Half Kapitza-Dirac effect of H2+ molecule in intense standing-wave laser fields

The half Kapitza-Dirac effect of H2+ molecule in an intense standing-wave laser field is studied with a focus on the influence of the molecular orbital symmetry and the molecular alignment on the photo-electron angular distributions (PADs). In standing-wave laser fields, the PADs split along the sca...

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Veröffentlicht in:Optics express 2011-12, Vol.19 (25), p.24858-24870
Hauptverfasser: Ren, Xianghe, Zhang, Jingtao, Xu, Zhizhan, Guo, D-S
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Xu, Zhizhan
Guo, D-S
description The half Kapitza-Dirac effect of H2+ molecule in an intense standing-wave laser field is studied with a focus on the influence of the molecular orbital symmetry and the molecular alignment on the photo-electron angular distributions (PADs). In standing-wave laser fields, the PADs split along the scattering angle due to the momentum change of electron with photons when it escapes from the laser fields. The structures and the symmetry of PADs are severely affected by the molecular orbital symmetry and the molecular alignment. For H2+ molecule in ground state (σg), the PADs are severely changed by the molecular alignment only when the photoelectron kinetic energy is sufficiently high. For H2+ molecule in the first excited state (σμ), the molecular alignment distinctively changes the PADs, irrelevant to the kinetic energy of photoelectrons. When the molecules are aligned either parallel with or perpendicular to the laser polarization, the PADs are symmetric about an axis. In other cases, the PADs do not show any symmetry. These results indicate that the molecular alignment can be used to control the splitting in the half Kapitza-Dirac effect.
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subjects Computer Simulation
Hydrogen - chemistry
Lasers
Models, Theoretical
Scattering, Radiation
title Half Kapitza-Dirac effect of H2+ molecule in intense standing-wave laser fields
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