Insulating State and Breakdown of Fermi Liquid Description in Molecular-Scale Single-Crystalline Wires of Gold
Electrical transport measurements on ultrathin single-crystalline Au nanowires, synthesized via a wet chemical route, show an unexpected insulating behavior. The linear response electrical resistance exhibits a power-law dependence on temperature. In addition, the variation of current over a wide ra...
Gespeichert in:
Veröffentlicht in: | ACS nano 2011-10, Vol.5 (10), p.8398-8403 |
---|---|
Hauptverfasser: | , , , , |
Format: | Artikel |
Sprache: | eng |
Schlagworte: | |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
container_end_page | 8403 |
---|---|
container_issue | 10 |
container_start_page | 8398 |
container_title | ACS nano |
container_volume | 5 |
creator | Chandni, U Kundu, Paromita Singh, Abhishek K Ravishankar, N Ghosh, Arindam |
description | Electrical transport measurements on ultrathin single-crystalline Au nanowires, synthesized via a wet chemical route, show an unexpected insulating behavior. The linear response electrical resistance exhibits a power-law dependence on temperature. In addition, the variation of current over a wide range of temperature and voltage obeys a universal scaling relation that provides compelling evidence for a non-Fermi liquid behavior. Our results demonstrate that the quantum ground state in ultrathin nanowires of simple metallic systems can be radically different from their bulk counterparts and can be described in terms of a Tomonaga–Luttinger liquid (TLL), in the presence of remarkably strong electron–electron interactions. |
doi_str_mv | 10.1021/nn2031935 |
format | Article |
fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_900641094</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>900641094</sourcerecordid><originalsourceid>FETCH-LOGICAL-a413t-c503a09367daf3156e6468750090dc10b61c64de8919095e2bce14bd801649ba3</originalsourceid><addsrcrecordid>eNp9kT1P5DAQhi3Eie-CP4DcILgixziJnbiE5eOQFlEsCLrIsWeRwWsvdqIT_x6j5bY6XTVTPPPM6B1CDhn8YlCyM-9LqJis-AbZyUUU0IrnzXXP2TbZTekVgDdtI7bIdslkXXLBd4i_9Wl0arD-hc4GNSBV3tCLiOrNhD-ehjm9xriwdGrfR2voJSYd7XKwwVPr6V1wqPN8LGZaOaSz7HFYTOJHGpRz1iN9shHTl-cmOLNPfsyVS3jwXffI4_XVw-R3Mb2_uZ2cTwtVs2ooNIdKQb6-MWpeMS5Q1KJtOIAEoxn0gmlRG2wlkyA5lr1GVvemBSZq2atqj5ysvMsY3kdMQ7ewSaNzymMYUycBRM1A1pk8_S_JGlHm3PLqjP5coTqGlCLOu2W0CxU_Ogbd1yO69SMye_StHfsFmjX5N_kMHK8ApVP3Gsbocx7_EH0CHSuNuQ</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1762057500</pqid></control><display><type>article</type><title>Insulating State and Breakdown of Fermi Liquid Description in Molecular-Scale Single-Crystalline Wires of Gold</title><source>ACS Publications</source><creator>Chandni, U ; Kundu, Paromita ; Singh, Abhishek K ; Ravishankar, N ; Ghosh, Arindam</creator><creatorcontrib>Chandni, U ; Kundu, Paromita ; Singh, Abhishek K ; Ravishankar, N ; Ghosh, Arindam</creatorcontrib><description>Electrical transport measurements on ultrathin single-crystalline Au nanowires, synthesized via a wet chemical route, show an unexpected insulating behavior. The linear response electrical resistance exhibits a power-law dependence on temperature. In addition, the variation of current over a wide range of temperature and voltage obeys a universal scaling relation that provides compelling evidence for a non-Fermi liquid behavior. Our results demonstrate that the quantum ground state in ultrathin nanowires of simple metallic systems can be radically different from their bulk counterparts and can be described in terms of a Tomonaga–Luttinger liquid (TLL), in the presence of remarkably strong electron–electron interactions.</description><identifier>ISSN: 1936-0851</identifier><identifier>EISSN: 1936-086X</identifier><identifier>DOI: 10.1021/nn2031935</identifier><identifier>PMID: 21942565</identifier><language>eng</language><publisher>United States: American Chemical Society</publisher><subject>Breakdown ; Electric potential ; Electric wire ; Fermi liquids ; Gold ; Liquids ; Nanowires ; Single crystals ; Voltage</subject><ispartof>ACS nano, 2011-10, Vol.5 (10), p.8398-8403</ispartof><rights>Copyright © 2011 American Chemical Society</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a413t-c503a09367daf3156e6468750090dc10b61c64de8919095e2bce14bd801649ba3</citedby><cites>FETCH-LOGICAL-a413t-c503a09367daf3156e6468750090dc10b61c64de8919095e2bce14bd801649ba3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/nn2031935$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/nn2031935$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,776,780,2752,27053,27901,27902,56713,56763</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/21942565$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Chandni, U</creatorcontrib><creatorcontrib>Kundu, Paromita</creatorcontrib><creatorcontrib>Singh, Abhishek K</creatorcontrib><creatorcontrib>Ravishankar, N</creatorcontrib><creatorcontrib>Ghosh, Arindam</creatorcontrib><title>Insulating State and Breakdown of Fermi Liquid Description in Molecular-Scale Single-Crystalline Wires of Gold</title><title>ACS nano</title><addtitle>ACS Nano</addtitle><description>Electrical transport measurements on ultrathin single-crystalline Au nanowires, synthesized via a wet chemical route, show an unexpected insulating behavior. The linear response electrical resistance exhibits a power-law dependence on temperature. In addition, the variation of current over a wide range of temperature and voltage obeys a universal scaling relation that provides compelling evidence for a non-Fermi liquid behavior. Our results demonstrate that the quantum ground state in ultrathin nanowires of simple metallic systems can be radically different from their bulk counterparts and can be described in terms of a Tomonaga–Luttinger liquid (TLL), in the presence of remarkably strong electron–electron interactions.</description><subject>Breakdown</subject><subject>Electric potential</subject><subject>Electric wire</subject><subject>Fermi liquids</subject><subject>Gold</subject><subject>Liquids</subject><subject>Nanowires</subject><subject>Single crystals</subject><subject>Voltage</subject><issn>1936-0851</issn><issn>1936-086X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2011</creationdate><recordtype>article</recordtype><recordid>eNp9kT1P5DAQhi3Eie-CP4DcILgixziJnbiE5eOQFlEsCLrIsWeRwWsvdqIT_x6j5bY6XTVTPPPM6B1CDhn8YlCyM-9LqJis-AbZyUUU0IrnzXXP2TbZTekVgDdtI7bIdslkXXLBd4i_9Wl0arD-hc4GNSBV3tCLiOrNhD-ehjm9xriwdGrfR2voJSYd7XKwwVPr6V1wqPN8LGZaOaSz7HFYTOJHGpRz1iN9shHTl-cmOLNPfsyVS3jwXffI4_XVw-R3Mb2_uZ2cTwtVs2ooNIdKQb6-MWpeMS5Q1KJtOIAEoxn0gmlRG2wlkyA5lr1GVvemBSZq2atqj5ysvMsY3kdMQ7ewSaNzymMYUycBRM1A1pk8_S_JGlHm3PLqjP5coTqGlCLOu2W0CxU_Ogbd1yO69SMye_StHfsFmjX5N_kMHK8ApVP3Gsbocx7_EH0CHSuNuQ</recordid><startdate>20111025</startdate><enddate>20111025</enddate><creator>Chandni, U</creator><creator>Kundu, Paromita</creator><creator>Singh, Abhishek K</creator><creator>Ravishankar, N</creator><creator>Ghosh, Arindam</creator><general>American Chemical Society</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope></search><sort><creationdate>20111025</creationdate><title>Insulating State and Breakdown of Fermi Liquid Description in Molecular-Scale Single-Crystalline Wires of Gold</title><author>Chandni, U ; Kundu, Paromita ; Singh, Abhishek K ; Ravishankar, N ; Ghosh, Arindam</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a413t-c503a09367daf3156e6468750090dc10b61c64de8919095e2bce14bd801649ba3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2011</creationdate><topic>Breakdown</topic><topic>Electric potential</topic><topic>Electric wire</topic><topic>Fermi liquids</topic><topic>Gold</topic><topic>Liquids</topic><topic>Nanowires</topic><topic>Single crystals</topic><topic>Voltage</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chandni, U</creatorcontrib><creatorcontrib>Kundu, Paromita</creatorcontrib><creatorcontrib>Singh, Abhishek K</creatorcontrib><creatorcontrib>Ravishankar, N</creatorcontrib><creatorcontrib>Ghosh, Arindam</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>ACS nano</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Chandni, U</au><au>Kundu, Paromita</au><au>Singh, Abhishek K</au><au>Ravishankar, N</au><au>Ghosh, Arindam</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Insulating State and Breakdown of Fermi Liquid Description in Molecular-Scale Single-Crystalline Wires of Gold</atitle><jtitle>ACS nano</jtitle><addtitle>ACS Nano</addtitle><date>2011-10-25</date><risdate>2011</risdate><volume>5</volume><issue>10</issue><spage>8398</spage><epage>8403</epage><pages>8398-8403</pages><issn>1936-0851</issn><eissn>1936-086X</eissn><abstract>Electrical transport measurements on ultrathin single-crystalline Au nanowires, synthesized via a wet chemical route, show an unexpected insulating behavior. The linear response electrical resistance exhibits a power-law dependence on temperature. In addition, the variation of current over a wide range of temperature and voltage obeys a universal scaling relation that provides compelling evidence for a non-Fermi liquid behavior. Our results demonstrate that the quantum ground state in ultrathin nanowires of simple metallic systems can be radically different from their bulk counterparts and can be described in terms of a Tomonaga–Luttinger liquid (TLL), in the presence of remarkably strong electron–electron interactions.</abstract><cop>United States</cop><pub>American Chemical Society</pub><pmid>21942565</pmid><doi>10.1021/nn2031935</doi><tpages>6</tpages></addata></record> |
fulltext | fulltext |
identifier | ISSN: 1936-0851 |
ispartof | ACS nano, 2011-10, Vol.5 (10), p.8398-8403 |
issn | 1936-0851 1936-086X |
language | eng |
recordid | cdi_proquest_miscellaneous_900641094 |
source | ACS Publications |
subjects | Breakdown Electric potential Electric wire Fermi liquids Gold Liquids Nanowires Single crystals Voltage |
title | Insulating State and Breakdown of Fermi Liquid Description in Molecular-Scale Single-Crystalline Wires of Gold |
url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-29T23%3A43%3A25IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Insulating%20State%20and%20Breakdown%20of%20Fermi%20Liquid%20Description%20in%20Molecular-Scale%20Single-Crystalline%20Wires%20of%20Gold&rft.jtitle=ACS%20nano&rft.au=Chandni,%20U&rft.date=2011-10-25&rft.volume=5&rft.issue=10&rft.spage=8398&rft.epage=8403&rft.pages=8398-8403&rft.issn=1936-0851&rft.eissn=1936-086X&rft_id=info:doi/10.1021/nn2031935&rft_dat=%3Cproquest_cross%3E900641094%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1762057500&rft_id=info:pmid/21942565&rfr_iscdi=true |