Toward Complete All-Optical Intensity Modulation of High-Harmonic Generation from Solids

Optical modulation of high-harmonics generation in solids enables the detection of material properties, such as the band structure, and promising new applications, such as super-resolution imaging in semiconductors. Various recent studies have shown optical modulation of high-harmonics generation in...

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Veröffentlicht in:ACS photonics 2024-05, Vol.11 (5), p.1832-1843
Hauptverfasser: van Essen, Pieter J., Nie, Zhonghui, de Keijzer, Brian, Kraus, Peter M.
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creator van Essen, Pieter J.
Nie, Zhonghui
de Keijzer, Brian
Kraus, Peter M.
description Optical modulation of high-harmonics generation in solids enables the detection of material properties, such as the band structure, and promising new applications, such as super-resolution imaging in semiconductors. Various recent studies have shown optical modulation of high-harmonics generation in solids, in particular, suppression of high-harmonics generation has been observed by synchronized or delayed multipulse sequences. Here we provide an overview of the underlying mechanisms attributed to this suppression and provide a perspective on the challenges and opportunities regarding these mechanisms. All-optical control of high-harmonic generation allows for femtosecond, and in the future possibly subfemtosecond, switching, which has numerous possible applications: These range from super-resolution microscopy to nanoscale controlled chemistry and highly tunable nonlinear light sources.
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title Toward Complete All-Optical Intensity Modulation of High-Harmonic Generation from Solids
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