In Situ Helium Isotope Microimaging of Meteorites
Isotope imaging is commonly used to investigate the localization of trace elements and their isotopes. In situ noble gas analysis of meteorites revealed the distribution of primordial noble gases that were trapped in the building blocks of asteroids and planets during the early stage of the solar sy...
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| Veröffentlicht in: | Analytical chemistry (Washington) 2024-04, Vol.96 (13), p.5143-5149 |
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| container_title | Analytical chemistry (Washington) |
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| creator | Bajo, Ken-ichi Kawasaki, Noriyuki Sakaguchi, Isao Suzuki, Taku T. Itose, Satoru Matsuya, Miyuki Ishihara, Morio Uchino, Kiichiro Yurimoto, Hisayoshi |
| description | Isotope imaging is commonly used to investigate the localization of trace elements and their isotopes. In situ noble gas analysis of meteorites revealed the distribution of primordial noble gases that were trapped in the building blocks of asteroids and planets during the early stage of the solar system evolution. Solar wind noble gases are among the primordial gases present in meteorites and were trapped through exposure to solar wind. Micrometer-resolution in situ noble gas analysis has not been achieved due to the lack of sensitivity and spatial resolution. The microscale imaging technique is crucial for identifying the carrier phase of the solar wind noble gases. We have developed 4He isotope imaging utilizing secondary neutral mass spectrometry with strong field postionization. This technique achieved a lateral resolution of 2 μm and a 4He detection limit of 2 × 1017 cm–3. This development allows for the study of a solar wind gas-rich meteorite, Northwest Africa 801 carbonaceous chondrite, with micrometer resolution. The solar wind 4He carriers are fine-grained particles and are sparsely scattered in the matrix region. |
| doi_str_mv | 10.1021/acs.analchem.3c05201 |
| format | Article |
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In situ noble gas analysis of meteorites revealed the distribution of primordial noble gases that were trapped in the building blocks of asteroids and planets during the early stage of the solar system evolution. Solar wind noble gases are among the primordial gases present in meteorites and were trapped through exposure to solar wind. Micrometer-resolution in situ noble gas analysis has not been achieved due to the lack of sensitivity and spatial resolution. The microscale imaging technique is crucial for identifying the carrier phase of the solar wind noble gases. We have developed 4He isotope imaging utilizing secondary neutral mass spectrometry with strong field postionization. This technique achieved a lateral resolution of 2 μm and a 4He detection limit of 2 × 1017 cm–3. This development allows for the study of a solar wind gas-rich meteorite, Northwest Africa 801 carbonaceous chondrite, with micrometer resolution. The solar wind 4He carriers are fine-grained particles and are sparsely scattered in the matrix region.</description><identifier>ISSN: 0003-2700</identifier><identifier>EISSN: 1520-6882</identifier><identifier>DOI: 10.1021/acs.analchem.3c05201</identifier><identifier>PMID: 38509446</identifier><language>eng</language><publisher>United States: American Chemical Society</publisher><subject>Asteroids ; Carbonaceous chondrites ; Gas analysis ; Gases ; Helium ; Helium isotopes ; Imaging techniques ; Isotopes ; Localization ; Mass spectrometry ; Mass spectroscopy ; Meteorites ; Meteors & meteorites ; Micrometers ; Planet formation ; Planetary evolution ; Rare gases ; Solar system ; Solar system evolution ; Solar wind ; Spatial discrimination ; Spatial resolution ; Trace elements</subject><ispartof>Analytical chemistry (Washington), 2024-04, Vol.96 (13), p.5143-5149</ispartof><rights>2024 American Chemical Society</rights><rights>Copyright American Chemical Society Apr 2, 2024</rights><rights>2024 American Chemical Society 2024 American Chemical Society</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-a447t-7eb401e936e26d1c28f1f46314627c25188432a66ae90cdeb35e294922095c273</cites><orcidid>0000-0002-9013-2730 ; 0000-0001-6041-4297</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acs.analchem.3c05201$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acs.analchem.3c05201$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>230,315,781,785,886,2766,27080,27928,27929,56742,56792</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/38509446$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Bajo, Ken-ichi</creatorcontrib><creatorcontrib>Kawasaki, Noriyuki</creatorcontrib><creatorcontrib>Sakaguchi, Isao</creatorcontrib><creatorcontrib>Suzuki, Taku T.</creatorcontrib><creatorcontrib>Itose, Satoru</creatorcontrib><creatorcontrib>Matsuya, Miyuki</creatorcontrib><creatorcontrib>Ishihara, Morio</creatorcontrib><creatorcontrib>Uchino, Kiichiro</creatorcontrib><creatorcontrib>Yurimoto, Hisayoshi</creatorcontrib><title>In Situ Helium Isotope Microimaging of Meteorites</title><title>Analytical chemistry (Washington)</title><addtitle>Anal. Chem</addtitle><description>Isotope imaging is commonly used to investigate the localization of trace elements and their isotopes. In situ noble gas analysis of meteorites revealed the distribution of primordial noble gases that were trapped in the building blocks of asteroids and planets during the early stage of the solar system evolution. Solar wind noble gases are among the primordial gases present in meteorites and were trapped through exposure to solar wind. Micrometer-resolution in situ noble gas analysis has not been achieved due to the lack of sensitivity and spatial resolution. The microscale imaging technique is crucial for identifying the carrier phase of the solar wind noble gases. We have developed 4He isotope imaging utilizing secondary neutral mass spectrometry with strong field postionization. This technique achieved a lateral resolution of 2 μm and a 4He detection limit of 2 × 1017 cm–3. This development allows for the study of a solar wind gas-rich meteorite, Northwest Africa 801 carbonaceous chondrite, with micrometer resolution. The solar wind 4He carriers are fine-grained particles and are sparsely scattered in the matrix region.</description><subject>Asteroids</subject><subject>Carbonaceous chondrites</subject><subject>Gas analysis</subject><subject>Gases</subject><subject>Helium</subject><subject>Helium isotopes</subject><subject>Imaging techniques</subject><subject>Isotopes</subject><subject>Localization</subject><subject>Mass spectrometry</subject><subject>Mass spectroscopy</subject><subject>Meteorites</subject><subject>Meteors & meteorites</subject><subject>Micrometers</subject><subject>Planet formation</subject><subject>Planetary evolution</subject><subject>Rare gases</subject><subject>Solar system</subject><subject>Solar system evolution</subject><subject>Solar wind</subject><subject>Spatial discrimination</subject><subject>Spatial resolution</subject><subject>Trace elements</subject><issn>0003-2700</issn><issn>1520-6882</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp9UcFu1DAQtRCoXUr_AKFIXLhkOzN27OSEUAV0pVYcgLPl9U62rpJ4iZNK_D1e7XYFHHqaw7z35s17QrxFWCIQXjmflm5wnb_nfik9VAT4Qiwwz1LXNb0UCwCQJRmAc_E6pQcAREB9Js5lXUGjlF4IXA3F9zDNxQ13Ye6LVYpT3HFxF_wYQ--2YdgWsS3ueOI4honTG_GqdV3iy-O8ED-_fP5xfVPefvu6uv50WzqlzFQaXitAbqRm0hv0VLfYKi1RaTKeKqxrJclp7bgBv-G1rJga1RBBU3ky8kJ8POju5nXPG8_DNLrO7sbsavxtowv2380Q7u02PlpETYS1zgofjgpj_DVzmmwfkueucwPHOVlqjMyBGKMy9P1_0Ic4jzndZCVIMlU2vbekDqicTUojtyc3CHZfis2l2KdS7LGUTHv39ycn0lMLGQAHwJ5-Ovys5h-Ke5mf</recordid><startdate>20240402</startdate><enddate>20240402</enddate><creator>Bajo, Ken-ichi</creator><creator>Kawasaki, Noriyuki</creator><creator>Sakaguchi, Isao</creator><creator>Suzuki, Taku T.</creator><creator>Itose, Satoru</creator><creator>Matsuya, Miyuki</creator><creator>Ishihara, Morio</creator><creator>Uchino, Kiichiro</creator><creator>Yurimoto, Hisayoshi</creator><general>American Chemical Society</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QF</scope><scope>7QO</scope><scope>7QQ</scope><scope>7SC</scope><scope>7SE</scope><scope>7SP</scope><scope>7SR</scope><scope>7TA</scope><scope>7TB</scope><scope>7TM</scope><scope>7U5</scope><scope>7U7</scope><scope>7U9</scope><scope>8BQ</scope><scope>8FD</scope><scope>C1K</scope><scope>F28</scope><scope>FR3</scope><scope>H8D</scope><scope>H8G</scope><scope>H94</scope><scope>JG9</scope><scope>JQ2</scope><scope>KR7</scope><scope>L7M</scope><scope>L~C</scope><scope>L~D</scope><scope>P64</scope><scope>7X8</scope><scope>5PM</scope><orcidid>https://orcid.org/0000-0002-9013-2730</orcidid><orcidid>https://orcid.org/0000-0001-6041-4297</orcidid></search><sort><creationdate>20240402</creationdate><title>In Situ Helium Isotope Microimaging of Meteorites</title><author>Bajo, Ken-ichi ; Kawasaki, Noriyuki ; Sakaguchi, Isao ; Suzuki, Taku T. ; Itose, Satoru ; Matsuya, Miyuki ; Ishihara, Morio ; Uchino, Kiichiro ; Yurimoto, Hisayoshi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a447t-7eb401e936e26d1c28f1f46314627c25188432a66ae90cdeb35e294922095c273</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Asteroids</topic><topic>Carbonaceous chondrites</topic><topic>Gas analysis</topic><topic>Gases</topic><topic>Helium</topic><topic>Helium isotopes</topic><topic>Imaging techniques</topic><topic>Isotopes</topic><topic>Localization</topic><topic>Mass spectrometry</topic><topic>Mass spectroscopy</topic><topic>Meteorites</topic><topic>Meteors & meteorites</topic><topic>Micrometers</topic><topic>Planet formation</topic><topic>Planetary evolution</topic><topic>Rare gases</topic><topic>Solar system</topic><topic>Solar system evolution</topic><topic>Solar wind</topic><topic>Spatial discrimination</topic><topic>Spatial resolution</topic><topic>Trace elements</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Bajo, Ken-ichi</creatorcontrib><creatorcontrib>Kawasaki, Noriyuki</creatorcontrib><creatorcontrib>Sakaguchi, Isao</creatorcontrib><creatorcontrib>Suzuki, Taku T.</creatorcontrib><creatorcontrib>Itose, Satoru</creatorcontrib><creatorcontrib>Matsuya, Miyuki</creatorcontrib><creatorcontrib>Ishihara, Morio</creatorcontrib><creatorcontrib>Uchino, Kiichiro</creatorcontrib><creatorcontrib>Yurimoto, Hisayoshi</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Aluminium Industry Abstracts</collection><collection>Biotechnology Research Abstracts</collection><collection>Ceramic Abstracts</collection><collection>Computer and Information Systems Abstracts</collection><collection>Corrosion Abstracts</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Materials Business File</collection><collection>Mechanical & Transportation Engineering Abstracts</collection><collection>Nucleic Acids Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Toxicology Abstracts</collection><collection>Virology and AIDS Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>Aerospace Database</collection><collection>Copper Technical Reference Library</collection><collection>AIDS and Cancer Research Abstracts</collection><collection>Materials Research Database</collection><collection>ProQuest Computer Science Collection</collection><collection>Civil Engineering Abstracts</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Computer and Information Systems Abstracts Academic</collection><collection>Computer and Information Systems Abstracts Professional</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>MEDLINE - Academic</collection><collection>PubMed Central (Full Participant titles)</collection><jtitle>Analytical chemistry (Washington)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Bajo, Ken-ichi</au><au>Kawasaki, Noriyuki</au><au>Sakaguchi, Isao</au><au>Suzuki, Taku T.</au><au>Itose, Satoru</au><au>Matsuya, Miyuki</au><au>Ishihara, Morio</au><au>Uchino, Kiichiro</au><au>Yurimoto, Hisayoshi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>In Situ Helium Isotope Microimaging of Meteorites</atitle><jtitle>Analytical chemistry (Washington)</jtitle><addtitle>Anal. Chem</addtitle><date>2024-04-02</date><risdate>2024</risdate><volume>96</volume><issue>13</issue><spage>5143</spage><epage>5149</epage><pages>5143-5149</pages><issn>0003-2700</issn><eissn>1520-6882</eissn><abstract>Isotope imaging is commonly used to investigate the localization of trace elements and their isotopes. In situ noble gas analysis of meteorites revealed the distribution of primordial noble gases that were trapped in the building blocks of asteroids and planets during the early stage of the solar system evolution. Solar wind noble gases are among the primordial gases present in meteorites and were trapped through exposure to solar wind. Micrometer-resolution in situ noble gas analysis has not been achieved due to the lack of sensitivity and spatial resolution. The microscale imaging technique is crucial for identifying the carrier phase of the solar wind noble gases. We have developed 4He isotope imaging utilizing secondary neutral mass spectrometry with strong field postionization. This technique achieved a lateral resolution of 2 μm and a 4He detection limit of 2 × 1017 cm–3. This development allows for the study of a solar wind gas-rich meteorite, Northwest Africa 801 carbonaceous chondrite, with micrometer resolution. The solar wind 4He carriers are fine-grained particles and are sparsely scattered in the matrix region.</abstract><cop>United States</cop><pub>American Chemical Society</pub><pmid>38509446</pmid><doi>10.1021/acs.analchem.3c05201</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0002-9013-2730</orcidid><orcidid>https://orcid.org/0000-0001-6041-4297</orcidid><oa>free_for_read</oa></addata></record> |
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| source | ACS Publications |
| subjects | Asteroids Carbonaceous chondrites Gas analysis Gases Helium Helium isotopes Imaging techniques Isotopes Localization Mass spectrometry Mass spectroscopy Meteorites Meteors & meteorites Micrometers Planet formation Planetary evolution Rare gases Solar system Solar system evolution Solar wind Spatial discrimination Spatial resolution Trace elements |
| title | In Situ Helium Isotope Microimaging of Meteorites |
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