Ionic circuitry with nanofluidic diodes
Ionic circuits composed of nanopores functionalized with polyelectrolyte chains can operate in aqueous solutions, thus allowing the control of electrical signals and information processing in physiological environments. We demonstrate experimentally and theoretically that different orientations of s...
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Veröffentlicht in: | Soft matter 2019-12, Vol.15 (47), p.9682-9689 |
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creator | Ali, Mubarak Ramirez, Patricio Nasir, Saima Cervera, Javier Mafe, Salvador Ensinger, Wolfgang |
description | Ionic circuits composed of nanopores functionalized with polyelectrolyte chains can operate in aqueous solutions, thus allowing the control of electrical signals and information processing in physiological environments. We demonstrate experimentally and theoretically that different orientations of single-pore membranes with the same and opposite surface charges can operate reliably in series, parallel, and mixed series-parallel arrangements of two, three, and four nanofluidic diodes using schemes similar to those of solid-state electronics. We consider also different experimental procedures to externally tune the fixed charges of the molecular chains functionalized on the pore surface, showing that single-pore membranes can be used efficiently in ionic circuitry with distinct ionic environments.
We demonstrate various orientations of single-pore membranes operating reliably in different arrangements of two, three, and four nanofluidic diodes using schemes similar to those of solid-state electronics with distinct ionic environments. |
doi_str_mv | 10.1039/c9sm01654f |
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We demonstrate various orientations of single-pore membranes operating reliably in different arrangements of two, three, and four nanofluidic diodes using schemes similar to those of solid-state electronics with distinct ionic environments.</description><identifier>ISSN: 1744-683X</identifier><identifier>EISSN: 1744-6848</identifier><identifier>DOI: 10.1039/c9sm01654f</identifier><identifier>PMID: 31720668</identifier><language>eng</language><publisher>England: Royal Society of Chemistry</publisher><subject>Aqueous solutions ; Circuits ; Data processing ; Diodes ; Fluidics ; Information processing ; Membranes ; Molecular chains ; Nanofluids ; Polyelectrolytes ; Porosity ; Signal processing</subject><ispartof>Soft matter, 2019-12, Vol.15 (47), p.9682-9689</ispartof><rights>Copyright Royal Society of Chemistry 2019</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c441t-84390e398cc19a665085854c42805e1d8e1244dd25086300bdb1d3c3e8a55e7e3</citedby><cites>FETCH-LOGICAL-c441t-84390e398cc19a665085854c42805e1d8e1244dd25086300bdb1d3c3e8a55e7e3</cites><orcidid>0000-0001-8965-9298 ; 0000-0002-2521-2718</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27903,27904</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/31720668$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Ali, Mubarak</creatorcontrib><creatorcontrib>Ramirez, Patricio</creatorcontrib><creatorcontrib>Nasir, Saima</creatorcontrib><creatorcontrib>Cervera, Javier</creatorcontrib><creatorcontrib>Mafe, Salvador</creatorcontrib><creatorcontrib>Ensinger, Wolfgang</creatorcontrib><title>Ionic circuitry with nanofluidic diodes</title><title>Soft matter</title><addtitle>Soft Matter</addtitle><description>Ionic circuits composed of nanopores functionalized with polyelectrolyte chains can operate in aqueous solutions, thus allowing the control of electrical signals and information processing in physiological environments. We demonstrate experimentally and theoretically that different orientations of single-pore membranes with the same and opposite surface charges can operate reliably in series, parallel, and mixed series-parallel arrangements of two, three, and four nanofluidic diodes using schemes similar to those of solid-state electronics. We consider also different experimental procedures to externally tune the fixed charges of the molecular chains functionalized on the pore surface, showing that single-pore membranes can be used efficiently in ionic circuitry with distinct ionic environments.
We demonstrate various orientations of single-pore membranes operating reliably in different arrangements of two, three, and four nanofluidic diodes using schemes similar to those of solid-state electronics with distinct ionic environments.</description><subject>Aqueous solutions</subject><subject>Circuits</subject><subject>Data processing</subject><subject>Diodes</subject><subject>Fluidics</subject><subject>Information processing</subject><subject>Membranes</subject><subject>Molecular chains</subject><subject>Nanofluids</subject><subject>Polyelectrolytes</subject><subject>Porosity</subject><subject>Signal processing</subject><issn>1744-683X</issn><issn>1744-6848</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNp90M1LwzAYBvAgipvTi3dlw4MiVPPd5CjD6WDiQQVvoUtSzGibmbTI_nujmxM8eMoLz4_3DQ8AxwheIUjktZaxhogzWu6APsopzbigYnc7k9ceOIhxASERFPF90CMox5Bz0QfnU984PdQu6M61YTX8cO3bsCkaX1adMykyzhsbD8FeWVTRHm3eAXiZ3D6P77PZ4910fDPLNKWozQQlEloihdZIFpwzKJhgVFMsILPICIswpcbgFHAC4dzMkSGaWFEwZnNLBuBivXcZ_HtnY6tqF7WtqqKxvosKE0Qx5YzkiZ79oQvfhSb9LikMJUnnRVKXa6WDjzHYUi2Dq4uwUgiqr_rUWD49fNc3Sfh0s7Kb19Zs6U9fCYzWIES9TX_7V0tTJnPynyGfxfx86Q</recordid><startdate>20191204</startdate><enddate>20191204</enddate><creator>Ali, Mubarak</creator><creator>Ramirez, Patricio</creator><creator>Nasir, Saima</creator><creator>Cervera, Javier</creator><creator>Mafe, Salvador</creator><creator>Ensinger, Wolfgang</creator><general>Royal Society of Chemistry</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QF</scope><scope>7QO</scope><scope>7QQ</scope><scope>7SC</scope><scope>7SE</scope><scope>7SP</scope><scope>7SR</scope><scope>7TA</scope><scope>7TB</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>F28</scope><scope>FR3</scope><scope>H8D</scope><scope>H8G</scope><scope>JG9</scope><scope>JQ2</scope><scope>KR7</scope><scope>L7M</scope><scope>L~C</scope><scope>L~D</scope><scope>P64</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0001-8965-9298</orcidid><orcidid>https://orcid.org/0000-0002-2521-2718</orcidid></search><sort><creationdate>20191204</creationdate><title>Ionic circuitry with nanofluidic diodes</title><author>Ali, Mubarak ; Ramirez, Patricio ; Nasir, Saima ; Cervera, Javier ; Mafe, Salvador ; Ensinger, Wolfgang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c441t-84390e398cc19a665085854c42805e1d8e1244dd25086300bdb1d3c3e8a55e7e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Aqueous solutions</topic><topic>Circuits</topic><topic>Data processing</topic><topic>Diodes</topic><topic>Fluidics</topic><topic>Information processing</topic><topic>Membranes</topic><topic>Molecular chains</topic><topic>Nanofluids</topic><topic>Polyelectrolytes</topic><topic>Porosity</topic><topic>Signal processing</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ali, Mubarak</creatorcontrib><creatorcontrib>Ramirez, Patricio</creatorcontrib><creatorcontrib>Nasir, Saima</creatorcontrib><creatorcontrib>Cervera, Javier</creatorcontrib><creatorcontrib>Mafe, Salvador</creatorcontrib><creatorcontrib>Ensinger, Wolfgang</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Aluminium Industry Abstracts</collection><collection>Biotechnology Research Abstracts</collection><collection>Ceramic Abstracts</collection><collection>Computer and Information Systems Abstracts</collection><collection>Corrosion Abstracts</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Materials Business File</collection><collection>Mechanical & Transportation Engineering Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>Aerospace Database</collection><collection>Copper Technical Reference Library</collection><collection>Materials Research Database</collection><collection>ProQuest Computer Science Collection</collection><collection>Civil Engineering Abstracts</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Computer and Information Systems Abstracts Academic</collection><collection>Computer and Information Systems Abstracts Professional</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>MEDLINE - Academic</collection><jtitle>Soft matter</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ali, Mubarak</au><au>Ramirez, Patricio</au><au>Nasir, Saima</au><au>Cervera, Javier</au><au>Mafe, Salvador</au><au>Ensinger, Wolfgang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Ionic circuitry with nanofluidic diodes</atitle><jtitle>Soft matter</jtitle><addtitle>Soft Matter</addtitle><date>2019-12-04</date><risdate>2019</risdate><volume>15</volume><issue>47</issue><spage>9682</spage><epage>9689</epage><pages>9682-9689</pages><issn>1744-683X</issn><eissn>1744-6848</eissn><abstract>Ionic circuits composed of nanopores functionalized with polyelectrolyte chains can operate in aqueous solutions, thus allowing the control of electrical signals and information processing in physiological environments. We demonstrate experimentally and theoretically that different orientations of single-pore membranes with the same and opposite surface charges can operate reliably in series, parallel, and mixed series-parallel arrangements of two, three, and four nanofluidic diodes using schemes similar to those of solid-state electronics. We consider also different experimental procedures to externally tune the fixed charges of the molecular chains functionalized on the pore surface, showing that single-pore membranes can be used efficiently in ionic circuitry with distinct ionic environments.
We demonstrate various orientations of single-pore membranes operating reliably in different arrangements of two, three, and four nanofluidic diodes using schemes similar to those of solid-state electronics with distinct ionic environments.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>31720668</pmid><doi>10.1039/c9sm01654f</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0001-8965-9298</orcidid><orcidid>https://orcid.org/0000-0002-2521-2718</orcidid></addata></record> |
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source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
subjects | Aqueous solutions Circuits Data processing Diodes Fluidics Information processing Membranes Molecular chains Nanofluids Polyelectrolytes Porosity Signal processing |
title | Ionic circuitry with nanofluidic diodes |
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