Unveiling and driving hidden resonances with high-fluence, high-intensity x-ray pulses
We show that high fluence, high-intensity x-ray pulses from the world's first hard x-ray free-electron laser produce nonlinear phenomena that differ dramatically from the linear x-ray-matter interaction processes that are encountered at synchrotron x-ray sources. We use intense x-ray pulses of...
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| Veröffentlicht in: | Phys. Rev. Lett 2011-12, Vol.107 (23), p.233001-233001, Article 233001 |
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| container_title | Phys. Rev. Lett |
| container_volume | 107 |
| creator | Kanter, E P Krässig, B Li, Y March, A M Ho, P Rohringer, N Santra, R Southworth, S H DiMauro, L F Doumy, G Roedig, C A Berrah, N Fang, L Hoener, M Bucksbaum, P H Ghimire, S Reis, D A Bozek, J D Bostedt, C Messerschmidt, M Young, L |
| description | We show that high fluence, high-intensity x-ray pulses from the world's first hard x-ray free-electron laser produce nonlinear phenomena that differ dramatically from the linear x-ray-matter interaction processes that are encountered at synchrotron x-ray sources. We use intense x-ray pulses of sub-10-fs duration to first reveal and subsequently drive the 1s↔2p resonance in singly ionized neon. This photon-driven cycling of an inner-shell electron modifies the Auger decay process, as evidenced by line shape modification. Our work demonstrates the propensity of high-fluence, femtosecond x-ray pulses to alter the target within a single pulse, i.e., to unveil hidden resonances, by cracking open inner shells energetically inaccessible via single-photon absorption, and to consequently trigger damaging electron cascades at unexpectedly low photon energies. |
| doi_str_mv | 10.1103/PhysRevLett.107.233001 |
| format | Article |
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Our work demonstrates the propensity of high-fluence, femtosecond x-ray pulses to alter the target within a single pulse, i.e., to unveil hidden resonances, by cracking open inner shells energetically inaccessible via single-photon absorption, and to consequently trigger damaging electron cascades at unexpectedly low photon energies.</description><identifier>ISSN: 0031-9007</identifier><identifier>EISSN: 1079-7114</identifier><identifier>DOI: 10.1103/PhysRevLett.107.233001</identifier><identifier>PMID: 22182083</identifier><language>eng</language><publisher>United States</publisher><ispartof>Phys. Rev. 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Our work demonstrates the propensity of high-fluence, femtosecond x-ray pulses to alter the target within a single pulse, i.e., to unveil hidden resonances, by cracking open inner shells energetically inaccessible via single-photon absorption, and to consequently trigger damaging electron cascades at unexpectedly low photon energies.</abstract><cop>United States</cop><pmid>22182083</pmid><doi>10.1103/PhysRevLett.107.233001</doi><tpages>1</tpages><oa>free_for_read</oa></addata></record> |
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| title | Unveiling and driving hidden resonances with high-fluence, high-intensity x-ray pulses |
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