Key site variables governing the functional characteristics of Dissolved Natural Organic Matter (DNOM) in Nordic forested catchments
The objective of this study was to extract and evaluate key catchment characteristics explaining the main variation in properties of dissolved natural organic matter (DNOM) in surface waters draining each catchment. A number of classical and sophisticated DNOM characterisation methodologies were use...
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| Veröffentlicht in: | Aquatic sciences 2004-06, Vol.66 (2), p.195-210 |
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| creator | VOGT, Rolf D AKKANEN, Jarkko PFLUGMACHER, Stephan STARR, Mike STEINBERG, Christian E. W SCHMITT-KOPPLIN, Philippe ZSOLNAY, Adam ANDERSEN, Dag Olav BRÜGGEMANN, Rainer CHATTERJEE, Bimal GJESSING, Egil KUKKONEN, Jussi V. K LARSEN, Hakon E LUSTER, Jorg PAUL, Andrea |
| description | The objective of this study was to extract and evaluate key catchment characteristics explaining the main variation in properties of dissolved natural organic matter (DNOM) in surface waters draining each catchment. A number of classical and sophisticated DNOM characterisation methodologies were used for this purpose. The explanatory capability of site characteristics on the variation in descriptors of DNOM, including elemental analysis (EA), DOC fractionation, SEC, CZE, CGE, UV/Vis- and FTIR spectra, FES, TLS, ESR, ESI/MS, super(13)C-CPMAS-NMR, potentiometric pH titration as well as functional characteristics such as biodegradability, and the response of macrophyte and PAH partitioning coefficients were evaluated. The sampling sites were all natural, coniferous, heathery-forested catchments with bogs, forming a climatic, anthropogenic deposition and proportional biotope cover gradient. Correlations to the main principal components, as well as a correlation matrix, singled out total S-deposition as the key explanatory site parameter, accounting for most of the variation in DNOM descriptors. Other significant factors were H super(+) concentration, length of growing season, biotope coverage (i.e., peatland/ or lake/watershed ratio), site elevation and TOC concentration. Total sulphur (S) deposition was strongly negatively correlated to the molecular weight, aromaticity, carboxylic acidity and sorption capacity of PAH. A greater proportion of lake and Histosol biotopes of the sampling sites were reflected in a greater aliphatic character of the DNOM. PCA clustering of samples from the same site in spring and fall showed a basic site-specific DNOM quality and a weak season effect. The Hasse diagram technique (a method of partial order theory) was used to show, for instance, how the relative Histosol coverage may determine NOM quality and, in turn, how this coincides with high macrophyte response. |
| doi_str_mv | 10.1007/s00027-004-0710-0 |
| format | Article |
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W ; SCHMITT-KOPPLIN, Philippe ; ZSOLNAY, Adam ; ANDERSEN, Dag Olav ; BRÜGGEMANN, Rainer ; CHATTERJEE, Bimal ; GJESSING, Egil ; KUKKONEN, Jussi V. K ; LARSEN, Hakon E ; LUSTER, Jorg ; PAUL, Andrea</creator><creatorcontrib>VOGT, Rolf D ; AKKANEN, Jarkko ; PFLUGMACHER, Stephan ; STARR, Mike ; STEINBERG, Christian E. W ; SCHMITT-KOPPLIN, Philippe ; ZSOLNAY, Adam ; ANDERSEN, Dag Olav ; BRÜGGEMANN, Rainer ; CHATTERJEE, Bimal ; GJESSING, Egil ; KUKKONEN, Jussi V. K ; LARSEN, Hakon E ; LUSTER, Jorg ; PAUL, Andrea</creatorcontrib><description>The objective of this study was to extract and evaluate key catchment characteristics explaining the main variation in properties of dissolved natural organic matter (DNOM) in surface waters draining each catchment. A number of classical and sophisticated DNOM characterisation methodologies were used for this purpose. The explanatory capability of site characteristics on the variation in descriptors of DNOM, including elemental analysis (EA), DOC fractionation, SEC, CZE, CGE, UV/Vis- and FTIR spectra, FES, TLS, ESR, ESI/MS, super(13)C-CPMAS-NMR, potentiometric pH titration as well as functional characteristics such as biodegradability, and the response of macrophyte and PAH partitioning coefficients were evaluated. The sampling sites were all natural, coniferous, heathery-forested catchments with bogs, forming a climatic, anthropogenic deposition and proportional biotope cover gradient. Correlations to the main principal components, as well as a correlation matrix, singled out total S-deposition as the key explanatory site parameter, accounting for most of the variation in DNOM descriptors. Other significant factors were H super(+) concentration, length of growing season, biotope coverage (i.e., peatland/ or lake/watershed ratio), site elevation and TOC concentration. Total sulphur (S) deposition was strongly negatively correlated to the molecular weight, aromaticity, carboxylic acidity and sorption capacity of PAH. A greater proportion of lake and Histosol biotopes of the sampling sites were reflected in a greater aliphatic character of the DNOM. PCA clustering of samples from the same site in spring and fall showed a basic site-specific DNOM quality and a weak season effect. The Hasse diagram technique (a method of partial order theory) was used to show, for instance, how the relative Histosol coverage may determine NOM quality and, in turn, how this coincides with high macrophyte response.</description><identifier>ISSN: 1015-1621</identifier><identifier>EISSN: 1420-9055</identifier><identifier>DOI: 10.1007/s00027-004-0710-0</identifier><language>eng</language><publisher>Heidelberg: Springer</publisher><subject>Acidity ; Anthropogenic factors ; Aquatic plants ; Biodegradation ; Biotopes ; Catchments ; Earth sciences ; Earth, ocean, space ; Engineering and environment geology. Geothermics ; Exact sciences and technology ; Forest watersheds ; Fractionation ; Freshwater ; Geochemistry ; Growing season ; Hydrology ; Hydrology. Hydrogeology ; Lakes ; Mineralogy ; Molecular weight ; Organic matter ; Pollution, environment geology ; Silicates ; Surface water ; Water geochemistry</subject><ispartof>Aquatic sciences, 2004-06, Vol.66 (2), p.195-210</ispartof><rights>2004 INIST-CNRS</rights><rights>EAWAG 2004</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a386t-104a4dbc3af5686f6bbd4e3005b0921c38111bc3dd13c1eaad700e07563ed5fe3</citedby></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>309,310,314,780,784,789,790,23929,23930,25139,27923,27924</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=15879910$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>VOGT, Rolf D</creatorcontrib><creatorcontrib>AKKANEN, Jarkko</creatorcontrib><creatorcontrib>PFLUGMACHER, Stephan</creatorcontrib><creatorcontrib>STARR, Mike</creatorcontrib><creatorcontrib>STEINBERG, Christian E. W</creatorcontrib><creatorcontrib>SCHMITT-KOPPLIN, Philippe</creatorcontrib><creatorcontrib>ZSOLNAY, Adam</creatorcontrib><creatorcontrib>ANDERSEN, Dag Olav</creatorcontrib><creatorcontrib>BRÜGGEMANN, Rainer</creatorcontrib><creatorcontrib>CHATTERJEE, Bimal</creatorcontrib><creatorcontrib>GJESSING, Egil</creatorcontrib><creatorcontrib>KUKKONEN, Jussi V. K</creatorcontrib><creatorcontrib>LARSEN, Hakon E</creatorcontrib><creatorcontrib>LUSTER, Jorg</creatorcontrib><creatorcontrib>PAUL, Andrea</creatorcontrib><title>Key site variables governing the functional characteristics of Dissolved Natural Organic Matter (DNOM) in Nordic forested catchments</title><title>Aquatic sciences</title><description>The objective of this study was to extract and evaluate key catchment characteristics explaining the main variation in properties of dissolved natural organic matter (DNOM) in surface waters draining each catchment. A number of classical and sophisticated DNOM characterisation methodologies were used for this purpose. The explanatory capability of site characteristics on the variation in descriptors of DNOM, including elemental analysis (EA), DOC fractionation, SEC, CZE, CGE, UV/Vis- and FTIR spectra, FES, TLS, ESR, ESI/MS, super(13)C-CPMAS-NMR, potentiometric pH titration as well as functional characteristics such as biodegradability, and the response of macrophyte and PAH partitioning coefficients were evaluated. The sampling sites were all natural, coniferous, heathery-forested catchments with bogs, forming a climatic, anthropogenic deposition and proportional biotope cover gradient. Correlations to the main principal components, as well as a correlation matrix, singled out total S-deposition as the key explanatory site parameter, accounting for most of the variation in DNOM descriptors. Other significant factors were H super(+) concentration, length of growing season, biotope coverage (i.e., peatland/ or lake/watershed ratio), site elevation and TOC concentration. Total sulphur (S) deposition was strongly negatively correlated to the molecular weight, aromaticity, carboxylic acidity and sorption capacity of PAH. A greater proportion of lake and Histosol biotopes of the sampling sites were reflected in a greater aliphatic character of the DNOM. PCA clustering of samples from the same site in spring and fall showed a basic site-specific DNOM quality and a weak season effect. The Hasse diagram technique (a method of partial order theory) was used to show, for instance, how the relative Histosol coverage may determine NOM quality and, in turn, how this coincides with high macrophyte response.</description><subject>Acidity</subject><subject>Anthropogenic factors</subject><subject>Aquatic plants</subject><subject>Biodegradation</subject><subject>Biotopes</subject><subject>Catchments</subject><subject>Earth sciences</subject><subject>Earth, ocean, space</subject><subject>Engineering and environment geology. Geothermics</subject><subject>Exact sciences and technology</subject><subject>Forest watersheds</subject><subject>Fractionation</subject><subject>Freshwater</subject><subject>Geochemistry</subject><subject>Growing season</subject><subject>Hydrology</subject><subject>Hydrology. Hydrogeology</subject><subject>Lakes</subject><subject>Mineralogy</subject><subject>Molecular weight</subject><subject>Organic matter</subject><subject>Pollution, environment geology</subject><subject>Silicates</subject><subject>Surface water</subject><subject>Water geochemistry</subject><issn>1015-1621</issn><issn>1420-9055</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2004</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp90U1v1DAQBuAIgUQp_ABuFhJfh8BMHMfeY9XyJdrdC5ytiePsusrGxeOs1Ds_HK-2EhIHTrbs5x1ZfqvqJcIHBNAfGQAaXQO0NWiEGh5VZ9g2UK9AqcdlD6hq7Bp8Wj1jvgXAxmhzVv3-7u8Fh-zFgVKgfvIstvHg0xzmrcg7L8ZldjnEmSbhdpTIZZ8C5-BYxFFcBeY4Hfwg1pSXVNAmbWkOTtxQLlK8u1pvbt6LMIt1TEM5H2PynEvAUXa7vZ8zP6-ejDSxf_Gwnlc_P3_6cfm1vt58-XZ5cV2TNF2uEVpqh95JGlVnurHr-6H1EkD1sGrQSYOI5XoYUDr0RIMG8KBVJ_2gRi_Pq7enuXcp_lrKK-w-sPPTRLOPC1sDujFGoyryzX8l6uKkaQp89Q-8jUsqn8VWqxV2qpVHhCfkUmROfrR3Kewp3VsEe6zPnuqzpT57rM9Cybx-GEzsaBoTzS7w36AyerVCkH8AslWbWA</recordid><startdate>20040601</startdate><enddate>20040601</enddate><creator>VOGT, Rolf D</creator><creator>AKKANEN, Jarkko</creator><creator>PFLUGMACHER, Stephan</creator><creator>STARR, Mike</creator><creator>STEINBERG, Christian E. 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Hydrogeology</topic><topic>Lakes</topic><topic>Mineralogy</topic><topic>Molecular weight</topic><topic>Organic matter</topic><topic>Pollution, environment geology</topic><topic>Silicates</topic><topic>Surface water</topic><topic>Water geochemistry</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>VOGT, Rolf D</creatorcontrib><creatorcontrib>AKKANEN, Jarkko</creatorcontrib><creatorcontrib>PFLUGMACHER, Stephan</creatorcontrib><creatorcontrib>STARR, Mike</creatorcontrib><creatorcontrib>STEINBERG, Christian E. W</creatorcontrib><creatorcontrib>SCHMITT-KOPPLIN, Philippe</creatorcontrib><creatorcontrib>ZSOLNAY, Adam</creatorcontrib><creatorcontrib>ANDERSEN, Dag Olav</creatorcontrib><creatorcontrib>BRÜGGEMANN, Rainer</creatorcontrib><creatorcontrib>CHATTERJEE, Bimal</creatorcontrib><creatorcontrib>GJESSING, Egil</creatorcontrib><creatorcontrib>KUKKONEN, Jussi V. 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W</au><au>SCHMITT-KOPPLIN, Philippe</au><au>ZSOLNAY, Adam</au><au>ANDERSEN, Dag Olav</au><au>BRÜGGEMANN, Rainer</au><au>CHATTERJEE, Bimal</au><au>GJESSING, Egil</au><au>KUKKONEN, Jussi V. K</au><au>LARSEN, Hakon E</au><au>LUSTER, Jorg</au><au>PAUL, Andrea</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Key site variables governing the functional characteristics of Dissolved Natural Organic Matter (DNOM) in Nordic forested catchments</atitle><jtitle>Aquatic sciences</jtitle><date>2004-06-01</date><risdate>2004</risdate><volume>66</volume><issue>2</issue><spage>195</spage><epage>210</epage><pages>195-210</pages><issn>1015-1621</issn><eissn>1420-9055</eissn><abstract>The objective of this study was to extract and evaluate key catchment characteristics explaining the main variation in properties of dissolved natural organic matter (DNOM) in surface waters draining each catchment. A number of classical and sophisticated DNOM characterisation methodologies were used for this purpose. The explanatory capability of site characteristics on the variation in descriptors of DNOM, including elemental analysis (EA), DOC fractionation, SEC, CZE, CGE, UV/Vis- and FTIR spectra, FES, TLS, ESR, ESI/MS, super(13)C-CPMAS-NMR, potentiometric pH titration as well as functional characteristics such as biodegradability, and the response of macrophyte and PAH partitioning coefficients were evaluated. The sampling sites were all natural, coniferous, heathery-forested catchments with bogs, forming a climatic, anthropogenic deposition and proportional biotope cover gradient. Correlations to the main principal components, as well as a correlation matrix, singled out total S-deposition as the key explanatory site parameter, accounting for most of the variation in DNOM descriptors. Other significant factors were H super(+) concentration, length of growing season, biotope coverage (i.e., peatland/ or lake/watershed ratio), site elevation and TOC concentration. Total sulphur (S) deposition was strongly negatively correlated to the molecular weight, aromaticity, carboxylic acidity and sorption capacity of PAH. A greater proportion of lake and Histosol biotopes of the sampling sites were reflected in a greater aliphatic character of the DNOM. PCA clustering of samples from the same site in spring and fall showed a basic site-specific DNOM quality and a weak season effect. The Hasse diagram technique (a method of partial order theory) was used to show, for instance, how the relative Histosol coverage may determine NOM quality and, in turn, how this coincides with high macrophyte response.</abstract><cop>Heidelberg</cop><pub>Springer</pub><doi>10.1007/s00027-004-0710-0</doi><tpages>16</tpages></addata></record> |
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| ispartof | Aquatic sciences, 2004-06, Vol.66 (2), p.195-210 |
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| subjects | Acidity Anthropogenic factors Aquatic plants Biodegradation Biotopes Catchments Earth sciences Earth, ocean, space Engineering and environment geology. Geothermics Exact sciences and technology Forest watersheds Fractionation Freshwater Geochemistry Growing season Hydrology Hydrology. Hydrogeology Lakes Mineralogy Molecular weight Organic matter Pollution, environment geology Silicates Surface water Water geochemistry |
| title | Key site variables governing the functional characteristics of Dissolved Natural Organic Matter (DNOM) in Nordic forested catchments |
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