Surface enhanced dynamic nuclear polarization solid-state NMR spectroscopy sheds light on Brønsted-Lewis acid synergy during the zeolite catalyzed methanol-to-hydrocarbon process

After a prolonged effort over two decades, the reaction mechanism of the zeolite-catalyzed methanol-to-hydrocarbon (MTH) process is now well-understood: the so-called 'direct mechanism' ( via direct coupling of two methanol molecules) is responsible for the formation of the initial carbon-...

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Veröffentlicht in:Chemical science (Cambridge) 2019-10, Vol.1 (39), p.8946-8954
Hauptverfasser: Dutta Chowdhury, Abhishek, Yarulina, Irina, Abou-Hamad, Edy, Gurinov, Andrei, Gascon, Jorge
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Sprache:eng
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