Electric and Magnetic Properties of the Multiferroic Composites Made Based on Pb(Fe1/2Nb1/2)1−xMnxO3 and the Nickel-Zinc Ferrite
This work presents the electrophysical properties of the multiferroic ceramic composites obtained as a result of combining both magnetic and ferroelectric material. The ferroelectric components of the composite are materials with the following chemical formulas: PbFe0.5Nb0.5O3 (PFN), Pb(Fe0.495Nb0.4...
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| description | This work presents the electrophysical properties of the multiferroic ceramic composites obtained as a result of combining both magnetic and ferroelectric material. The ferroelectric components of the composite are materials with the following chemical formulas: PbFe0.5Nb0.5O3 (PFN), Pb(Fe0.495Nb0.495Mn0.01)O3 (PFNM1), and Pb(Fe0.49Nb0.49Mn0.02)O3 (PFNM2), while the magnetic component of the composite is the nickel-zinc ferrite (Ni0.64Zn0.36Fe2O4 marked as F). The crystal structure, microstructure, DC electric conductivity, and ferroelectric, dielectric, magnetic, and piezoelectric properties of the multiferroic composites are performed. The conducted tests confirm that the composite samples have good dielectric and magnetic properties at room temperature. Multiferroic ceramic composites have a two-phase crystal structure (ferroelectric from a tetragonal system and magnetic from a spinel structure) without a foreign phase. Composites with an admixture of manganese have a better set of functional parameters. The manganese admixture increases the microstructure’s homogeneity, improves the magnetic properties, and reduces the electrical conductivity of composite samples. On the other hand, in the case of electric permittivity, a decrease in the maximum values of εm is observed with an increase in the amount of manganese in the ferroelectric component of composite compositions. However, the dielectric dispersion at high temperatures (associated with high conductivity) disappears. |
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The ferroelectric components of the composite are materials with the following chemical formulas: PbFe0.5Nb0.5O3 (PFN), Pb(Fe0.495Nb0.495Mn0.01)O3 (PFNM1), and Pb(Fe0.49Nb0.49Mn0.02)O3 (PFNM2), while the magnetic component of the composite is the nickel-zinc ferrite (Ni0.64Zn0.36Fe2O4 marked as F). The crystal structure, microstructure, DC electric conductivity, and ferroelectric, dielectric, magnetic, and piezoelectric properties of the multiferroic composites are performed. The conducted tests confirm that the composite samples have good dielectric and magnetic properties at room temperature. Multiferroic ceramic composites have a two-phase crystal structure (ferroelectric from a tetragonal system and magnetic from a spinel structure) without a foreign phase. Composites with an admixture of manganese have a better set of functional parameters. The manganese admixture increases the microstructure’s homogeneity, improves the magnetic properties, and reduces the electrical conductivity of composite samples. On the other hand, in the case of electric permittivity, a decrease in the maximum values of εm is observed with an increase in the amount of manganese in the ferroelectric component of composite compositions. However, the dielectric dispersion at high temperatures (associated with high conductivity) disappears.</description><identifier>ISSN: 1996-1944</identifier><identifier>EISSN: 1996-1944</identifier><identifier>DOI: 10.3390/ma16103785</identifier><identifier>PMID: 37241414</identifier><language>eng</language><publisher>Basel: MDPI AG</publisher><subject>Admixtures ; Composite materials ; Crystal structure ; Dielectric properties ; Electrical resistivity ; Ferroelectric materials ; Ferroelectricity ; Ferroelectrics ; Grain size ; High temperature ; Homogeneity ; Magnetic properties ; Manganese ; Microstructure ; Multiferroic materials ; Nickel ; Phase transitions ; Piezoelectricity ; Room temperature ; Zinc ferrites</subject><ispartof>Materials, 2023-05, Vol.16 (10), p.3785</ispartof><rights>2023 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). 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The ferroelectric components of the composite are materials with the following chemical formulas: PbFe0.5Nb0.5O3 (PFN), Pb(Fe0.495Nb0.495Mn0.01)O3 (PFNM1), and Pb(Fe0.49Nb0.49Mn0.02)O3 (PFNM2), while the magnetic component of the composite is the nickel-zinc ferrite (Ni0.64Zn0.36Fe2O4 marked as F). The crystal structure, microstructure, DC electric conductivity, and ferroelectric, dielectric, magnetic, and piezoelectric properties of the multiferroic composites are performed. The conducted tests confirm that the composite samples have good dielectric and magnetic properties at room temperature. Multiferroic ceramic composites have a two-phase crystal structure (ferroelectric from a tetragonal system and magnetic from a spinel structure) without a foreign phase. Composites with an admixture of manganese have a better set of functional parameters. The manganese admixture increases the microstructure’s homogeneity, improves the magnetic properties, and reduces the electrical conductivity of composite samples. On the other hand, in the case of electric permittivity, a decrease in the maximum values of εm is observed with an increase in the amount of manganese in the ferroelectric component of composite compositions. However, the dielectric dispersion at high temperatures (associated with high conductivity) disappears.</description><subject>Admixtures</subject><subject>Composite materials</subject><subject>Crystal structure</subject><subject>Dielectric properties</subject><subject>Electrical resistivity</subject><subject>Ferroelectric materials</subject><subject>Ferroelectricity</subject><subject>Ferroelectrics</subject><subject>Grain size</subject><subject>High temperature</subject><subject>Homogeneity</subject><subject>Magnetic properties</subject><subject>Manganese</subject><subject>Microstructure</subject><subject>Multiferroic materials</subject><subject>Nickel</subject><subject>Phase transitions</subject><subject>Piezoelectricity</subject><subject>Room temperature</subject><subject>Zinc ferrites</subject><issn>1996-1944</issn><issn>1996-1944</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNpdkc1u1TAQhS0EolXbDU9giU1BCvXYcRKvEFz1FqTetgvYsLF8nUnrktgX20Fly6rrPmKfBPdH_Hkke0bn6JNHh5AXwN4IodjBZKABJtpOPiHboFRTgarrp3_1W2QvpUtWjhDQcfWcbImW11Bqm_w8HNHm6Cw1vqcrc-4xl-Eshg3G7DDRMNB8gXQ1j9kNGGMo8iJMm5BcLvLK9Ejfm4Q9DZ6erfeXCAf8ZF2uV3B7fXO18len4p5-hzlx9iuO1RfnLV0WWmHskmeDGRPuPb475PPy8NPiQ3V8evRx8e64sqKrcwVWSsVFNwCTKFVvuRC8ZW1XdzUv-xjTKLBNx3vBxNr2Qzu0jENprJAMQeyQtw_czbyesLfoczSj3kQ3mfhDB-P0v4p3F_o8fNfAOOeS8ULYfyTE8G3GlPXkksVxNB7DnDTvOGNQK1DF-vI_62WYoy_7FVdJpZGNkMX1-sFlY0gp4vD7N8D0Xbz6T7ziF44ElLI</recordid><startdate>20230517</startdate><enddate>20230517</enddate><creator>Bochenek, Dariusz</creator><creator>Chrobak, Artur</creator><creator>Ziółkowski, Grzegorz</creator><general>MDPI AG</general><general>MDPI</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>7X8</scope><scope>5PM</scope><orcidid>https://orcid.org/0000-0002-6482-3319</orcidid><orcidid>https://orcid.org/0000-0003-0608-2505</orcidid><orcidid>https://orcid.org/0000-0003-4733-1846</orcidid></search><sort><creationdate>20230517</creationdate><title>Electric and Magnetic Properties of the Multiferroic Composites Made Based on Pb(Fe1/2Nb1/2)1−xMnxO3 and the Nickel-Zinc Ferrite</title><author>Bochenek, Dariusz ; Chrobak, Artur ; Ziółkowski, Grzegorz</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c384t-1c559238f105e59dc233270784842724aa691c682d303bcdf7f7021cdfc350e13</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Admixtures</topic><topic>Composite materials</topic><topic>Crystal structure</topic><topic>Dielectric properties</topic><topic>Electrical resistivity</topic><topic>Ferroelectric materials</topic><topic>Ferroelectricity</topic><topic>Ferroelectrics</topic><topic>Grain size</topic><topic>High temperature</topic><topic>Homogeneity</topic><topic>Magnetic properties</topic><topic>Manganese</topic><topic>Microstructure</topic><topic>Multiferroic materials</topic><topic>Nickel</topic><topic>Phase transitions</topic><topic>Piezoelectricity</topic><topic>Room temperature</topic><topic>Zinc ferrites</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Bochenek, Dariusz</creatorcontrib><creatorcontrib>Chrobak, Artur</creatorcontrib><creatorcontrib>Ziółkowski, Grzegorz</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni)</collection><collection>ProQuest Central</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>https://resources.nclive.org/materials</collection><collection>Materials science collection</collection><collection>Publicly Available Content Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>MEDLINE - Academic</collection><collection>PubMed Central (Full Participant titles)</collection><jtitle>Materials</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Bochenek, Dariusz</au><au>Chrobak, Artur</au><au>Ziółkowski, Grzegorz</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Electric and Magnetic Properties of the Multiferroic Composites Made Based on Pb(Fe1/2Nb1/2)1−xMnxO3 and the Nickel-Zinc Ferrite</atitle><jtitle>Materials</jtitle><date>2023-05-17</date><risdate>2023</risdate><volume>16</volume><issue>10</issue><spage>3785</spage><pages>3785-</pages><issn>1996-1944</issn><eissn>1996-1944</eissn><abstract>This work presents the electrophysical properties of the multiferroic ceramic composites obtained as a result of combining both magnetic and ferroelectric material. The ferroelectric components of the composite are materials with the following chemical formulas: PbFe0.5Nb0.5O3 (PFN), Pb(Fe0.495Nb0.495Mn0.01)O3 (PFNM1), and Pb(Fe0.49Nb0.49Mn0.02)O3 (PFNM2), while the magnetic component of the composite is the nickel-zinc ferrite (Ni0.64Zn0.36Fe2O4 marked as F). The crystal structure, microstructure, DC electric conductivity, and ferroelectric, dielectric, magnetic, and piezoelectric properties of the multiferroic composites are performed. The conducted tests confirm that the composite samples have good dielectric and magnetic properties at room temperature. Multiferroic ceramic composites have a two-phase crystal structure (ferroelectric from a tetragonal system and magnetic from a spinel structure) without a foreign phase. Composites with an admixture of manganese have a better set of functional parameters. The manganese admixture increases the microstructure’s homogeneity, improves the magnetic properties, and reduces the electrical conductivity of composite samples. On the other hand, in the case of electric permittivity, a decrease in the maximum values of εm is observed with an increase in the amount of manganese in the ferroelectric component of composite compositions. However, the dielectric dispersion at high temperatures (associated with high conductivity) disappears.</abstract><cop>Basel</cop><pub>MDPI AG</pub><pmid>37241414</pmid><doi>10.3390/ma16103785</doi><orcidid>https://orcid.org/0000-0002-6482-3319</orcidid><orcidid>https://orcid.org/0000-0003-0608-2505</orcidid><orcidid>https://orcid.org/0000-0003-4733-1846</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | Admixtures Composite materials Crystal structure Dielectric properties Electrical resistivity Ferroelectric materials Ferroelectricity Ferroelectrics Grain size High temperature Homogeneity Magnetic properties Manganese Microstructure Multiferroic materials Nickel Phase transitions Piezoelectricity Room temperature Zinc ferrites |
| title | Electric and Magnetic Properties of the Multiferroic Composites Made Based on Pb(Fe1/2Nb1/2)1−xMnxO3 and the Nickel-Zinc Ferrite |
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