Characterization of particulate matter emission from open burning of rice straw

Emission from field burning of crop residue, a common practice in many parts of the world today, has potential effects on air quality, atmosphere and climate. This study provides a comprehensive size and compositional characterization of particulate matter (PM) emission from rice straw (RS) burning...

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Veröffentlicht in:Atmospheric environment (1994) 2011, Vol.45 (2), p.493-502
Hauptverfasser: Kim Oanh, Nguyen Thi, Ly, Bich Thuy, Tipayarom, Danutawat, Manandhar, Bhai Raja, Prapat, Pongkiatkul, Simpson, Christopher D., Sally Liu, L.-J.
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container_end_page 502
container_issue 2
container_start_page 493
container_title Atmospheric environment (1994)
container_volume 45
creator Kim Oanh, Nguyen Thi
Ly, Bich Thuy
Tipayarom, Danutawat
Manandhar, Bhai Raja
Prapat, Pongkiatkul
Simpson, Christopher D.
Sally Liu, L.-J.
description Emission from field burning of crop residue, a common practice in many parts of the world today, has potential effects on air quality, atmosphere and climate. This study provides a comprehensive size and compositional characterization of particulate matter (PM) emission from rice straw (RS) burning using both in situ experiments (11 spread field burning) and laboratory hood experiments (3 pile and 6 spread burning) that were conducted during 2003-2006 in Thailand. The carbon balance and emission ratio method was used to determine PM emission factors (EF) in the field experiments. The obtained EF varied from field to hood experiments reflecting multiple factors affecting combustion and emission. In the hood experiments, EF were found to be depending on the burning types (spread or pile), moisture content and the combustion efficiency. In addition, in the field experiments, burning rate and EF were also influenced by weather conditions, i.e. wind. Hood pile burning produced significantly higher EF (20 ± 8 g kg −1 RS) than hood spread burning (4.7 ± 2.2 g kg −1 RS). The majority of PM emitted from the field burning was PM 2.5 with EF of 5.1 ± 0.7 g m −2 or 8.3 ± 2.7 g kg −1 RS burned. The coarse PM fraction (PM 10–2.5) was mainly generated by fire attention activities and was relatively small, hence the resulting EF of PM 10 (9.4 ± 3.5 g kg −1 RS) was not significantly higher than PM 2.5. PM size distribution was measured across 8 size ranges (from 9.0 μm). The largest fractions of PM, EC and OC were associated with PM 1.1. The most significant components in PM 2.5 and PM 10 include OC, water soluble ions and levoglucosan. Relative abundance of some methoxyphenols (e.g., acetylsyringone), PAHs (e.g., fluoranthene and pyrene), organochlorine pesticides and PCBs may also serve as additional signatures for the PM emission. Presence of these toxic compounds in PM of burning smoke increases the potential toxic effects of the emission. For illustration, an estimation of the annual RS field burning in Thailand was made using the obtained in situ field burning EF and preliminary burning activity data.
doi_str_mv 10.1016/j.atmosenv.2010.09.023
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The majority of PM emitted from the field burning was PM 2.5 with EF of 5.1 ± 0.7 g m −2 or 8.3 ± 2.7 g kg −1 RS burned. The coarse PM fraction (PM 10–2.5) was mainly generated by fire attention activities and was relatively small, hence the resulting EF of PM 10 (9.4 ± 3.5 g kg −1 RS) was not significantly higher than PM 2.5. PM size distribution was measured across 8 size ranges (from &lt;0.4 μm to &gt;9.0 μm). The largest fractions of PM, EC and OC were associated with PM 1.1. The most significant components in PM 2.5 and PM 10 include OC, water soluble ions and levoglucosan. Relative abundance of some methoxyphenols (e.g., acetylsyringone), PAHs (e.g., fluoranthene and pyrene), organochlorine pesticides and PCBs may also serve as additional signatures for the PM emission. Presence of these toxic compounds in PM of burning smoke increases the potential toxic effects of the emission. 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source Elsevier ScienceDirect Journals
subjects air quality
Applied sciences
Atmospheric pollution
burning
carbon
climate
combustion
emissions factor
Exact sciences and technology
field experimentation
ions
laboratory experimentation
Levoglucosan
Methoxyphenols
organochlorine pesticides
Oryza sativa
particulate emissions
particulates
Pile burning
PM composition
Pollution
rice straw
Rice straw field burning
Semi-VOC
smoke
Thailand
toxicity
water content
weather
title Characterization of particulate matter emission from open burning of rice straw
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