Spherical Bilayer Vesicles of Fullerene-Based Surfactants in Water: A Laser Light Scattering Study
The low solubility of fullerenes in aqueous solution limits their applications in biology. By appropriate substitution, the fullerenes can be transformed into stabilized anions that are water soluble and can form large aggregated structures. A laser light scattering study of the association behavior...
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| Veröffentlicht in: | Science (American Association for the Advancement of Science) 2001-03, Vol.291 (5510), p.1944-1947 |
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| container_issue | 5510 |
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| container_title | Science (American Association for the Advancement of Science) |
| container_volume | 291 |
| creator | Zhou, Shuiqin Burger, Christian Chu, Benjamin Sawamura, Masaya Nagahama, Noriaki Toganoh, Motoki Hackler, Ulrich E. Isobe, Hiroyuki Nakamura, Eiichi |
| description | The low solubility of fullerenes in aqueous solution limits their applications in biology. By appropriate substitution, the fullerenes can be transformed into stabilized anions that are water soluble and can form large aggregated structures. A laser light scattering study of the association behavior of the potassium salt of pentaphenyl fullerene (Ph5C
60K) in water revealed that the hydrocarbon anions Ph5C
60
-associate into bilayers, forming stable spherical vesicles with an average hydrodynamic radius and a radius of gyration of about 17 nanometers at a very low critical aggregation concentration of less than 10-7moles per liter. The average aggregation number of associated particles in these large spherical vesicles is about 1.2 × 104. |
| doi_str_mv | 10.1126/science.291.5510.1944 |
| format | Article |
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60K) in water revealed that the hydrocarbon anions Ph5C
60
-associate into bilayers, forming stable spherical vesicles with an average hydrodynamic radius and a radius of gyration of about 17 nanometers at a very low critical aggregation concentration of less than 10-7moles per liter. The average aggregation number of associated particles in these large spherical vesicles is about 1.2 × 104.</description><identifier>ISSN: 0036-8075</identifier><identifier>EISSN: 1095-9203</identifier><identifier>DOI: 10.1126/science.291.5510.1944</identifier><identifier>PMID: 11239150</identifier><identifier>CODEN: SCIEAS</identifier><language>eng</language><publisher>Washington, DC: American Society for the Advancement of Science</publisher><subject>Anions ; Chemistry ; Colloidal state and disperse state ; Electrostatics ; Evaporation ; Exact sciences and technology ; Fullerenes ; General and physical chemistry ; Hydrodynamics ; Lasers ; Light scattering ; Membranes ; Molecules ; Oxides ; Potassium ; Potassium salts ; Radius of a sphere ; Rotation ; Salt ; Water</subject><ispartof>Science (American Association for the Advancement of Science), 2001-03, Vol.291 (5510), p.1944-1947</ispartof><rights>Copyright 2001 American Association for the Advancement of Science</rights><rights>2001 INIST-CNRS</rights><rights>COPYRIGHT 2001 American Association for the Advancement of Science</rights><rights>Copyright American Association for the Advancement of Science Mar 9, 2001</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c781t-1895ffe8558d16a9578a6325911c424513e52514885151f51ec15f2245d4f7323</citedby><cites>FETCH-LOGICAL-c781t-1895ffe8558d16a9578a6325911c424513e52514885151f51ec15f2245d4f7323</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.jstor.org/stable/pdf/3082447$$EPDF$$P50$$Gjstor$$H</linktopdf><linktohtml>$$Uhttps://www.jstor.org/stable/3082447$$EHTML$$P50$$Gjstor$$H</linktohtml><link.rule.ids>314,776,780,799,2870,2871,27903,27904,57995,58228</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=997154$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/11239150$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Zhou, Shuiqin</creatorcontrib><creatorcontrib>Burger, Christian</creatorcontrib><creatorcontrib>Chu, Benjamin</creatorcontrib><creatorcontrib>Sawamura, Masaya</creatorcontrib><creatorcontrib>Nagahama, Noriaki</creatorcontrib><creatorcontrib>Toganoh, Motoki</creatorcontrib><creatorcontrib>Hackler, Ulrich E.</creatorcontrib><creatorcontrib>Isobe, Hiroyuki</creatorcontrib><creatorcontrib>Nakamura, Eiichi</creatorcontrib><title>Spherical Bilayer Vesicles of Fullerene-Based Surfactants in Water: A Laser Light Scattering Study</title><title>Science (American Association for the Advancement of Science)</title><addtitle>Science</addtitle><description>The low solubility of fullerenes in aqueous solution limits their applications in biology. By appropriate substitution, the fullerenes can be transformed into stabilized anions that are water soluble and can form large aggregated structures. A laser light scattering study of the association behavior of the potassium salt of pentaphenyl fullerene (Ph5C
60K) in water revealed that the hydrocarbon anions Ph5C
60
-associate into bilayers, forming stable spherical vesicles with an average hydrodynamic radius and a radius of gyration of about 17 nanometers at a very low critical aggregation concentration of less than 10-7moles per liter. 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solution limits their applications in biology. By appropriate substitution, the fullerenes can be transformed into stabilized anions that are water soluble and can form large aggregated structures. A laser light scattering study of the association behavior of the potassium salt of pentaphenyl fullerene (Ph5C
60K) in water revealed that the hydrocarbon anions Ph5C
60
-associate into bilayers, forming stable spherical vesicles with an average hydrodynamic radius and a radius of gyration of about 17 nanometers at a very low critical aggregation concentration of less than 10-7moles per liter. The average aggregation number of associated particles in these large spherical vesicles is about 1.2 × 104.</abstract><cop>Washington, DC</cop><pub>American Society for the Advancement of Science</pub><pmid>11239150</pmid><doi>10.1126/science.291.5510.1944</doi><tpages>4</tpages></addata></record> |
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| recordid | cdi_proquest_miscellaneous_76960615 |
| source | American Association for the Advancement of Science; Jstor Complete Legacy |
| subjects | Anions Chemistry Colloidal state and disperse state Electrostatics Evaporation Exact sciences and technology Fullerenes General and physical chemistry Hydrodynamics Lasers Light scattering Membranes Molecules Oxides Potassium Potassium salts Radius of a sphere Rotation Salt Water |
| title | Spherical Bilayer Vesicles of Fullerene-Based Surfactants in Water: A Laser Light Scattering Study |
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