A simple strategy to design 3-layered Au-TiO 2 dual nanoparticles immobilized cellulose membranes with enhanced photocatalytic activity

Cellulose-based photocatalysts of supported nanoparticles feature high photocatalytic activity but their facile construction and photocatalytic mechanism exploration are highly challenging. Herein, a simple structural design principle and synergistic properties of 3-layered porous cellulose-based me...

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Veröffentlicht in:Carbohydrate polymers 2020-03, Vol.231, p.115694
Hauptverfasser: Yu, Yuqing, Zhu, Xingrong, Wang, Langrun, Wu, Fengshou, Liu, Shilin, Chang, Chunyu, Luo, Xiaogang
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container_issue
container_start_page 115694
container_title Carbohydrate polymers
container_volume 231
creator Yu, Yuqing
Zhu, Xingrong
Wang, Langrun
Wu, Fengshou
Liu, Shilin
Chang, Chunyu
Luo, Xiaogang
description Cellulose-based photocatalysts of supported nanoparticles feature high photocatalytic activity but their facile construction and photocatalytic mechanism exploration are highly challenging. Herein, a simple structural design principle and synergistic properties of 3-layered porous cellulose-based membranes are used for catalytic degradation of Rhodamine B in an aqua system. The 3-layered Au-TiO cellulose membranes were fabricated through the tape method and the suction filtration process. The composite membranes with strong redox ability, high charge-separation efficiency, and wide absorption range could stimulate the solar-driven plasma evaporation of Au nanoparticles and the photocatalytic function of TiO nanoparticles simultaneously. As characterized by Scanning Electron Microscopy, well-defined Au nanoparticles with an average size of 18.24 ± 3.17 nm were uniformly distributed on the TiO -CM surface. Compared with TiO -CM, TiO -Au-CM showed better catalytic degradation of organic dye. This work demonstrated that a simple strategy design of Au-TiO -CM could efficiently enhance the photocatalytic activity for the degradation of dyes in water.
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Herein, a simple structural design principle and synergistic properties of 3-layered porous cellulose-based membranes are used for catalytic degradation of Rhodamine B in an aqua system. The 3-layered Au-TiO cellulose membranes were fabricated through the tape method and the suction filtration process. The composite membranes with strong redox ability, high charge-separation efficiency, and wide absorption range could stimulate the solar-driven plasma evaporation of Au nanoparticles and the photocatalytic function of TiO nanoparticles simultaneously. As characterized by Scanning Electron Microscopy, well-defined Au nanoparticles with an average size of 18.24 ± 3.17 nm were uniformly distributed on the TiO -CM surface. Compared with TiO -CM, TiO -Au-CM showed better catalytic degradation of organic dye. 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title A simple strategy to design 3-layered Au-TiO 2 dual nanoparticles immobilized cellulose membranes with enhanced photocatalytic activity
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