Dynamic modelling of atmospherically-deposited Ni, Cu, Zn, Cd and Pb in Pennine catchments (northern England)
Simulation modelling with CHUM-AM was carried out to investigate the accumulation and release of atmospherically-deposited heavy metals (Ni, Cu, Zn, Cd and Pb) in six moorland catchments, five with organic-rich soils, one with calcareous brown earths, in the Pennine chain of northern England. The mo...
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| Veröffentlicht in: | Environmental pollution (1987) 2010-05, Vol.158 (5), p.1521-1529 |
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| container_title | Environmental pollution (1987) |
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| creator | Tipping, E. Rothwell, J.J. Shotbolt, L. Lawlor, A.J. |
| description | Simulation modelling with CHUM-AM was carried out to investigate the accumulation and release of atmospherically-deposited heavy metals (Ni, Cu, Zn, Cd and Pb) in six moorland catchments, five with organic-rich soils, one with calcareous brown earths, in the Pennine chain of northern England. The model considers two soil layers and a third layer of weathering mineral matter, and operates on a yearly timestep, driven by deposition scenarios covering the period 1400–2010. The principal processes controlling heavy metals are competitive solid–solution partitioning of solutes, chemical interactions in solution, and chemical weathering. Agreement between observed and simulated soil metal pools and surface water concentrations for recent years was generally satisfactory, the results confirming that most contemporary soil metal is from atmospheric pollution. Metals in catchments with organic-rich soils show some mobility, especially under more acid conditions, but the calcareous mineral soils have retained nearly all anthropogenic metal inputs. Complexation by dissolved organic matter and co-transport accounts for up to 80% of the Cu in surface waters.
CHUM-AM is applied to six differing moorland catchments to account for the accumulation and leaching of atmospherically-deposited trace metals over the past several centuries. |
| doi_str_mv | 10.1016/j.envpol.2009.12.026 |
| format | Article |
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CHUM-AM is applied to six differing moorland catchments to account for the accumulation and leaching of atmospherically-deposited trace metals over the past several centuries.</description><identifier>ISSN: 0269-7491</identifier><identifier>EISSN: 1873-6424</identifier><identifier>DOI: 10.1016/j.envpol.2009.12.026</identifier><identifier>PMID: 20045236</identifier><identifier>CODEN: ENVPAF</identifier><language>eng</language><publisher>Kidlington: Elsevier Ltd</publisher><subject>Air Pollutants - analysis ; Applied sciences ; Atmospheric deposition ; Cadmium ; Catchment ; Catchments ; chemical interactions ; Computer simulation ; Continental surface waters ; Copper ; dissolved organic matter ; dynamic models ; Earth sciences ; Earth, ocean, space ; Engineering and environment geology. Geothermics ; England ; Environmental Pollution ; Exact sciences and technology ; Geologic Sediments - analysis ; heathlands ; Heavy metals ; lead ; Lead (metal) ; Metals, Heavy - analysis ; mineral soils ; Modelling ; Models, Theoretical ; Natural water pollution ; Nickel ; Pollution ; Pollution, environment geology ; simulation models ; Soil organic matter ; Soil Pollutants - analysis ; Soils ; solutes ; Surface water ; Water treatment and pollution ; watersheds ; Weathering ; zinc</subject><ispartof>Environmental pollution (1987), 2010-05, Vol.158 (5), p.1521-1529</ispartof><rights>2010 Elsevier Ltd</rights><rights>2015 INIST-CNRS</rights><rights>Copyright 2010 Elsevier Ltd. All rights reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a503t-7001a6b43afb4390bb50cebdf274bc419c531d1c588f980896dbf1f665c3b8e03</citedby><cites>FETCH-LOGICAL-a503t-7001a6b43afb4390bb50cebdf274bc419c531d1c588f980896dbf1f665c3b8e03</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.envpol.2009.12.026$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,777,781,3537,27905,27906,45976</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=22681333$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/20045236$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Tipping, E.</creatorcontrib><creatorcontrib>Rothwell, J.J.</creatorcontrib><creatorcontrib>Shotbolt, L.</creatorcontrib><creatorcontrib>Lawlor, A.J.</creatorcontrib><title>Dynamic modelling of atmospherically-deposited Ni, Cu, Zn, Cd and Pb in Pennine catchments (northern England)</title><title>Environmental pollution (1987)</title><addtitle>Environ Pollut</addtitle><description>Simulation modelling with CHUM-AM was carried out to investigate the accumulation and release of atmospherically-deposited heavy metals (Ni, Cu, Zn, Cd and Pb) in six moorland catchments, five with organic-rich soils, one with calcareous brown earths, in the Pennine chain of northern England. The model considers two soil layers and a third layer of weathering mineral matter, and operates on a yearly timestep, driven by deposition scenarios covering the period 1400–2010. The principal processes controlling heavy metals are competitive solid–solution partitioning of solutes, chemical interactions in solution, and chemical weathering. Agreement between observed and simulated soil metal pools and surface water concentrations for recent years was generally satisfactory, the results confirming that most contemporary soil metal is from atmospheric pollution. Metals in catchments with organic-rich soils show some mobility, especially under more acid conditions, but the calcareous mineral soils have retained nearly all anthropogenic metal inputs. Complexation by dissolved organic matter and co-transport accounts for up to 80% of the Cu in surface waters.
CHUM-AM is applied to six differing moorland catchments to account for the accumulation and leaching of atmospherically-deposited trace metals over the past several centuries.</description><subject>Air Pollutants - analysis</subject><subject>Applied sciences</subject><subject>Atmospheric deposition</subject><subject>Cadmium</subject><subject>Catchment</subject><subject>Catchments</subject><subject>chemical interactions</subject><subject>Computer simulation</subject><subject>Continental surface waters</subject><subject>Copper</subject><subject>dissolved organic matter</subject><subject>dynamic models</subject><subject>Earth sciences</subject><subject>Earth, ocean, space</subject><subject>Engineering and environment geology. Geothermics</subject><subject>England</subject><subject>Environmental Pollution</subject><subject>Exact sciences and technology</subject><subject>Geologic Sediments - analysis</subject><subject>heathlands</subject><subject>Heavy metals</subject><subject>lead</subject><subject>Lead (metal)</subject><subject>Metals, Heavy - analysis</subject><subject>mineral soils</subject><subject>Modelling</subject><subject>Models, Theoretical</subject><subject>Natural water pollution</subject><subject>Nickel</subject><subject>Pollution</subject><subject>Pollution, environment geology</subject><subject>simulation models</subject><subject>Soil organic matter</subject><subject>Soil Pollutants - analysis</subject><subject>Soils</subject><subject>solutes</subject><subject>Surface water</subject><subject>Water treatment and pollution</subject><subject>watersheds</subject><subject>Weathering</subject><subject>zinc</subject><issn>0269-7491</issn><issn>1873-6424</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2010</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqN0V1rFDEUBuAgil2r_0A0N2KFzpozySSZG0HW-gFFC9obb0ImyWyzzCRjMlvYf2_KrHpXvMmB8JyTjxeh50DWQIC_3a1duJ3isK4JaddQr0nNH6AVSEErzmr2EK3KTlsJ1sIJepLzjhDCKKWP0UlpYU1N-QqNHw5Bj97gMVo3DD5sceyxnseYpxuXvNHDcKism2L2s7P4qz_Hm_05_hlKtVgHi6867AO-ciH44LDRs7kZXZgzPgsxzWVIwBdhOxT65il61Oshu2fHeoquP1782HyuLr99-rJ5f1nphtC5EoSA5h2jui9LS7quIcZ1tq8F6wyD1jQULJhGyr6VRLbcdj30nDeGdtIReopeL3OnFH_tXZ7V6LMp79PBxX1WgnFgshb_ISmVDCTIIs_ulSCEgEYQBoWyhZoUc06uV1Pyo04HBUTdhad2aglP3YWnoFYlqtL24njCvhud_dv0J60CXh2BziWYPulgfP7nai6hBFzcy8X1Oiq9TcVcf68JsPKvgnDRFPFuEa6kcOtdUtl4F4yzPjkzKxv9_Xf9DTPfwVk</recordid><startdate>20100501</startdate><enddate>20100501</enddate><creator>Tipping, E.</creator><creator>Rothwell, J.J.</creator><creator>Shotbolt, L.</creator><creator>Lawlor, A.J.</creator><general>Elsevier Ltd</general><general>Elsevier Science Ltd</general><general>Elsevier</general><scope>FBQ</scope><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SU</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>KR7</scope><scope>7X8</scope><scope>7ST</scope><scope>7TG</scope><scope>7TV</scope><scope>7U7</scope><scope>KL.</scope><scope>SOI</scope></search><sort><creationdate>20100501</creationdate><title>Dynamic modelling of atmospherically-deposited Ni, Cu, Zn, Cd and Pb in Pennine catchments (northern England)</title><author>Tipping, E. ; Rothwell, J.J. ; Shotbolt, L. ; Lawlor, A.J.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a503t-7001a6b43afb4390bb50cebdf274bc419c531d1c588f980896dbf1f665c3b8e03</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2010</creationdate><topic>Air Pollutants - analysis</topic><topic>Applied sciences</topic><topic>Atmospheric deposition</topic><topic>Cadmium</topic><topic>Catchment</topic><topic>Catchments</topic><topic>chemical interactions</topic><topic>Computer simulation</topic><topic>Continental surface waters</topic><topic>Copper</topic><topic>dissolved organic matter</topic><topic>dynamic models</topic><topic>Earth sciences</topic><topic>Earth, ocean, space</topic><topic>Engineering and environment geology. Geothermics</topic><topic>England</topic><topic>Environmental Pollution</topic><topic>Exact sciences and technology</topic><topic>Geologic Sediments - analysis</topic><topic>heathlands</topic><topic>Heavy metals</topic><topic>lead</topic><topic>Lead (metal)</topic><topic>Metals, Heavy - analysis</topic><topic>mineral soils</topic><topic>Modelling</topic><topic>Models, Theoretical</topic><topic>Natural water pollution</topic><topic>Nickel</topic><topic>Pollution</topic><topic>Pollution, environment geology</topic><topic>simulation models</topic><topic>Soil organic matter</topic><topic>Soil Pollutants - analysis</topic><topic>Soils</topic><topic>solutes</topic><topic>Surface water</topic><topic>Water treatment and pollution</topic><topic>watersheds</topic><topic>Weathering</topic><topic>zinc</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Tipping, E.</creatorcontrib><creatorcontrib>Rothwell, J.J.</creatorcontrib><creatorcontrib>Shotbolt, L.</creatorcontrib><creatorcontrib>Lawlor, A.J.</creatorcontrib><collection>AGRIS</collection><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Environmental Engineering Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>Civil Engineering Abstracts</collection><collection>MEDLINE - Academic</collection><collection>Environment Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Environment Abstracts</collection><jtitle>Environmental pollution (1987)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Tipping, E.</au><au>Rothwell, J.J.</au><au>Shotbolt, L.</au><au>Lawlor, A.J.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Dynamic modelling of atmospherically-deposited Ni, Cu, Zn, Cd and Pb in Pennine catchments (northern England)</atitle><jtitle>Environmental pollution (1987)</jtitle><addtitle>Environ Pollut</addtitle><date>2010-05-01</date><risdate>2010</risdate><volume>158</volume><issue>5</issue><spage>1521</spage><epage>1529</epage><pages>1521-1529</pages><issn>0269-7491</issn><eissn>1873-6424</eissn><coden>ENVPAF</coden><abstract>Simulation modelling with CHUM-AM was carried out to investigate the accumulation and release of atmospherically-deposited heavy metals (Ni, Cu, Zn, Cd and Pb) in six moorland catchments, five with organic-rich soils, one with calcareous brown earths, in the Pennine chain of northern England. The model considers two soil layers and a third layer of weathering mineral matter, and operates on a yearly timestep, driven by deposition scenarios covering the period 1400–2010. The principal processes controlling heavy metals are competitive solid–solution partitioning of solutes, chemical interactions in solution, and chemical weathering. Agreement between observed and simulated soil metal pools and surface water concentrations for recent years was generally satisfactory, the results confirming that most contemporary soil metal is from atmospheric pollution. Metals in catchments with organic-rich soils show some mobility, especially under more acid conditions, but the calcareous mineral soils have retained nearly all anthropogenic metal inputs. Complexation by dissolved organic matter and co-transport accounts for up to 80% of the Cu in surface waters.
CHUM-AM is applied to six differing moorland catchments to account for the accumulation and leaching of atmospherically-deposited trace metals over the past several centuries.</abstract><cop>Kidlington</cop><pub>Elsevier Ltd</pub><pmid>20045236</pmid><doi>10.1016/j.envpol.2009.12.026</doi><tpages>9</tpages></addata></record> |
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| ispartof | Environmental pollution (1987), 2010-05, Vol.158 (5), p.1521-1529 |
| issn | 0269-7491 1873-6424 |
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| source | MEDLINE; Elsevier ScienceDirect Journals |
| subjects | Air Pollutants - analysis Applied sciences Atmospheric deposition Cadmium Catchment Catchments chemical interactions Computer simulation Continental surface waters Copper dissolved organic matter dynamic models Earth sciences Earth, ocean, space Engineering and environment geology. Geothermics England Environmental Pollution Exact sciences and technology Geologic Sediments - analysis heathlands Heavy metals lead Lead (metal) Metals, Heavy - analysis mineral soils Modelling Models, Theoretical Natural water pollution Nickel Pollution Pollution, environment geology simulation models Soil organic matter Soil Pollutants - analysis Soils solutes Surface water Water treatment and pollution watersheds Weathering zinc |
| title | Dynamic modelling of atmospherically-deposited Ni, Cu, Zn, Cd and Pb in Pennine catchments (northern England) |
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