Photonic enhancement in photoluminescent metal halide perovskite-photonic crystal bead hybrids
We report two photonic crystal-perovskite nanocrystal microbead hybrids with photoluminescence matching that of the parent nanocrystals but with increased photoluminescence quantum yields. Time-resolved photoluminescence spectroscopy quantifies the radiative enhancement afforded by the photonic envi...
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Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2023-08, Vol.59 (69), p.138-1383 |
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creator | Lapointe, Victoria Imperiale, Christian J Chengadu, Sollavi Pomilio, Cristina M Ganesh, Meera Kéna-Cohen, Stephane Majewski, Marek B |
description | We report two photonic crystal-perovskite nanocrystal microbead hybrids with photoluminescence matching that of the parent nanocrystals but with increased photoluminescence quantum yields. Time-resolved photoluminescence spectroscopy quantifies the radiative enhancement afforded by the photonic environment of the microbeads. The reported hybrids also demonstrate markedly better resistance to degradation in water over 30 days of immersion.
Photonic crystal-perovskite nanocrystal hybrid beads exhibit Purcell enhancement and increased quantum yields of photoluminescence. The photonic crystal matrix is key for modulating the optoelectronic properties of the incorporated nanocrystals. |
doi_str_mv | 10.1039/d3cc02962j |
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Photonic crystal-perovskite nanocrystal hybrid beads exhibit Purcell enhancement and increased quantum yields of photoluminescence. The photonic crystal matrix is key for modulating the optoelectronic properties of the incorporated nanocrystals.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/d3cc02962j</identifier><identifier>PMID: 37548908</identifier><language>eng</language><publisher>England: Royal Society of Chemistry</publisher><subject>Metal halides ; Nanocrystals ; Nanoparticles ; Perovskites ; Photoluminescence ; Photonic crystals</subject><ispartof>Chemical communications (Cambridge, England), 2023-08, Vol.59 (69), p.138-1383</ispartof><rights>Copyright Royal Society of Chemistry 2023</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c337t-46bdf1adedeb96bd2cdaf71b0ca1400f1440dccc7a6b7387fa93c60dc41407ab3</citedby><cites>FETCH-LOGICAL-c337t-46bdf1adedeb96bd2cdaf71b0ca1400f1440dccc7a6b7387fa93c60dc41407ab3</cites><orcidid>0000-0002-5190-7193</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/37548908$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Lapointe, Victoria</creatorcontrib><creatorcontrib>Imperiale, Christian J</creatorcontrib><creatorcontrib>Chengadu, Sollavi</creatorcontrib><creatorcontrib>Pomilio, Cristina M</creatorcontrib><creatorcontrib>Ganesh, Meera</creatorcontrib><creatorcontrib>Kéna-Cohen, Stephane</creatorcontrib><creatorcontrib>Majewski, Marek B</creatorcontrib><title>Photonic enhancement in photoluminescent metal halide perovskite-photonic crystal bead hybrids</title><title>Chemical communications (Cambridge, England)</title><addtitle>Chem Commun (Camb)</addtitle><description>We report two photonic crystal-perovskite nanocrystal microbead hybrids with photoluminescence matching that of the parent nanocrystals but with increased photoluminescence quantum yields. Time-resolved photoluminescence spectroscopy quantifies the radiative enhancement afforded by the photonic environment of the microbeads. The reported hybrids also demonstrate markedly better resistance to degradation in water over 30 days of immersion.
Photonic crystal-perovskite nanocrystal hybrid beads exhibit Purcell enhancement and increased quantum yields of photoluminescence. The photonic crystal matrix is key for modulating the optoelectronic properties of the incorporated nanocrystals.</description><subject>Metal halides</subject><subject>Nanocrystals</subject><subject>Nanoparticles</subject><subject>Perovskites</subject><subject>Photoluminescence</subject><subject>Photonic crystals</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNpdkctLxDAQxoMo7rp68a4UvIhQTZq0aY9S3yzoQcGTJa_SrG1ak1bY_97UfQjOZYZvfnwM3wBwjOAlgji7klgIGGVJtNgBU4QTEsYkfd8d5zgLKSbxBBw4t4C-UJzugwmmnshgOgUfL1Xbt0aLQJmKGaEaZfpAm6Ab9XpotFFOjFqjelYHFau1VEGnbPvtPnWvwm5jIOzSjQhXTAbVklst3SHYK1nt1NG6z8Db3e1r_hDOn-8f8-t5KDCmfUgSLkvEpJKKZ36OhGQlRRwKhgiEJSIESiEEZQmnOKUly7BIvET8mjKOZ-B85dvZ9mtQri8a7c-ua2ZUO7giSonPwbtgj579QxftYI2_zlNxElEYp8RTFytK2NY5q8qis7phdlkgWIypFzc4z39Tf_Lw6dpy4I2SW3QTswdOVoB1Yrv9exv-AVN4iRA</recordid><startdate>20230824</startdate><enddate>20230824</enddate><creator>Lapointe, Victoria</creator><creator>Imperiale, Christian J</creator><creator>Chengadu, Sollavi</creator><creator>Pomilio, Cristina M</creator><creator>Ganesh, Meera</creator><creator>Kéna-Cohen, Stephane</creator><creator>Majewski, Marek B</creator><general>Royal Society of Chemistry</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-5190-7193</orcidid></search><sort><creationdate>20230824</creationdate><title>Photonic enhancement in photoluminescent metal halide perovskite-photonic crystal bead hybrids</title><author>Lapointe, Victoria ; Imperiale, Christian J ; Chengadu, Sollavi ; Pomilio, Cristina M ; Ganesh, Meera ; Kéna-Cohen, Stephane ; Majewski, Marek B</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c337t-46bdf1adedeb96bd2cdaf71b0ca1400f1440dccc7a6b7387fa93c60dc41407ab3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Metal halides</topic><topic>Nanocrystals</topic><topic>Nanoparticles</topic><topic>Perovskites</topic><topic>Photoluminescence</topic><topic>Photonic crystals</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Lapointe, Victoria</creatorcontrib><creatorcontrib>Imperiale, Christian J</creatorcontrib><creatorcontrib>Chengadu, Sollavi</creatorcontrib><creatorcontrib>Pomilio, Cristina M</creatorcontrib><creatorcontrib>Ganesh, Meera</creatorcontrib><creatorcontrib>Kéna-Cohen, Stephane</creatorcontrib><creatorcontrib>Majewski, Marek B</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lapointe, Victoria</au><au>Imperiale, Christian J</au><au>Chengadu, Sollavi</au><au>Pomilio, Cristina M</au><au>Ganesh, Meera</au><au>Kéna-Cohen, Stephane</au><au>Majewski, Marek B</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Photonic enhancement in photoluminescent metal halide perovskite-photonic crystal bead hybrids</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><addtitle>Chem Commun (Camb)</addtitle><date>2023-08-24</date><risdate>2023</risdate><volume>59</volume><issue>69</issue><spage>138</spage><epage>1383</epage><pages>138-1383</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>We report two photonic crystal-perovskite nanocrystal microbead hybrids with photoluminescence matching that of the parent nanocrystals but with increased photoluminescence quantum yields. Time-resolved photoluminescence spectroscopy quantifies the radiative enhancement afforded by the photonic environment of the microbeads. The reported hybrids also demonstrate markedly better resistance to degradation in water over 30 days of immersion.
Photonic crystal-perovskite nanocrystal hybrid beads exhibit Purcell enhancement and increased quantum yields of photoluminescence. The photonic crystal matrix is key for modulating the optoelectronic properties of the incorporated nanocrystals.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>37548908</pmid><doi>10.1039/d3cc02962j</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0002-5190-7193</orcidid></addata></record> |
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source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
subjects | Metal halides Nanocrystals Nanoparticles Perovskites Photoluminescence Photonic crystals |
title | Photonic enhancement in photoluminescent metal halide perovskite-photonic crystal bead hybrids |
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