Adsorption, Adhesion, and Wettability of Commercially Available Cleansers at Dental Polymer (PMMA) Surfaces
This study aims to evaluate the adsorptive, adhesive, and wetting energetic properties of five commercially available cleansers in contact with model dental polymer (PMMA). It was assumed that the selected parameters allow for determining the optimal concentration and place of key component accumula...
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| Veröffentlicht in: | Materials 2024-09, Vol.17 (19), p.4755 |
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| creator | Pogorzelski, Stanisław Janowicz, Paulina Dorywalski, Krzysztof Boniewicz-Szmyt, Katarzyna Rochowski, Paweł |
| description | This study aims to evaluate the adsorptive, adhesive, and wetting energetic properties of five commercially available cleansers in contact with model dental polymer (PMMA). It was assumed that the selected parameters allow for determining the optimal concentration and place of key component accumulation for antibacterial activity in the bulk liquid phase and prevention of oral plaque formation at the prosthetic material surface. The adsorptive (Gibbs' excesses
, critical micellar concentration) and thermal (entropy and enthalpy) surface characteristics originated from surface tension
and
dependences. The surface wetting properties were quantified upon the contact angle hysteresis formalism on the advancing
, receding
contact angles, and
as the input data, which yield a set of wettability parameters: 2D adsorptive film pressure, surface free energy with its dispersive and polar components, work of adhesion, and adhesional tension, considered as interfacial interaction indicators. In particular, molecular partitioning
and
are indicators of the efficiency of particular active substance accumulation in the volume phase, while
,
/
, and
point to the degree of its accumulation at the immersed polymer surface. Finally, the liquid penetration coefficient
and the Marangoni temperature gradient-driven liquid flow speed were estimated. |
| doi_str_mv | 10.3390/ma17194755 |
| format | Article |
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, critical micellar concentration) and thermal (entropy and enthalpy) surface characteristics originated from surface tension
and
dependences. The surface wetting properties were quantified upon the contact angle hysteresis formalism on the advancing
, receding
contact angles, and
as the input data, which yield a set of wettability parameters: 2D adsorptive film pressure, surface free energy with its dispersive and polar components, work of adhesion, and adhesional tension, considered as interfacial interaction indicators. In particular, molecular partitioning
and
are indicators of the efficiency of particular active substance accumulation in the volume phase, while
,
/
, and
point to the degree of its accumulation at the immersed polymer surface. Finally, the liquid penetration coefficient
and the Marangoni temperature gradient-driven liquid flow speed were estimated.</description><identifier>ISSN: 1996-1944</identifier><identifier>EISSN: 1996-1944</identifier><identifier>DOI: 10.3390/ma17194755</identifier><identifier>PMID: 39410331</identifier><language>eng</language><publisher>Switzerland: MDPI AG</publisher><subject>Accumulation ; Adhesion ; Adhesives ; Adsorption ; Adsorptivity ; Analysis ; Biofilms ; Blood vessels ; Cleaning compounds ; Contact angle ; Contact pressure ; Dental plaque ; Enthalpy ; Free energy ; Indicators ; Liquid flow ; Liquid phases ; Parameters ; Polymer industry ; Polymers ; Polymethyl methacrylate ; Prostheses ; Surface properties ; Surface tension ; Surfactants ; Viscosity ; Wettability ; Wetting</subject><ispartof>Materials, 2024-09, Vol.17 (19), p.4755</ispartof><rights>COPYRIGHT 2024 MDPI AG</rights><rights>2024 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><rights>2024 by the authors. 2024</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c335t-d0b63c7ce7f411128b80de068306ab0b7f5060e36db7777d9daeabc24ef89af43</cites><orcidid>0000-0003-1693-6623 ; 0000-0002-9433-2166</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC11477960/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC11477960/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,314,727,780,784,885,27924,27925,53791,53793</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/39410331$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Pogorzelski, Stanisław</creatorcontrib><creatorcontrib>Janowicz, Paulina</creatorcontrib><creatorcontrib>Dorywalski, Krzysztof</creatorcontrib><creatorcontrib>Boniewicz-Szmyt, Katarzyna</creatorcontrib><creatorcontrib>Rochowski, Paweł</creatorcontrib><title>Adsorption, Adhesion, and Wettability of Commercially Available Cleansers at Dental Polymer (PMMA) Surfaces</title><title>Materials</title><addtitle>Materials (Basel)</addtitle><description>This study aims to evaluate the adsorptive, adhesive, and wetting energetic properties of five commercially available cleansers in contact with model dental polymer (PMMA). It was assumed that the selected parameters allow for determining the optimal concentration and place of key component accumulation for antibacterial activity in the bulk liquid phase and prevention of oral plaque formation at the prosthetic material surface. The adsorptive (Gibbs' excesses
, critical micellar concentration) and thermal (entropy and enthalpy) surface characteristics originated from surface tension
and
dependences. The surface wetting properties were quantified upon the contact angle hysteresis formalism on the advancing
, receding
contact angles, and
as the input data, which yield a set of wettability parameters: 2D adsorptive film pressure, surface free energy with its dispersive and polar components, work of adhesion, and adhesional tension, considered as interfacial interaction indicators. In particular, molecular partitioning
and
are indicators of the efficiency of particular active substance accumulation in the volume phase, while
,
/
, and
point to the degree of its accumulation at the immersed polymer surface. Finally, the liquid penetration coefficient
and the Marangoni temperature gradient-driven liquid flow speed were estimated.</description><subject>Accumulation</subject><subject>Adhesion</subject><subject>Adhesives</subject><subject>Adsorption</subject><subject>Adsorptivity</subject><subject>Analysis</subject><subject>Biofilms</subject><subject>Blood vessels</subject><subject>Cleaning compounds</subject><subject>Contact angle</subject><subject>Contact pressure</subject><subject>Dental plaque</subject><subject>Enthalpy</subject><subject>Free energy</subject><subject>Indicators</subject><subject>Liquid flow</subject><subject>Liquid phases</subject><subject>Parameters</subject><subject>Polymer industry</subject><subject>Polymers</subject><subject>Polymethyl methacrylate</subject><subject>Prostheses</subject><subject>Surface properties</subject><subject>Surface tension</subject><subject>Surfactants</subject><subject>Viscosity</subject><subject>Wettability</subject><subject>Wetting</subject><issn>1996-1944</issn><issn>1996-1944</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNpdkd9vFCEQxzfGxjZtX_wDDIkv1XgVlj1Ynszm_NWkjU3U-EhmYWip7HLCbpP77-V6tVaHB2bgM9-ZyVTVc0ZPOVf07QBMMtXI5fJJdcCUEosSNU8f-fvVcc43tBjnrK3Vs2qfq4Zto4PqZ2dzTOvJx_EN6ew15jsPRkt-4DRB74OfNiQ6sorDgMl4CGFDulvwAfqAZBUQxowpE5jIexwnCOQyhk1hycnlxUX3inydkwOD-ajacxAyHt_fh9X3jx--rT4vzr98Olt15wvD-XJaWNoLbqRB6RrGWN32LbVIRcupgJ720i2poMiF7WUxqywg9KZu0LUKXMMPq3c73fXcD2hNaSpB0OvkB0gbHcHrf39Gf62v4q1mrJFSCVoUTu4VUvw1Y5704LPBEGDEOGfNGZNUtlzVBX35H3oT5zSW-baUEKLm7VbwdEddQUDtRxdLYVOOxcGbOKLz5b1rWcOVUFKWhNe7BJNizgndQ_uM6u3i9d_FF_jF44Ef0D9r5r8BN3eoQA</recordid><startdate>20240927</startdate><enddate>20240927</enddate><creator>Pogorzelski, Stanisław</creator><creator>Janowicz, Paulina</creator><creator>Dorywalski, Krzysztof</creator><creator>Boniewicz-Szmyt, Katarzyna</creator><creator>Rochowski, Paweł</creator><general>MDPI AG</general><general>MDPI</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>7X8</scope><scope>5PM</scope><orcidid>https://orcid.org/0000-0003-1693-6623</orcidid><orcidid>https://orcid.org/0000-0002-9433-2166</orcidid></search><sort><creationdate>20240927</creationdate><title>Adsorption, Adhesion, and Wettability of Commercially Available Cleansers at Dental Polymer (PMMA) Surfaces</title><author>Pogorzelski, Stanisław ; Janowicz, Paulina ; Dorywalski, Krzysztof ; Boniewicz-Szmyt, Katarzyna ; Rochowski, Paweł</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c335t-d0b63c7ce7f411128b80de068306ab0b7f5060e36db7777d9daeabc24ef89af43</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Accumulation</topic><topic>Adhesion</topic><topic>Adhesives</topic><topic>Adsorption</topic><topic>Adsorptivity</topic><topic>Analysis</topic><topic>Biofilms</topic><topic>Blood vessels</topic><topic>Cleaning compounds</topic><topic>Contact angle</topic><topic>Contact pressure</topic><topic>Dental plaque</topic><topic>Enthalpy</topic><topic>Free energy</topic><topic>Indicators</topic><topic>Liquid flow</topic><topic>Liquid phases</topic><topic>Parameters</topic><topic>Polymer industry</topic><topic>Polymers</topic><topic>Polymethyl methacrylate</topic><topic>Prostheses</topic><topic>Surface properties</topic><topic>Surface tension</topic><topic>Surfactants</topic><topic>Viscosity</topic><topic>Wettability</topic><topic>Wetting</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Pogorzelski, Stanisław</creatorcontrib><creatorcontrib>Janowicz, Paulina</creatorcontrib><creatorcontrib>Dorywalski, Krzysztof</creatorcontrib><creatorcontrib>Boniewicz-Szmyt, Katarzyna</creatorcontrib><creatorcontrib>Rochowski, Paweł</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>Materials Science Database</collection><collection>Materials Science Collection</collection><collection>Publicly Available Content Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>MEDLINE - Academic</collection><collection>PubMed Central (Full Participant titles)</collection><jtitle>Materials</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Pogorzelski, Stanisław</au><au>Janowicz, Paulina</au><au>Dorywalski, Krzysztof</au><au>Boniewicz-Szmyt, Katarzyna</au><au>Rochowski, Paweł</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Adsorption, Adhesion, and Wettability of Commercially Available Cleansers at Dental Polymer (PMMA) Surfaces</atitle><jtitle>Materials</jtitle><addtitle>Materials (Basel)</addtitle><date>2024-09-27</date><risdate>2024</risdate><volume>17</volume><issue>19</issue><spage>4755</spage><pages>4755-</pages><issn>1996-1944</issn><eissn>1996-1944</eissn><abstract>This study aims to evaluate the adsorptive, adhesive, and wetting energetic properties of five commercially available cleansers in contact with model dental polymer (PMMA). It was assumed that the selected parameters allow for determining the optimal concentration and place of key component accumulation for antibacterial activity in the bulk liquid phase and prevention of oral plaque formation at the prosthetic material surface. The adsorptive (Gibbs' excesses
, critical micellar concentration) and thermal (entropy and enthalpy) surface characteristics originated from surface tension
and
dependences. The surface wetting properties were quantified upon the contact angle hysteresis formalism on the advancing
, receding
contact angles, and
as the input data, which yield a set of wettability parameters: 2D adsorptive film pressure, surface free energy with its dispersive and polar components, work of adhesion, and adhesional tension, considered as interfacial interaction indicators. In particular, molecular partitioning
and
are indicators of the efficiency of particular active substance accumulation in the volume phase, while
,
/
, and
point to the degree of its accumulation at the immersed polymer surface. Finally, the liquid penetration coefficient
and the Marangoni temperature gradient-driven liquid flow speed were estimated.</abstract><cop>Switzerland</cop><pub>MDPI AG</pub><pmid>39410331</pmid><doi>10.3390/ma17194755</doi><orcidid>https://orcid.org/0000-0003-1693-6623</orcidid><orcidid>https://orcid.org/0000-0002-9433-2166</orcidid><oa>free_for_read</oa></addata></record> |
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| identifier | ISSN: 1996-1944 |
| ispartof | Materials, 2024-09, Vol.17 (19), p.4755 |
| issn | 1996-1944 1996-1944 |
| language | eng |
| recordid | cdi_pubmedcentral_primary_oai_pubmedcentral_nih_gov_11477960 |
| source | PubMed Central Open Access; MDPI - Multidisciplinary Digital Publishing Institute; EZB-FREE-00999 freely available EZB journals; PubMed Central; Free Full-Text Journals in Chemistry |
| subjects | Accumulation Adhesion Adhesives Adsorption Adsorptivity Analysis Biofilms Blood vessels Cleaning compounds Contact angle Contact pressure Dental plaque Enthalpy Free energy Indicators Liquid flow Liquid phases Parameters Polymer industry Polymers Polymethyl methacrylate Prostheses Surface properties Surface tension Surfactants Viscosity Wettability Wetting |
| title | Adsorption, Adhesion, and Wettability of Commercially Available Cleansers at Dental Polymer (PMMA) Surfaces |
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