Photostability of single-photon emission from a single quantum dot in the 650-nm wavelength band at room temperature

The photoluminescence correlation from a single CdSe nanocrystal under pulsed excitation is studied, and a single photon is realized at wavelength 655 nm at room temperature. The single colloidal CdSe quantum dot is prepared on a SiO 2 /silicon surface by a drop-and-drag technique. The long-term sta...

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Veröffentlicht in:Applied physics. B, Lasers and optics Lasers and optics, 2009-03, Vol.94 (4), p.577-583
Hauptverfasser: Xu, X., Yamada, T., Otomo, A.
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container_title Applied physics. B, Lasers and optics
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creator Xu, X.
Yamada, T.
Otomo, A.
description The photoluminescence correlation from a single CdSe nanocrystal under pulsed excitation is studied, and a single photon is realized at wavelength 655 nm at room temperature. The single colloidal CdSe quantum dot is prepared on a SiO 2 /silicon surface by a drop-and-drag technique. The long-term stability of the single-photon source is investigated; it is found that the antibunching effect weakens with excitation time, and the reason for the weakening is attributed to photobleaching. The lifetimes of photoluminescence from a single quantum dot are analyzed at different excitation times. By analyzing the probability distribution of on and off times of photoluminescence, the Auger assisted tunneling and Auger assisted photobleaching models are applied to explain the antibunching phenomenon.
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The long-term stability of the single-photon source is investigated; it is found that the antibunching effect weakens with excitation time, and the reason for the weakening is attributed to photobleaching. The lifetimes of photoluminescence from a single quantum dot are analyzed at different excitation times. By analyzing the probability distribution of on and off times of photoluminescence, the Auger assisted tunneling and Auger assisted photobleaching models are applied to explain the antibunching phenomenon.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer-Verlag</pub><doi>10.1007/s00340-009-3378-2</doi><tpages>7</tpages></addata></record>
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subjects Augers
Cadmium selenides
Engineering
Exact sciences and technology
Excitation
Fundamental areas of phenomenology (including applications)
Intermetallics
Lasers
Nanocrystals
Nonclassical field states
squeezed, antibunched and sub-poissonian states
operational definitions of the phase of the field
phase measurements
Optical Devices
Optics
Photoluminescence
Photon statistics and coherence theory
Photonics
Physical Chemistry
Physics
Physics and Astronomy
Quantum dots
Quantum Optics
Wavelengths
title Photostability of single-photon emission from a single quantum dot in the 650-nm wavelength band at room temperature
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