Short-term temporal variations in speciation of Pb, Cu, Zn and Sb in a shooting range runoff stream
This study was designed to explore the changes in physico-chemical forms of Pb, Cu, Zn and Sb in a stream draining a contaminated shooting range, located at Steinsjøen in the South-Eastern part of Norway, during a period of 21 days. To obtain information on the element species distribution, an inter...
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| Veröffentlicht in: | The Science of the total environment 2010-05, Vol.408 (11), p.2409-2417 |
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| creator | Heier, Lene Sørlie Meland, Sondre Ljønes, Marita Salbu, Brit Strømseng, Arnljot Einride |
| description | This study was designed to explore the changes in physico-chemical forms of Pb, Cu, Zn and Sb in a stream draining a contaminated shooting range, located at Steinsjøen in the South-Eastern part of Norway, during a period of 21
days. To obtain information on the element species distribution, an interphased size and charge fractionation system was applied, where membrane filtration (0.45
µm) and ultrafiltration using hollow fibre (nominal cut off 10
kDa) were performed prior to charge fractionation using chromatography (cationic and anionic exchange resins). The results show that Pb mainly was present as particulate and colloidal high molecular mass (HMM) species, Cu as colloidal (HMM) and low molecular mass (LMM) species, while Sb and Zn were mainly present as LMM species. The total element concentrations of Pb, Cu, Zn and Sb were positively correlated to water flow and dissolved organic carbon (DOC), suggesting these are important factors in controlling the run-off of the investigated elements in this catchment. During episodes of higher water flow, the increase in element concentration was mainly in the colloidal fraction. Partial redundancy analysis (pRDA) revealed that variations in pH, HMM organic carbon (HMM OC) and LMM organic carbon (LMM OC) explained 47% of the variation in size distribution of the elements, while variations in precipitation and water flow explained 48% of the variation in the charge distribution of the elements. The variation in concentrations during the period varied by a factor of 4, also stressing the importance of frequent sampling opposed to spot sampling in environmental surveys and risk assessments. |
| doi_str_mv | 10.1016/j.scitotenv.2010.02.019 |
| format | Article |
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days. To obtain information on the element species distribution, an interphased size and charge fractionation system was applied, where membrane filtration (0.45
µm) and ultrafiltration using hollow fibre (nominal cut off 10
kDa) were performed prior to charge fractionation using chromatography (cationic and anionic exchange resins). The results show that Pb mainly was present as particulate and colloidal high molecular mass (HMM) species, Cu as colloidal (HMM) and low molecular mass (LMM) species, while Sb and Zn were mainly present as LMM species. The total element concentrations of Pb, Cu, Zn and Sb were positively correlated to water flow and dissolved organic carbon (DOC), suggesting these are important factors in controlling the run-off of the investigated elements in this catchment. During episodes of higher water flow, the increase in element concentration was mainly in the colloidal fraction. Partial redundancy analysis (pRDA) revealed that variations in pH, HMM organic carbon (HMM OC) and LMM organic carbon (LMM OC) explained 47% of the variation in size distribution of the elements, while variations in precipitation and water flow explained 48% of the variation in the charge distribution of the elements. The variation in concentrations during the period varied by a factor of 4, also stressing the importance of frequent sampling opposed to spot sampling in environmental surveys and risk assessments.</description><identifier>ISSN: 0048-9697</identifier><identifier>EISSN: 1879-1026</identifier><identifier>DOI: 10.1016/j.scitotenv.2010.02.019</identifier><identifier>PMID: 20206376</identifier><identifier>CODEN: STENDL</identifier><language>eng</language><publisher>Kidlington: Elsevier B.V</publisher><subject>Antimony ; Antimony - analysis ; Antimony - chemistry ; Applied sciences ; Carbon ; Chromatography, Ion Exchange ; Colloids ; Continental surface waters ; Copper ; Copper - analysis ; Copper - chemistry ; Earth sciences ; Earth, ocean, space ; Engineering and environment geology. Geothermics ; Environmental Monitoring ; Exact sciences and technology ; Firearms ; Fresh Water - chemistry ; Ion Exchange Resins ; Lead (metal) ; Lead - analysis ; Lead - chemistry ; Mathematical models ; Metal speciation ; Metals, Heavy - analysis ; Metals, Heavy - chemistry ; Natural water pollution ; Norway ; Pollution ; Pollution, environment geology ; Rainwaters, run off water and others ; Redundancy analysis (RDA) ; Soil Pollutants - analysis ; Soil Pollutants - chemistry ; Temporal variations ; Time Factors ; Water flow ; Water Movements ; Water Pollutants, Chemical - chemistry ; Water treatment and pollution ; Zinc ; Zinc - analysis ; Zinc - chemistry</subject><ispartof>The Science of the total environment, 2010-05, Vol.408 (11), p.2409-2417</ispartof><rights>2010 Elsevier B.V.</rights><rights>2015 INIST-CNRS</rights><rights>Copyright 2010 Elsevier B.V. All rights reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c465t-d734061a9c6a31bb193fa534d5a4a0041bc21d26865a15ef40beb9a2e3eec88c3</citedby><cites>FETCH-LOGICAL-c465t-d734061a9c6a31bb193fa534d5a4a0041bc21d26865a15ef40beb9a2e3eec88c3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0048969710001300$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3537,27901,27902,65306</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=22611017$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/20206376$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Heier, Lene Sørlie</creatorcontrib><creatorcontrib>Meland, Sondre</creatorcontrib><creatorcontrib>Ljønes, Marita</creatorcontrib><creatorcontrib>Salbu, Brit</creatorcontrib><creatorcontrib>Strømseng, Arnljot Einride</creatorcontrib><title>Short-term temporal variations in speciation of Pb, Cu, Zn and Sb in a shooting range runoff stream</title><title>The Science of the total environment</title><addtitle>Sci Total Environ</addtitle><description>This study was designed to explore the changes in physico-chemical forms of Pb, Cu, Zn and Sb in a stream draining a contaminated shooting range, located at Steinsjøen in the South-Eastern part of Norway, during a period of 21
days. To obtain information on the element species distribution, an interphased size and charge fractionation system was applied, where membrane filtration (0.45
µm) and ultrafiltration using hollow fibre (nominal cut off 10
kDa) were performed prior to charge fractionation using chromatography (cationic and anionic exchange resins). The results show that Pb mainly was present as particulate and colloidal high molecular mass (HMM) species, Cu as colloidal (HMM) and low molecular mass (LMM) species, while Sb and Zn were mainly present as LMM species. The total element concentrations of Pb, Cu, Zn and Sb were positively correlated to water flow and dissolved organic carbon (DOC), suggesting these are important factors in controlling the run-off of the investigated elements in this catchment. During episodes of higher water flow, the increase in element concentration was mainly in the colloidal fraction. Partial redundancy analysis (pRDA) revealed that variations in pH, HMM organic carbon (HMM OC) and LMM organic carbon (LMM OC) explained 47% of the variation in size distribution of the elements, while variations in precipitation and water flow explained 48% of the variation in the charge distribution of the elements. The variation in concentrations during the period varied by a factor of 4, also stressing the importance of frequent sampling opposed to spot sampling in environmental surveys and risk assessments.</description><subject>Antimony</subject><subject>Antimony - analysis</subject><subject>Antimony - chemistry</subject><subject>Applied sciences</subject><subject>Carbon</subject><subject>Chromatography, Ion Exchange</subject><subject>Colloids</subject><subject>Continental surface waters</subject><subject>Copper</subject><subject>Copper - analysis</subject><subject>Copper - chemistry</subject><subject>Earth sciences</subject><subject>Earth, ocean, space</subject><subject>Engineering and environment geology. Geothermics</subject><subject>Environmental Monitoring</subject><subject>Exact sciences and technology</subject><subject>Firearms</subject><subject>Fresh Water - chemistry</subject><subject>Ion Exchange Resins</subject><subject>Lead (metal)</subject><subject>Lead - analysis</subject><subject>Lead - chemistry</subject><subject>Mathematical models</subject><subject>Metal speciation</subject><subject>Metals, Heavy - analysis</subject><subject>Metals, Heavy - chemistry</subject><subject>Natural water pollution</subject><subject>Norway</subject><subject>Pollution</subject><subject>Pollution, environment geology</subject><subject>Rainwaters, run off water and others</subject><subject>Redundancy analysis (RDA)</subject><subject>Soil Pollutants - analysis</subject><subject>Soil Pollutants - chemistry</subject><subject>Temporal variations</subject><subject>Time Factors</subject><subject>Water flow</subject><subject>Water Movements</subject><subject>Water Pollutants, Chemical - chemistry</subject><subject>Water treatment and pollution</subject><subject>Zinc</subject><subject>Zinc - analysis</subject><subject>Zinc - chemistry</subject><issn>0048-9697</issn><issn>1879-1026</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2010</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqFkU1v1DAQhi0EotvCXwBfUHtoFn8kdnKsVnxJlUAqXLhYE2fSepXYi-2sxL_Hq13KjfoysvXMvH7nJeQtZ2vOuHq_XSfrcsjo92vByisTa8a7Z2TFW91VnAn1nKwYq9uqU50-I-cpbVk5uuUvyZlggimp1YrYu4cQc5UxzjTjvAsRJrqH6CC74BN1nqYd2uOVhpF-66_pZrmmPz0FP9C7_oAATQ8hZOfvaQR_jzQuPowjTTkizK_IixGmhK9P9YL8-Pjh--Zzdfv105fNzW1la9XkatCyZopDZxVI3ve8kyM0sh4aqKFY4b0VfBCqVQ3wBsea9dh3IFAi2ra18oJcHufuYvi1YMpmdsniNIHHsCSja8WK8eL8SVJK0bVSt4W8-i_JtWaS13XbFFQfURtDShFHs4tuhvjbcGYOqZmteUzNHFIzTJiSWul8cxJZ-hmHx76_MRXg3QmAZGEay5KtS_84oXgR0IW7OXJY1rx3GA-C6C0OLqLNZgjuyc_8AelJuQo</recordid><startdate>20100501</startdate><enddate>20100501</enddate><creator>Heier, Lene Sørlie</creator><creator>Meland, Sondre</creator><creator>Ljønes, Marita</creator><creator>Salbu, Brit</creator><creator>Strømseng, Arnljot Einride</creator><general>Elsevier B.V</general><general>Elsevier</general><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SU</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>KR7</scope><scope>7X8</scope><scope>7QH</scope><scope>7ST</scope><scope>7TV</scope><scope>7U1</scope><scope>7U2</scope><scope>7U6</scope><scope>7UA</scope><scope>F1W</scope><scope>H96</scope><scope>L.G</scope><scope>SOI</scope></search><sort><creationdate>20100501</creationdate><title>Short-term temporal variations in speciation of Pb, Cu, Zn and Sb in a shooting range runoff stream</title><author>Heier, Lene Sørlie ; Meland, Sondre ; Ljønes, Marita ; Salbu, Brit ; Strømseng, Arnljot Einride</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c465t-d734061a9c6a31bb193fa534d5a4a0041bc21d26865a15ef40beb9a2e3eec88c3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2010</creationdate><topic>Antimony</topic><topic>Antimony - analysis</topic><topic>Antimony - chemistry</topic><topic>Applied sciences</topic><topic>Carbon</topic><topic>Chromatography, Ion Exchange</topic><topic>Colloids</topic><topic>Continental surface waters</topic><topic>Copper</topic><topic>Copper - analysis</topic><topic>Copper - chemistry</topic><topic>Earth sciences</topic><topic>Earth, ocean, space</topic><topic>Engineering and environment geology. Geothermics</topic><topic>Environmental Monitoring</topic><topic>Exact sciences and technology</topic><topic>Firearms</topic><topic>Fresh Water - chemistry</topic><topic>Ion Exchange Resins</topic><topic>Lead (metal)</topic><topic>Lead - analysis</topic><topic>Lead - chemistry</topic><topic>Mathematical models</topic><topic>Metal speciation</topic><topic>Metals, Heavy - analysis</topic><topic>Metals, Heavy - chemistry</topic><topic>Natural water pollution</topic><topic>Norway</topic><topic>Pollution</topic><topic>Pollution, environment geology</topic><topic>Rainwaters, run off water and others</topic><topic>Redundancy analysis (RDA)</topic><topic>Soil Pollutants - analysis</topic><topic>Soil Pollutants - chemistry</topic><topic>Temporal variations</topic><topic>Time Factors</topic><topic>Water flow</topic><topic>Water Movements</topic><topic>Water Pollutants, Chemical - chemistry</topic><topic>Water treatment and pollution</topic><topic>Zinc</topic><topic>Zinc - analysis</topic><topic>Zinc - chemistry</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Heier, Lene Sørlie</creatorcontrib><creatorcontrib>Meland, Sondre</creatorcontrib><creatorcontrib>Ljønes, Marita</creatorcontrib><creatorcontrib>Salbu, Brit</creatorcontrib><creatorcontrib>Strømseng, Arnljot Einride</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Environmental Engineering Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>Civil Engineering Abstracts</collection><collection>MEDLINE - Academic</collection><collection>Aqualine</collection><collection>Environment Abstracts</collection><collection>Pollution Abstracts</collection><collection>Risk Abstracts</collection><collection>Safety Science and Risk</collection><collection>Sustainability Science Abstracts</collection><collection>Water Resources Abstracts</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 2: Ocean Technology, Policy & Non-Living Resources</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><collection>Environment Abstracts</collection><jtitle>The Science of the total environment</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Heier, Lene Sørlie</au><au>Meland, Sondre</au><au>Ljønes, Marita</au><au>Salbu, Brit</au><au>Strømseng, Arnljot Einride</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Short-term temporal variations in speciation of Pb, Cu, Zn and Sb in a shooting range runoff stream</atitle><jtitle>The Science of the total environment</jtitle><addtitle>Sci Total Environ</addtitle><date>2010-05-01</date><risdate>2010</risdate><volume>408</volume><issue>11</issue><spage>2409</spage><epage>2417</epage><pages>2409-2417</pages><issn>0048-9697</issn><eissn>1879-1026</eissn><coden>STENDL</coden><abstract>This study was designed to explore the changes in physico-chemical forms of Pb, Cu, Zn and Sb in a stream draining a contaminated shooting range, located at Steinsjøen in the South-Eastern part of Norway, during a period of 21
days. To obtain information on the element species distribution, an interphased size and charge fractionation system was applied, where membrane filtration (0.45
µm) and ultrafiltration using hollow fibre (nominal cut off 10
kDa) were performed prior to charge fractionation using chromatography (cationic and anionic exchange resins). The results show that Pb mainly was present as particulate and colloidal high molecular mass (HMM) species, Cu as colloidal (HMM) and low molecular mass (LMM) species, while Sb and Zn were mainly present as LMM species. The total element concentrations of Pb, Cu, Zn and Sb were positively correlated to water flow and dissolved organic carbon (DOC), suggesting these are important factors in controlling the run-off of the investigated elements in this catchment. During episodes of higher water flow, the increase in element concentration was mainly in the colloidal fraction. Partial redundancy analysis (pRDA) revealed that variations in pH, HMM organic carbon (HMM OC) and LMM organic carbon (LMM OC) explained 47% of the variation in size distribution of the elements, while variations in precipitation and water flow explained 48% of the variation in the charge distribution of the elements. The variation in concentrations during the period varied by a factor of 4, also stressing the importance of frequent sampling opposed to spot sampling in environmental surveys and risk assessments.</abstract><cop>Kidlington</cop><pub>Elsevier B.V</pub><pmid>20206376</pmid><doi>10.1016/j.scitotenv.2010.02.019</doi><tpages>9</tpages></addata></record> |
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| identifier | ISSN: 0048-9697 |
| ispartof | The Science of the total environment, 2010-05, Vol.408 (11), p.2409-2417 |
| issn | 0048-9697 1879-1026 |
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| source | MEDLINE; Elsevier ScienceDirect Journals |
| subjects | Antimony Antimony - analysis Antimony - chemistry Applied sciences Carbon Chromatography, Ion Exchange Colloids Continental surface waters Copper Copper - analysis Copper - chemistry Earth sciences Earth, ocean, space Engineering and environment geology. Geothermics Environmental Monitoring Exact sciences and technology Firearms Fresh Water - chemistry Ion Exchange Resins Lead (metal) Lead - analysis Lead - chemistry Mathematical models Metal speciation Metals, Heavy - analysis Metals, Heavy - chemistry Natural water pollution Norway Pollution Pollution, environment geology Rainwaters, run off water and others Redundancy analysis (RDA) Soil Pollutants - analysis Soil Pollutants - chemistry Temporal variations Time Factors Water flow Water Movements Water Pollutants, Chemical - chemistry Water treatment and pollution Zinc Zinc - analysis Zinc - chemistry |
| title | Short-term temporal variations in speciation of Pb, Cu, Zn and Sb in a shooting range runoff stream |
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