Effects of beam polarization on coherent anti-Stokes Raman scattering using noisy light
The effects of different linear polarization schemes on the noisy light‐based coherent anti‐Stokes Raman scattering [I(2)CARS] signal were investigated. It was found that certain polarization schemes can selectively shut down the contributions from terms represented by various factorized time correl...
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| Veröffentlicht in: | Journal of Raman spectroscopy 2005-05, Vol.36 (5), p.409-419 |
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| container_title | Journal of Raman spectroscopy |
| container_volume | 36 |
| creator | Aung, Pye Phyo Cosert, Krista M. Weisel, Lindsay R. Schulz, Tanner F. Gealy, M. W. Ulness, Darin J. |
| description | The effects of different linear polarization schemes on the noisy light‐based coherent anti‐Stokes Raman scattering [I(2)CARS] signal were investigated. It was found that certain polarization schemes can selectively shut down the contributions from terms represented by various factorized time correlation (FTC) diagrams to the I(2)CARS spectrogram. FTC diagram analysis was used in conjunction with the symmetry properties of the hyperpolarizability to provide a theoretical understanding of this phenomenon and serve as the basis for simulation of the I(2)CARS spectrogram. Striking agreement is seen between the simulations and the experimental results for benzene and several methylated benzene derivatives. Copyright © 2005 John Wiley & Sons, Ltd. |
| doi_str_mv | 10.1002/jrs.1311 |
| format | Article |
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W.</creatorcontrib><creatorcontrib>Ulness, Darin J.</creatorcontrib><title>Effects of beam polarization on coherent anti-Stokes Raman scattering using noisy light</title><title>Journal of Raman spectroscopy</title><addtitle>J. Raman Spectrosc</addtitle><description>The effects of different linear polarization schemes on the noisy light‐based coherent anti‐Stokes Raman scattering [I(2)CARS] signal were investigated. It was found that certain polarization schemes can selectively shut down the contributions from terms represented by various factorized time correlation (FTC) diagrams to the I(2)CARS spectrogram. FTC diagram analysis was used in conjunction with the symmetry properties of the hyperpolarizability to provide a theoretical understanding of this phenomenon and serve as the basis for simulation of the I(2)CARS spectrogram. Striking agreement is seen between the simulations and the experimental results for benzene and several methylated benzene derivatives. Copyright © 2005 John Wiley & Sons, Ltd.</description><subject>Benzene</subject><subject>coherent anti-Stokes Raman scattering</subject><subject>Coherent scattering</subject><subject>Derivatives</subject><subject>Linear polarization</subject><subject>noisy light spectroscopy</subject><subject>Polarization</subject><subject>Raman scattering</subject><subject>Simulation</subject><subject>Spectrograms</subject><issn>0377-0486</issn><issn>1097-4555</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2005</creationdate><recordtype>article</recordtype><recordid>eNp10E1LAzEQBuAgCtYP8CfkppfVpNndbI5S_KQq-HkM02Si0e2mJilaf71bKoIHYZi5PLwDLyF7nB1yxoZHrzEdcsH5GhlwpmRRVlW1TgZMSFmwsqk3yVZKr4wxpWo-IE8nzqHJiQZHJwhTOgstRP8F2YeO9mPCC0bsMoUu--IuhzdM9Bam0NFkIGeMvnum87TcXfBpQVv__JJ3yIaDNuHuz90mD6cn96PzYnxzdjE6HhdGiIoXjoEDMbHOcuGMsjXUxmEjXalMUwNiY4fMKGHtpBwitwxKW0lp7VApXsFEbJP9Ve4shvc5pqynPhlsW-gwzJOWjWSK8Vr28mAlTQwpRXR6Fv0U4kJzppfV6b46vayup8WKfvgWF_86fXl799f7lPHz10N80_1jWemn6zM94o9XbFxeaim-AYWwgOk</recordid><startdate>200505</startdate><enddate>200505</enddate><creator>Aung, Pye Phyo</creator><creator>Cosert, Krista M.</creator><creator>Weisel, Lindsay R.</creator><creator>Schulz, Tanner F.</creator><creator>Gealy, M. 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FTC diagram analysis was used in conjunction with the symmetry properties of the hyperpolarizability to provide a theoretical understanding of this phenomenon and serve as the basis for simulation of the I(2)CARS spectrogram. Striking agreement is seen between the simulations and the experimental results for benzene and several methylated benzene derivatives. Copyright © 2005 John Wiley & Sons, Ltd.</abstract><cop>Chichester, UK</cop><pub>John Wiley & Sons, Ltd</pub><doi>10.1002/jrs.1311</doi><tpages>11</tpages></addata></record> |
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| source | Wiley Online Library Journals Frontfile Complete |
| subjects | Benzene coherent anti-Stokes Raman scattering Coherent scattering Derivatives Linear polarization noisy light spectroscopy Polarization Raman scattering Simulation Spectrograms |
| title | Effects of beam polarization on coherent anti-Stokes Raman scattering using noisy light |
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