Design of an efficient photocatalytic reactor for the decomposition of gaseous organic contaminants in air
[Display omitted] ► Linear velocity for the designed reactor was optimized for photocatalytic reaction. ► Fiber based support for immobilizing TiO2 improved the photocatalytic performance. ► Optimum photocatalytic system for degradation of organic pollutant was designed. ► Suggested reactor exhibite...
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Veröffentlicht in: | Chemical engineering journal (Lausanne, Switzerland : 1996) Switzerland : 1996), 2012-04, Vol.187, p.203-209 |
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container_title | Chemical engineering journal (Lausanne, Switzerland : 1996) |
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creator | Lee, David Minzae Yun, Hyeong Jin Yu, Sungju Yun, Seong Jin Lee, Sun Young Kang, Sang Hyeon Yi, Jongheop |
description | [Display omitted]
► Linear velocity for the designed reactor was optimized for photocatalytic reaction. ► Fiber based support for immobilizing TiO2 improved the photocatalytic performance. ► Optimum photocatalytic system for degradation of organic pollutant was designed. ► Suggested reactor exhibited very high stability for photocatalytic reaction.
Here, a strategy for decomposing gaseous organic contaminants by photocatalytic reactions is reported. A photocatalytic reactor is designed, based on an open tubular reactor with a UV light source installed at the center of the glass tube to permit the vertical irradiation of light onto the photocatalyst. TiO2 immobilized on a stainless steel plate and a fiber based material, respectively, are placed on the inner wall of an open tubular reactor. The fibers of felt induce wake and eddy flow near the inner surface of the reactor, resulting in compression of boundary layer. The compressed boundary layer provides a higher probability of contact between organic contaminants and the photocatalyst, consequently resulting in the enhanced photocatalytic oxidative decomposition of organic compounds. The inlet of photoreactor is modified in order to better control the bulk stream to form spiral-like flow. The reactor with a single tangent inlet exhibits the highest photocatalytic performance among the reactors examined, as an evidence of the improved probability of contact. Importantly, the reactor with a single tangent inlet, in which TiO2 immobilized felt is installed, maintains its photocatalytic activities for as long as twenty days. |
doi_str_mv | 10.1016/j.cej.2012.01.121 |
format | Article |
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► Linear velocity for the designed reactor was optimized for photocatalytic reaction. ► Fiber based support for immobilizing TiO2 improved the photocatalytic performance. ► Optimum photocatalytic system for degradation of organic pollutant was designed. ► Suggested reactor exhibited very high stability for photocatalytic reaction.
Here, a strategy for decomposing gaseous organic contaminants by photocatalytic reactions is reported. A photocatalytic reactor is designed, based on an open tubular reactor with a UV light source installed at the center of the glass tube to permit the vertical irradiation of light onto the photocatalyst. TiO2 immobilized on a stainless steel plate and a fiber based material, respectively, are placed on the inner wall of an open tubular reactor. The fibers of felt induce wake and eddy flow near the inner surface of the reactor, resulting in compression of boundary layer. The compressed boundary layer provides a higher probability of contact between organic contaminants and the photocatalyst, consequently resulting in the enhanced photocatalytic oxidative decomposition of organic compounds. The inlet of photoreactor is modified in order to better control the bulk stream to form spiral-like flow. The reactor with a single tangent inlet exhibits the highest photocatalytic performance among the reactors examined, as an evidence of the improved probability of contact. Importantly, the reactor with a single tangent inlet, in which TiO2 immobilized felt is installed, maintains its photocatalytic activities for as long as twenty days.</description><identifier>ISSN: 1385-8947</identifier><identifier>EISSN: 1873-3212</identifier><identifier>DOI: 10.1016/j.cej.2012.01.121</identifier><language>eng</language><publisher>Oxford: Elsevier B.V</publisher><subject>air ; Air purification ; Applied sciences ; Catalysis ; Catalytic reactions ; Chemical engineering ; Chemistry ; Contact ; Contact probability ; Contaminants ; Exact sciences and technology ; Fibers ; General and physical chemistry ; glass ; Inlets ; irradiation ; organic compounds ; Photocatalysis ; probability ; Reactor design ; Reactors ; stainless steel ; Tangents ; Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry ; TiO2 ; Titanium dioxide ; ultraviolet radiation</subject><ispartof>Chemical engineering journal (Lausanne, Switzerland : 1996), 2012-04, Vol.187, p.203-209</ispartof><rights>2012 Elsevier B.V.</rights><rights>2015 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c453t-37fe63ee8d557cd9008ff6944fce5f53e565e65bef51398cfa3f222185f28d203</citedby><cites>FETCH-LOGICAL-c453t-37fe63ee8d557cd9008ff6944fce5f53e565e65bef51398cfa3f222185f28d203</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.cej.2012.01.121$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=25785185$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>Lee, David Minzae</creatorcontrib><creatorcontrib>Yun, Hyeong Jin</creatorcontrib><creatorcontrib>Yu, Sungju</creatorcontrib><creatorcontrib>Yun, Seong Jin</creatorcontrib><creatorcontrib>Lee, Sun Young</creatorcontrib><creatorcontrib>Kang, Sang Hyeon</creatorcontrib><creatorcontrib>Yi, Jongheop</creatorcontrib><title>Design of an efficient photocatalytic reactor for the decomposition of gaseous organic contaminants in air</title><title>Chemical engineering journal (Lausanne, Switzerland : 1996)</title><description>[Display omitted]
► Linear velocity for the designed reactor was optimized for photocatalytic reaction. ► Fiber based support for immobilizing TiO2 improved the photocatalytic performance. ► Optimum photocatalytic system for degradation of organic pollutant was designed. ► Suggested reactor exhibited very high stability for photocatalytic reaction.
Here, a strategy for decomposing gaseous organic contaminants by photocatalytic reactions is reported. A photocatalytic reactor is designed, based on an open tubular reactor with a UV light source installed at the center of the glass tube to permit the vertical irradiation of light onto the photocatalyst. TiO2 immobilized on a stainless steel plate and a fiber based material, respectively, are placed on the inner wall of an open tubular reactor. The fibers of felt induce wake and eddy flow near the inner surface of the reactor, resulting in compression of boundary layer. The compressed boundary layer provides a higher probability of contact between organic contaminants and the photocatalyst, consequently resulting in the enhanced photocatalytic oxidative decomposition of organic compounds. The inlet of photoreactor is modified in order to better control the bulk stream to form spiral-like flow. The reactor with a single tangent inlet exhibits the highest photocatalytic performance among the reactors examined, as an evidence of the improved probability of contact. Importantly, the reactor with a single tangent inlet, in which TiO2 immobilized felt is installed, maintains its photocatalytic activities for as long as twenty days.</description><subject>air</subject><subject>Air purification</subject><subject>Applied sciences</subject><subject>Catalysis</subject><subject>Catalytic reactions</subject><subject>Chemical engineering</subject><subject>Chemistry</subject><subject>Contact</subject><subject>Contact probability</subject><subject>Contaminants</subject><subject>Exact sciences and technology</subject><subject>Fibers</subject><subject>General and physical chemistry</subject><subject>glass</subject><subject>Inlets</subject><subject>irradiation</subject><subject>organic compounds</subject><subject>Photocatalysis</subject><subject>probability</subject><subject>Reactor design</subject><subject>Reactors</subject><subject>stainless steel</subject><subject>Tangents</subject><subject>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</subject><subject>TiO2</subject><subject>Titanium dioxide</subject><subject>ultraviolet radiation</subject><issn>1385-8947</issn><issn>1873-3212</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2012</creationdate><recordtype>article</recordtype><recordid>eNp9kU1vFSEYhSdGE2v1B7iSTVM3M-VjYCCuTLUfSRMX2jV5ZV5umcyFW6Am_fdye5suuyCweM7JCU_XfWZ0YJSps2VwuAycMj5QNjDO3nRHTE-iF5zxt-0ttOy1Gaf33YdSFkqpMswcdcsPLGETSfIEIkHvgwsYK9ndpZocVFgfa3AkI7iaMvHt1DskM7q03aUSakhP4Q0UTA-FpLyB2AIuxQrbECHWQkIkEPLH7p2HteCn5_u4u734-ef8qr_5dXl9_v2md6MUtReTRyUQ9Szl5GZDqfZemXH0DqWXAqWSqORf9JIJo50H4TnnTEvP9cypOO5OD727nO4fsFS7DcXhukLcT7RGaTZRbkwjv75KNsxMSppRNZQdUJdTKRm93eWwhfxoGbV7A3axzYDdG7CU2WagZU6e66E4WH2G6EJ5CXI5adlmN-7LgfOQLGxyY25_tyJJKaOSirER3w4Etn_7FzDbstfkcA4ZXbVzCq_s-A9BpKVo</recordid><startdate>20120401</startdate><enddate>20120401</enddate><creator>Lee, David Minzae</creator><creator>Yun, Hyeong Jin</creator><creator>Yu, Sungju</creator><creator>Yun, Seong Jin</creator><creator>Lee, Sun Young</creator><creator>Kang, Sang Hyeon</creator><creator>Yi, Jongheop</creator><general>Elsevier B.V</general><general>Elsevier</general><scope>FBQ</scope><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>JG9</scope><scope>7ST</scope><scope>C1K</scope><scope>SOI</scope></search><sort><creationdate>20120401</creationdate><title>Design of an efficient photocatalytic reactor for the decomposition of gaseous organic contaminants in air</title><author>Lee, David Minzae ; Yun, Hyeong Jin ; Yu, Sungju ; Yun, Seong Jin ; Lee, Sun Young ; Kang, Sang Hyeon ; Yi, Jongheop</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c453t-37fe63ee8d557cd9008ff6944fce5f53e565e65bef51398cfa3f222185f28d203</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2012</creationdate><topic>air</topic><topic>Air purification</topic><topic>Applied sciences</topic><topic>Catalysis</topic><topic>Catalytic reactions</topic><topic>Chemical engineering</topic><topic>Chemistry</topic><topic>Contact</topic><topic>Contact probability</topic><topic>Contaminants</topic><topic>Exact sciences and technology</topic><topic>Fibers</topic><topic>General and physical chemistry</topic><topic>glass</topic><topic>Inlets</topic><topic>irradiation</topic><topic>organic compounds</topic><topic>Photocatalysis</topic><topic>probability</topic><topic>Reactor design</topic><topic>Reactors</topic><topic>stainless steel</topic><topic>Tangents</topic><topic>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</topic><topic>TiO2</topic><topic>Titanium dioxide</topic><topic>ultraviolet radiation</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Lee, David Minzae</creatorcontrib><creatorcontrib>Yun, Hyeong Jin</creatorcontrib><creatorcontrib>Yu, Sungju</creatorcontrib><creatorcontrib>Yun, Seong Jin</creatorcontrib><creatorcontrib>Lee, Sun Young</creatorcontrib><creatorcontrib>Kang, Sang Hyeon</creatorcontrib><creatorcontrib>Yi, Jongheop</creatorcontrib><collection>AGRIS</collection><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Environment Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Environment Abstracts</collection><jtitle>Chemical engineering journal (Lausanne, Switzerland : 1996)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lee, David Minzae</au><au>Yun, Hyeong Jin</au><au>Yu, Sungju</au><au>Yun, Seong Jin</au><au>Lee, Sun Young</au><au>Kang, Sang Hyeon</au><au>Yi, Jongheop</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Design of an efficient photocatalytic reactor for the decomposition of gaseous organic contaminants in air</atitle><jtitle>Chemical engineering journal (Lausanne, Switzerland : 1996)</jtitle><date>2012-04-01</date><risdate>2012</risdate><volume>187</volume><spage>203</spage><epage>209</epage><pages>203-209</pages><issn>1385-8947</issn><eissn>1873-3212</eissn><abstract>[Display omitted]
► Linear velocity for the designed reactor was optimized for photocatalytic reaction. ► Fiber based support for immobilizing TiO2 improved the photocatalytic performance. ► Optimum photocatalytic system for degradation of organic pollutant was designed. ► Suggested reactor exhibited very high stability for photocatalytic reaction.
Here, a strategy for decomposing gaseous organic contaminants by photocatalytic reactions is reported. A photocatalytic reactor is designed, based on an open tubular reactor with a UV light source installed at the center of the glass tube to permit the vertical irradiation of light onto the photocatalyst. TiO2 immobilized on a stainless steel plate and a fiber based material, respectively, are placed on the inner wall of an open tubular reactor. The fibers of felt induce wake and eddy flow near the inner surface of the reactor, resulting in compression of boundary layer. The compressed boundary layer provides a higher probability of contact between organic contaminants and the photocatalyst, consequently resulting in the enhanced photocatalytic oxidative decomposition of organic compounds. The inlet of photoreactor is modified in order to better control the bulk stream to form spiral-like flow. The reactor with a single tangent inlet exhibits the highest photocatalytic performance among the reactors examined, as an evidence of the improved probability of contact. Importantly, the reactor with a single tangent inlet, in which TiO2 immobilized felt is installed, maintains its photocatalytic activities for as long as twenty days.</abstract><cop>Oxford</cop><pub>Elsevier B.V</pub><doi>10.1016/j.cej.2012.01.121</doi><tpages>7</tpages></addata></record> |
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subjects | air Air purification Applied sciences Catalysis Catalytic reactions Chemical engineering Chemistry Contact Contact probability Contaminants Exact sciences and technology Fibers General and physical chemistry glass Inlets irradiation organic compounds Photocatalysis probability Reactor design Reactors stainless steel Tangents Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry TiO2 Titanium dioxide ultraviolet radiation |
title | Design of an efficient photocatalytic reactor for the decomposition of gaseous organic contaminants in air |
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