Fine particle emission profile for a large coke production facility based on highly time-resolved fence line measurements
This paper presents a fine particle emission profile for a large metallurgical coke production facility. The profile is developed from highly time-resolved, ambient air quality measurements made at a fence line site adjacent to the plant. A fence line approach was employed because the coke plant has...
Gespeichert in:
| Veröffentlicht in: | Atmospheric environment (1994) 2005-11, Vol.39 (36), p.6719-6733 |
|---|---|
| Hauptverfasser: | , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 6733 |
|---|---|
| container_issue | 36 |
| container_start_page | 6719 |
| container_title | Atmospheric environment (1994) |
| container_volume | 39 |
| creator | Weitkamp, Emily A. Lipsky, Eric M. Pancras, Patrick J. Ondov, John M. Polidori, Andrea Turpin, Barbara J. Robinson, Allen L. |
| description | This paper presents a fine particle emission profile for a large metallurgical coke production facility. The profile is developed from highly time-resolved, ambient air quality measurements made at a fence line site adjacent to the plant. A fence line approach was employed because the coke plant has hundreds of stacks and other emission points, making it difficult to develop an integrated, facility-wide emission profile using stack sampling techniques. Continuous or semi-continuous measurements of PM
2.5 mass, PM
10 mass, SO
2, NO
x
, organic and elemental carbon (OC and EC), particle size and number, 11 trace metals, wind direction and wind speed were made. Background pollutant levels were also measured. A combination of highly time-resolved meteorology and air quality data were used to determine when the coke facility emissions influenced the sampling site. Concentrations for most pollutants at the fence line site were one to two orders of magnitude higher than background levels when the facility plume heavily influenced the fence line site. Highly time-resolved measurements are essential to resolve these relatively short-duration, large spikes in pollutant concentrations. Simply measuring wind direction is insufficient. From these highly time-resolved measurements an average PM
2.5 emission profile for the coke facility was developed. The profile is dominated by OC (40%±9% of PM
2.5 mass emissions) and EC (25%±5% of PM
2.5 mass emissions). Significant contributions of certain trace metals were also observed, including As, Zn, Se, and Pb. The particle emissions are dominated by the fine fraction, with PM
2.5 estimated to contribute 84%±14% of the PM
10 mass. |
| doi_str_mv | 10.1016/j.atmosenv.2005.06.028 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_817610614</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><els_id>S1352231005005467</els_id><sourcerecordid>1671548358</sourcerecordid><originalsourceid>FETCH-LOGICAL-c500t-2e73a40bfb5e0d67a09608837f426853ad00429c1601fb49d8e0b83d08708bae3</originalsourceid><addsrcrecordid>eNqFkk1r3DAQhk1oIWnSv1B06cfFzujDknxrCUkbCOTSnoUsjxJtZXsreRf231dmU3rLniRmnpl3hnmr6gOFhgKV15vGLuOccdo3DKBtQDbA9Fl1QbXiNdNCvCl_3rKacQrn1bucNwDAVacuqsNdmJBsbVqCi0hwDDmHeSLbNPtQAn5OxJJo0xMSN__GNTHs3LIy3roQw3Igvc04kBJ5Dk_P8UCWMGKdMM9xX-IeJ4ckrjoj2rxLOOK05Kvqrbcx4_uX97L6dXf78-ZH_fD4_f7m20PtWoClZqi4FdD7vkUYpLLQSdCaKy-Y1C23A4BgnaMSqO9FN2iEXvMBtALdW-SX1edj3zL5nx3mxZQdHcZoJ5x32WiqJAVJRSE_vUqyTuqu69hJkCrGWylW8MvroFS0FZq3-nRPUcYsOxZQHkGX5pwTerNNYbTpYCiY1RBmY_4ZwqyGMCBNMUQp_PiiYLOz0Sc7uZD_V5ehQbWqcF-PHJar7AMmk11YbziEhG4xwxxOSf0F6CfP1A</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>14761601</pqid></control><display><type>article</type><title>Fine particle emission profile for a large coke production facility based on highly time-resolved fence line measurements</title><source>Elsevier ScienceDirect Journals</source><creator>Weitkamp, Emily A. ; Lipsky, Eric M. ; Pancras, Patrick J. ; Ondov, John M. ; Polidori, Andrea ; Turpin, Barbara J. ; Robinson, Allen L.</creator><creatorcontrib>Weitkamp, Emily A. ; Lipsky, Eric M. ; Pancras, Patrick J. ; Ondov, John M. ; Polidori, Andrea ; Turpin, Barbara J. ; Robinson, Allen L.</creatorcontrib><description>This paper presents a fine particle emission profile for a large metallurgical coke production facility. The profile is developed from highly time-resolved, ambient air quality measurements made at a fence line site adjacent to the plant. A fence line approach was employed because the coke plant has hundreds of stacks and other emission points, making it difficult to develop an integrated, facility-wide emission profile using stack sampling techniques. Continuous or semi-continuous measurements of PM
2.5 mass, PM
10 mass, SO
2, NO
x
, organic and elemental carbon (OC and EC), particle size and number, 11 trace metals, wind direction and wind speed were made. Background pollutant levels were also measured. A combination of highly time-resolved meteorology and air quality data were used to determine when the coke facility emissions influenced the sampling site. Concentrations for most pollutants at the fence line site were one to two orders of magnitude higher than background levels when the facility plume heavily influenced the fence line site. Highly time-resolved measurements are essential to resolve these relatively short-duration, large spikes in pollutant concentrations. Simply measuring wind direction is insufficient. From these highly time-resolved measurements an average PM
2.5 emission profile for the coke facility was developed. The profile is dominated by OC (40%±9% of PM
2.5 mass emissions) and EC (25%±5% of PM
2.5 mass emissions). Significant contributions of certain trace metals were also observed, including As, Zn, Se, and Pb. The particle emissions are dominated by the fine fraction, with PM
2.5 estimated to contribute 84%±14% of the PM
10 mass.</description><identifier>ISSN: 1352-2310</identifier><identifier>EISSN: 1873-2844</identifier><identifier>DOI: 10.1016/j.atmosenv.2005.06.028</identifier><language>eng</language><publisher>Oxford: Elsevier Ltd</publisher><subject>Air quality ; Applied sciences ; Atmospheric pollution ; Coal ; Coke ; Emission ; Emission characterization ; Emission inventory ; Emission profile ; Exact sciences and technology ; Fences ; Metallurgical coke production ; Other pollution sources in industry ; Particle emission ; PM 2.5 ; Pollutants ; Pollution ; Pollution sources. Measurement results ; Primary OC ; Receptor modeling ; Sampling ; Source sampling ; Wind direction</subject><ispartof>Atmospheric environment (1994), 2005-11, Vol.39 (36), p.6719-6733</ispartof><rights>2005 Elsevier Ltd</rights><rights>2006 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c500t-2e73a40bfb5e0d67a09608837f426853ad00429c1601fb49d8e0b83d08708bae3</citedby><cites>FETCH-LOGICAL-c500t-2e73a40bfb5e0d67a09608837f426853ad00429c1601fb49d8e0b83d08708bae3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S1352231005005467$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3537,27901,27902,65306</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=17230757$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>Weitkamp, Emily A.</creatorcontrib><creatorcontrib>Lipsky, Eric M.</creatorcontrib><creatorcontrib>Pancras, Patrick J.</creatorcontrib><creatorcontrib>Ondov, John M.</creatorcontrib><creatorcontrib>Polidori, Andrea</creatorcontrib><creatorcontrib>Turpin, Barbara J.</creatorcontrib><creatorcontrib>Robinson, Allen L.</creatorcontrib><title>Fine particle emission profile for a large coke production facility based on highly time-resolved fence line measurements</title><title>Atmospheric environment (1994)</title><description>This paper presents a fine particle emission profile for a large metallurgical coke production facility. The profile is developed from highly time-resolved, ambient air quality measurements made at a fence line site adjacent to the plant. A fence line approach was employed because the coke plant has hundreds of stacks and other emission points, making it difficult to develop an integrated, facility-wide emission profile using stack sampling techniques. Continuous or semi-continuous measurements of PM
2.5 mass, PM
10 mass, SO
2, NO
x
, organic and elemental carbon (OC and EC), particle size and number, 11 trace metals, wind direction and wind speed were made. Background pollutant levels were also measured. A combination of highly time-resolved meteorology and air quality data were used to determine when the coke facility emissions influenced the sampling site. Concentrations for most pollutants at the fence line site were one to two orders of magnitude higher than background levels when the facility plume heavily influenced the fence line site. Highly time-resolved measurements are essential to resolve these relatively short-duration, large spikes in pollutant concentrations. Simply measuring wind direction is insufficient. From these highly time-resolved measurements an average PM
2.5 emission profile for the coke facility was developed. The profile is dominated by OC (40%±9% of PM
2.5 mass emissions) and EC (25%±5% of PM
2.5 mass emissions). Significant contributions of certain trace metals were also observed, including As, Zn, Se, and Pb. The particle emissions are dominated by the fine fraction, with PM
2.5 estimated to contribute 84%±14% of the PM
10 mass.</description><subject>Air quality</subject><subject>Applied sciences</subject><subject>Atmospheric pollution</subject><subject>Coal</subject><subject>Coke</subject><subject>Emission</subject><subject>Emission characterization</subject><subject>Emission inventory</subject><subject>Emission profile</subject><subject>Exact sciences and technology</subject><subject>Fences</subject><subject>Metallurgical coke production</subject><subject>Other pollution sources in industry</subject><subject>Particle emission</subject><subject>PM 2.5</subject><subject>Pollutants</subject><subject>Pollution</subject><subject>Pollution sources. Measurement results</subject><subject>Primary OC</subject><subject>Receptor modeling</subject><subject>Sampling</subject><subject>Source sampling</subject><subject>Wind direction</subject><issn>1352-2310</issn><issn>1873-2844</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2005</creationdate><recordtype>article</recordtype><recordid>eNqFkk1r3DAQhk1oIWnSv1B06cfFzujDknxrCUkbCOTSnoUsjxJtZXsreRf231dmU3rLniRmnpl3hnmr6gOFhgKV15vGLuOccdo3DKBtQDbA9Fl1QbXiNdNCvCl_3rKacQrn1bucNwDAVacuqsNdmJBsbVqCi0hwDDmHeSLbNPtQAn5OxJJo0xMSN__GNTHs3LIy3roQw3Igvc04kBJ5Dk_P8UCWMGKdMM9xX-IeJ4ckrjoj2rxLOOK05Kvqrbcx4_uX97L6dXf78-ZH_fD4_f7m20PtWoClZqi4FdD7vkUYpLLQSdCaKy-Y1C23A4BgnaMSqO9FN2iEXvMBtALdW-SX1edj3zL5nx3mxZQdHcZoJ5x32WiqJAVJRSE_vUqyTuqu69hJkCrGWylW8MvroFS0FZq3-nRPUcYsOxZQHkGX5pwTerNNYbTpYCiY1RBmY_4ZwqyGMCBNMUQp_PiiYLOz0Sc7uZD_V5ehQbWqcF-PHJar7AMmk11YbziEhG4xwxxOSf0F6CfP1A</recordid><startdate>20051101</startdate><enddate>20051101</enddate><creator>Weitkamp, Emily A.</creator><creator>Lipsky, Eric M.</creator><creator>Pancras, Patrick J.</creator><creator>Ondov, John M.</creator><creator>Polidori, Andrea</creator><creator>Turpin, Barbara J.</creator><creator>Robinson, Allen L.</creator><general>Elsevier Ltd</general><general>Elsevier Science</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7ST</scope><scope>C1K</scope><scope>SOI</scope><scope>7SU</scope><scope>8FD</scope><scope>FR3</scope><scope>H8D</scope><scope>KR7</scope><scope>L7M</scope><scope>7TG</scope><scope>7TV</scope><scope>KL.</scope><scope>8BQ</scope><scope>JG9</scope></search><sort><creationdate>20051101</creationdate><title>Fine particle emission profile for a large coke production facility based on highly time-resolved fence line measurements</title><author>Weitkamp, Emily A. ; Lipsky, Eric M. ; Pancras, Patrick J. ; Ondov, John M. ; Polidori, Andrea ; Turpin, Barbara J. ; Robinson, Allen L.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c500t-2e73a40bfb5e0d67a09608837f426853ad00429c1601fb49d8e0b83d08708bae3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2005</creationdate><topic>Air quality</topic><topic>Applied sciences</topic><topic>Atmospheric pollution</topic><topic>Coal</topic><topic>Coke</topic><topic>Emission</topic><topic>Emission characterization</topic><topic>Emission inventory</topic><topic>Emission profile</topic><topic>Exact sciences and technology</topic><topic>Fences</topic><topic>Metallurgical coke production</topic><topic>Other pollution sources in industry</topic><topic>Particle emission</topic><topic>PM 2.5</topic><topic>Pollutants</topic><topic>Pollution</topic><topic>Pollution sources. Measurement results</topic><topic>Primary OC</topic><topic>Receptor modeling</topic><topic>Sampling</topic><topic>Source sampling</topic><topic>Wind direction</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Weitkamp, Emily A.</creatorcontrib><creatorcontrib>Lipsky, Eric M.</creatorcontrib><creatorcontrib>Pancras, Patrick J.</creatorcontrib><creatorcontrib>Ondov, John M.</creatorcontrib><creatorcontrib>Polidori, Andrea</creatorcontrib><creatorcontrib>Turpin, Barbara J.</creatorcontrib><creatorcontrib>Robinson, Allen L.</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Environment Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Environment Abstracts</collection><collection>Environmental Engineering Abstracts</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Aerospace Database</collection><collection>Civil Engineering Abstracts</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Pollution Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>METADEX</collection><collection>Materials Research Database</collection><jtitle>Atmospheric environment (1994)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Weitkamp, Emily A.</au><au>Lipsky, Eric M.</au><au>Pancras, Patrick J.</au><au>Ondov, John M.</au><au>Polidori, Andrea</au><au>Turpin, Barbara J.</au><au>Robinson, Allen L.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Fine particle emission profile for a large coke production facility based on highly time-resolved fence line measurements</atitle><jtitle>Atmospheric environment (1994)</jtitle><date>2005-11-01</date><risdate>2005</risdate><volume>39</volume><issue>36</issue><spage>6719</spage><epage>6733</epage><pages>6719-6733</pages><issn>1352-2310</issn><eissn>1873-2844</eissn><abstract>This paper presents a fine particle emission profile for a large metallurgical coke production facility. The profile is developed from highly time-resolved, ambient air quality measurements made at a fence line site adjacent to the plant. A fence line approach was employed because the coke plant has hundreds of stacks and other emission points, making it difficult to develop an integrated, facility-wide emission profile using stack sampling techniques. Continuous or semi-continuous measurements of PM
2.5 mass, PM
10 mass, SO
2, NO
x
, organic and elemental carbon (OC and EC), particle size and number, 11 trace metals, wind direction and wind speed were made. Background pollutant levels were also measured. A combination of highly time-resolved meteorology and air quality data were used to determine when the coke facility emissions influenced the sampling site. Concentrations for most pollutants at the fence line site were one to two orders of magnitude higher than background levels when the facility plume heavily influenced the fence line site. Highly time-resolved measurements are essential to resolve these relatively short-duration, large spikes in pollutant concentrations. Simply measuring wind direction is insufficient. From these highly time-resolved measurements an average PM
2.5 emission profile for the coke facility was developed. The profile is dominated by OC (40%±9% of PM
2.5 mass emissions) and EC (25%±5% of PM
2.5 mass emissions). Significant contributions of certain trace metals were also observed, including As, Zn, Se, and Pb. The particle emissions are dominated by the fine fraction, with PM
2.5 estimated to contribute 84%±14% of the PM
10 mass.</abstract><cop>Oxford</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.atmosenv.2005.06.028</doi><tpages>15</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1352-2310 |
| ispartof | Atmospheric environment (1994), 2005-11, Vol.39 (36), p.6719-6733 |
| issn | 1352-2310 1873-2844 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_817610614 |
| source | Elsevier ScienceDirect Journals |
| subjects | Air quality Applied sciences Atmospheric pollution Coal Coke Emission Emission characterization Emission inventory Emission profile Exact sciences and technology Fences Metallurgical coke production Other pollution sources in industry Particle emission PM 2.5 Pollutants Pollution Pollution sources. Measurement results Primary OC Receptor modeling Sampling Source sampling Wind direction |
| title | Fine particle emission profile for a large coke production facility based on highly time-resolved fence line measurements |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-05T16%3A29%3A16IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Fine%20particle%20emission%20profile%20for%20a%20large%20coke%20production%20facility%20based%20on%20highly%20time-resolved%20fence%20line%20measurements&rft.jtitle=Atmospheric%20environment%20(1994)&rft.au=Weitkamp,%20Emily%20A.&rft.date=2005-11-01&rft.volume=39&rft.issue=36&rft.spage=6719&rft.epage=6733&rft.pages=6719-6733&rft.issn=1352-2310&rft.eissn=1873-2844&rft_id=info:doi/10.1016/j.atmosenv.2005.06.028&rft_dat=%3Cproquest_cross%3E1671548358%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=14761601&rft_id=info:pmid/&rft_els_id=S1352231005005467&rfr_iscdi=true |