Can Amorphous Nuclei Grow Crystalline Clathrates? The Size and Crystallinity of Critical Clathrate Nuclei

Recent studies reveal that amorphous intermediates are involved in the formation of clathrate hydrates under conditions of high driving force, raising two questions: first, how could amorphous nuclei grow into crystalline clathrates and, second, whether amorphous nuclei are intermediates in the form...

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Veröffentlicht in:Journal of the American Chemical Society 2011-04, Vol.133 (16), p.6458-6463
Hauptverfasser: Jacobson, Liam C, Molinero, Valeria
Format: Artikel
Sprache:eng
Online-Zugang:Volltext
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