Toward ultrafast soft x-ray spectroscopy of organic photovoltaic devices
Novel ultrafast x-ray sources based on high harmonic generation and at x-ray free electron lasers are opening up new opportunities to resolve complex ultrafast processes in condensed phase systems with exceptional temporal resolution and atomic site specificity. In this perspective, we present techn...
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| Veröffentlicht in: | Structural dynamics (Melville, N.Y.) N.Y.), 2024-01, Vol.11 (1), p.010901-010901 |
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| creator | Garratt, Douglas Matthews, Mary Marangos, Jon |
| description | Novel ultrafast x-ray sources based on high harmonic generation and at x-ray free electron lasers are opening up new opportunities to resolve complex ultrafast processes in condensed phase systems with exceptional temporal resolution and atomic site specificity. In this perspective, we present techniques for resolving charge localization, transfer, and separation processes in organic semiconductors and organic photovoltaic devices with time-resolved soft x-ray spectroscopy. We review recent results in ultrafast soft x-ray spectroscopy of these systems and discuss routes to overcome the technical challenges in performing time-resolved x-ray experiments on photosensitive materials with poor thermal conductivity and low pump intensity thresholds for nonlinear effects. |
| doi_str_mv | 10.1063/4.0000214 |
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| source | DOAJ Directory of Open Access Journals; Elektronische Zeitschriftenbibliothek - Frei zugängliche E-Journals; PubMed Central |
| subjects | Carbon Charge transfer Efficiency Electrons Free electron lasers Harmonic generations INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY Nitrogen Organic semiconductors Photosensitivity Photovoltaic cells s (Invited) Semiconductors Soft X ray spectroscopy Soft x rays Solar energy Spectrum analysis Temporal resolution Thermal conductivity X ray sources |
| title | Toward ultrafast soft x-ray spectroscopy of organic photovoltaic devices |
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