creatorcontrib><creatorcontrib>Gao, Yuan</creatorcontrib><creatorcontrib>Assaf, Badih A.</creatorcontrib><creatorcontrib>Lin, Hwaider</creatorcontrib><creatorcontrib>Velu, Siddharth</creatorcontrib><creatorcontrib>Wang, Xinjun</creatorcontrib><creatorcontrib>Luo, Haosu</creatorcontrib><creatorcontrib>Chen, Jimmy</creatorcontrib><creatorcontrib>Akhtar, Saad</creatorcontrib><creatorcontrib>Hu, Edward</creatorcontrib><creatorcontrib>Rajiv, Rohit</creatorcontrib><creatorcontrib>Krishnan, Kavin</creatorcontrib><creatorcontrib>Sreedhar, Shalini</creatorcontrib><creatorcontrib>Heiman, Don</creatorcontrib><creatorcontrib>Howe, Brandon M.</creatorcontrib><creatorcontrib>Brown, Gail J.</creatorcontrib><creatorcontrib>Sun, Nian X.</creatorcontrib><title>Quantification of strain and charge co-mediated magnetoelectric coupling on ultra-thin Permalloy/PMN-PT interface</title><title>Scientific reports</title><addtitle>Sci Rep</addtitle><addtitle>Sci Rep</addtitle><description>Strain and charge co-mediated magnetoelectric coupling are expected in ultra-thin ferromagnetic/ferroelectric multiferroic heterostructures, which could lead to significantly enhanced magnetoelectric coupling. It is however challenging to observe the combined strain charge mediated magnetoelectric coupling and difficult in quantitatively distinguish these two magnetoelectric coupling mechanisms. We demonstrated in this work, the quantification of the coexistence of strain and surface charge mediated magnetoelectric coupling on ultra-thin Ni
0.79
Fe
0.21
/PMN-PT interface by using a Ni
0.79
Fe
0.21
/Cu/PMN-PT heterostructure with only strain-mediated magnetoelectric coupling as a control. The NiFe/PMN-PT heterostructure exhibited a high voltage induced effective magnetic field change of 375 Oe enhanced by the surface charge at the PMN-PT interface. Without the enhancement of the charge-mediated magnetoelectric effect by inserting a Cu layer at the PMN-PT interface, the electric field modification of effective magnetic field was 202 Oe. By distinguishing the magnetoelectric coupling mechanisms, a pure surface charge modification of magnetism shows a strong correlation to polarization of PMN-PT. A non-volatile effective magnetic field change of 104 Oe was observed at zero electric field originates from the different remnant polarization state of PMN-PT. The strain and charge co-mediated magnetoelectric coupling in ultra-thin magnetic/ferroelectric heterostructures could lead to power efficient and non-volatile magnetoelectric devices with enhanced magnetoelectric coupling.</description><subject>639/301/119/996</subject><subject>639/301/119/997</subject><subject>Coexistence</subject><subject>Electric fields</subject><subject>High voltage</subject><subject>Humanities and Social Sciences</subject><subject>Magnetic fields</subject><subject>Magnetism</subject><subject>multidisciplinary</subject><subject>Polarization</subject><subject>Science</subject><subject>Surface 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charge</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Nan, Tianxiang</creatorcontrib><creatorcontrib>Zhou, Ziyao</creatorcontrib><creatorcontrib>Liu, Ming</creatorcontrib><creatorcontrib>Yang, Xi</creatorcontrib><creatorcontrib>Gao, Yuan</creatorcontrib><creatorcontrib>Assaf, Badih A.</creatorcontrib><creatorcontrib>Lin, Hwaider</creatorcontrib><creatorcontrib>Velu, Siddharth</creatorcontrib><creatorcontrib>Wang, Xinjun</creatorcontrib><creatorcontrib>Luo, Haosu</creatorcontrib><creatorcontrib>Chen, Jimmy</creatorcontrib><creatorcontrib>Akhtar, Saad</creatorcontrib><creatorcontrib>Hu, Edward</creatorcontrib><creatorcontrib>Rajiv, Rohit</creatorcontrib><creatorcontrib>Krishnan, Kavin</creatorcontrib><creatorcontrib>Sreedhar, Shalini</creatorcontrib><creatorcontrib>Heiman, Don</creatorcontrib><creatorcontrib>Howe, Brandon M.</creatorcontrib><creatorcontrib>Brown, Gail J.</creatorcontrib><creatorcontrib>Sun, Nian 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interface</atitle><jtitle>Scientific reports</jtitle><stitle>Sci Rep</stitle><addtitle>Sci Rep</addtitle><date>2014-01-14</date><risdate>2014</risdate><volume>4</volume><issue>1</issue><spage>3688</spage><epage>3688</epage><pages>3688-3688</pages><artnum>3688</artnum><issn>2045-2322</issn><eissn>2045-2322</eissn><abstract>Strain and charge co-mediated magnetoelectric coupling are expected in ultra-thin ferromagnetic/ferroelectric multiferroic heterostructures, which could lead to significantly enhanced magnetoelectric coupling. It is however challenging to observe the combined strain charge mediated magnetoelectric coupling and difficult in quantitatively distinguish these two magnetoelectric coupling mechanisms. We demonstrated in this work, the quantification of the coexistence of strain and surface charge mediated magnetoelectric coupling on ultra-thin Ni
0.79
Fe
0.21
/PMN-PT interface by using a Ni
0.79
Fe
0.21
/Cu/PMN-PT heterostructure with only strain-mediated magnetoelectric coupling as a control. The NiFe/PMN-PT heterostructure exhibited a high voltage induced effective magnetic field change of 375 Oe enhanced by the surface charge at the PMN-PT interface. Without the enhancement of the charge-mediated magnetoelectric effect by inserting a Cu layer at the PMN-PT interface, the electric field modification of effective magnetic field was 202 Oe. By distinguishing the magnetoelectric coupling mechanisms, a pure surface charge modification of magnetism shows a strong correlation to polarization of PMN-PT. A non-volatile effective magnetic field change of 104 Oe was observed at zero electric field originates from the different remnant polarization state of PMN-PT. The strain and charge co-mediated magnetoelectric coupling in ultra-thin magnetic/ferroelectric heterostructures could lead to power efficient and non-volatile magnetoelectric devices with enhanced magnetoelectric coupling.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>24418911</pmid><doi>10.1038/srep03688</doi><tpages>1</tpages><oa>free_for_read</oa></addata></record> |
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subjects | 639/301/119/996 639/301/119/997 Coexistence Electric fields High voltage Humanities and Social Sciences Magnetic fields Magnetism multidisciplinary Polarization Science Surface charge |
title | Quantification of strain and charge co-mediated magnetoelectric coupling on ultra-thin Permalloy/PMN-PT interface |
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