Ionic circuitry with nanofluidic diodes

Ionic circuits composed of nanopores functionalized with polyelectrolyte chains can operate in aqueous solutions, thus allowing the control of electrical signals and information processing in physiological environments. We demonstrate experimentally and theoretically that different orientations of s...

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Veröffentlicht in:Soft matter 2019-12, Vol.15 (47), p.9682-9689
Hauptverfasser: Ali, Mubarak, Ramirez, Patricio, Nasir, Saima, Cervera, Javier, Mafe, Salvador, Ensinger, Wolfgang
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container_end_page 9689
container_issue 47
container_start_page 9682
container_title Soft matter
container_volume 15
creator Ali, Mubarak
Ramirez, Patricio
Nasir, Saima
Cervera, Javier
Mafe, Salvador
Ensinger, Wolfgang
description Ionic circuits composed of nanopores functionalized with polyelectrolyte chains can operate in aqueous solutions, thus allowing the control of electrical signals and information processing in physiological environments. We demonstrate experimentally and theoretically that different orientations of single-pore membranes with the same and opposite surface charges can operate reliably in series, parallel, and mixed series-parallel arrangements of two, three, and four nanofluidic diodes using schemes similar to those of solid-state electronics. We consider also different experimental procedures to externally tune the fixed charges of the molecular chains functionalized on the pore surface, showing that single-pore membranes can be used efficiently in ionic circuitry with distinct ionic environments. We demonstrate various orientations of single-pore membranes operating reliably in different arrangements of two, three, and four nanofluidic diodes using schemes similar to those of solid-state electronics with distinct ionic environments.
doi_str_mv 10.1039/c9sm01654f
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source Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection
subjects Aqueous solutions
Circuits
Data processing
Diodes
Fluidics
Information processing
Membranes
Molecular chains
Nanofluids
Polyelectrolytes
Porosity
Signal processing
title Ionic circuitry with nanofluidic diodes
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