Photochromism in single nitrogen-vacancy defect in diamond
Photochromism in single nitrogen-vacancy optical centers in diamond is demonstrated. Time-resolved optical spectroscopy shows that intense irradiation at 514 nm switches the nitrogen-vacancy defects to the negative form. This defect state relaxes back to the neutral form under dark conditions. Tempo...
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Veröffentlicht in: | Applied physics. B, Lasers and optics Lasers and optics, 2006-02, Vol.82 (2), p.243-246 |
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container_title | Applied physics. B, Lasers and optics |
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creator | Gaebel, T. Domhan, M. Wittmann, C. Popa, I. Jelezko, F. Rabeau, J. Greentree, A. Prawer, S. Trajkov, E. Hemmer, P.R. Wrachtrup, J. |
description | Photochromism in single nitrogen-vacancy optical centers in diamond is demonstrated. Time-resolved optical spectroscopy shows that intense irradiation at 514 nm switches the nitrogen-vacancy defects to the negative form. This defect state relaxes back to the neutral form under dark conditions. Temporal anticorrelation of photons emitted by the different charge states of the optical center unambiguously indicates that the nitrogen-vacancy defect accounts for both 575 nm and 638 nm emission bands. Possible mechanism of photochromism involving nitrogen donors is discussed. |
doi_str_mv | 10.1007/s00340-005-2056-2 |
format | Article |
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B, Lasers and optics</title><description>Photochromism in single nitrogen-vacancy optical centers in diamond is demonstrated. Time-resolved optical spectroscopy shows that intense irradiation at 514 nm switches the nitrogen-vacancy defects to the negative form. This defect state relaxes back to the neutral form under dark conditions. Temporal anticorrelation of photons emitted by the different charge states of the optical center unambiguously indicates that the nitrogen-vacancy defect accounts for both 575 nm and 638 nm emission bands. Possible mechanism of photochromism involving nitrogen donors is discussed.</description><subject>Bands</subject><subject>Defects</subject><subject>Emission</subject><subject>Lasers</subject><subject>Photochromism</subject><subject>Photons</subject><subject>Switches</subject><subject>Temporal logic</subject><issn>0946-2171</issn><issn>1432-0649</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2006</creationdate><recordtype>article</recordtype><recordid>eNotkE1LAzEQhoMoWKs_wNvePEUnH5tNvEnRKhT0oOeQ5qNd2U1qshX6702pcxl4eXiZeRC6JXBPALqHAsA4YIAWU2gFpmdoRjijGARX52gGiteQdOQSXZXyDXWElDP0-LFNU7LbnMa-jE0fm9LHzeCb2E85bXzEv8aaaA-N88Hb6Ui43owpumt0EcxQ_M3_nqOvl-fPxStevS_fFk8rbBlnE6a25V4xGdY0COGkMVRJFwIVwvK14w68dQI6ERRxgtaMtVIo40F2QAJnc3R36t3l9LP3ZdL1VOuHwUSf9kUroupzsmsrSU6kzamU7IPe5X40-aAJ6KMmfdKkqyZ91KQp-wOXmlq3</recordid><startdate>20060201</startdate><enddate>20060201</enddate><creator>Gaebel, T.</creator><creator>Domhan, M.</creator><creator>Wittmann, C.</creator><creator>Popa, I.</creator><creator>Jelezko, F.</creator><creator>Rabeau, J.</creator><creator>Greentree, A.</creator><creator>Prawer, S.</creator><creator>Trajkov, E.</creator><creator>Hemmer, P.R.</creator><creator>Wrachtrup, J.</creator><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope></search><sort><creationdate>20060201</creationdate><title>Photochromism in single nitrogen-vacancy defect in diamond</title><author>Gaebel, T. ; Domhan, M. ; Wittmann, C. ; Popa, I. ; Jelezko, F. ; Rabeau, J. ; Greentree, A. ; Prawer, S. ; Trajkov, E. ; Hemmer, P.R. ; Wrachtrup, J.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c343t-2c54e938fb2f66d8aa298dff266c4bd4d0ecd6076f91d62c4b35869ae08701f43</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2006</creationdate><topic>Bands</topic><topic>Defects</topic><topic>Emission</topic><topic>Lasers</topic><topic>Photochromism</topic><topic>Photons</topic><topic>Switches</topic><topic>Temporal logic</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Gaebel, T.</creatorcontrib><creatorcontrib>Domhan, M.</creatorcontrib><creatorcontrib>Wittmann, C.</creatorcontrib><creatorcontrib>Popa, I.</creatorcontrib><creatorcontrib>Jelezko, F.</creatorcontrib><creatorcontrib>Rabeau, J.</creatorcontrib><creatorcontrib>Greentree, A.</creatorcontrib><creatorcontrib>Prawer, S.</creatorcontrib><creatorcontrib>Trajkov, E.</creatorcontrib><creatorcontrib>Hemmer, P.R.</creatorcontrib><creatorcontrib>Wrachtrup, J.</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Applied physics. B, Lasers and optics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Gaebel, T.</au><au>Domhan, M.</au><au>Wittmann, C.</au><au>Popa, I.</au><au>Jelezko, F.</au><au>Rabeau, J.</au><au>Greentree, A.</au><au>Prawer, S.</au><au>Trajkov, E.</au><au>Hemmer, P.R.</au><au>Wrachtrup, J.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Photochromism in single nitrogen-vacancy defect in diamond</atitle><jtitle>Applied physics. B, Lasers and optics</jtitle><date>2006-02-01</date><risdate>2006</risdate><volume>82</volume><issue>2</issue><spage>243</spage><epage>246</epage><pages>243-246</pages><issn>0946-2171</issn><eissn>1432-0649</eissn><abstract>Photochromism in single nitrogen-vacancy optical centers in diamond is demonstrated. Time-resolved optical spectroscopy shows that intense irradiation at 514 nm switches the nitrogen-vacancy defects to the negative form. This defect state relaxes back to the neutral form under dark conditions. Temporal anticorrelation of photons emitted by the different charge states of the optical center unambiguously indicates that the nitrogen-vacancy defect accounts for both 575 nm and 638 nm emission bands. Possible mechanism of photochromism involving nitrogen donors is discussed.</abstract><doi>10.1007/s00340-005-2056-2</doi><tpages>4</tpages></addata></record> |
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subjects | Bands Defects Emission Lasers Photochromism Photons Switches Temporal logic |
title | Photochromism in single nitrogen-vacancy defect in diamond |
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