Attosecond Synchronization of High-Harmonic Soft X-rays
Subfemtosecond light pulses can be obtained by superposing several high harmonics of an intense laser pulse. Provided that the harmonics are emitted simultaneously, increasing their number should result in shorter pulses. However, we found that the high harmonics were not synchronized on an attoseco...
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Veröffentlicht in: | Science (American Association for the Advancement of Science) 2003-11, Vol.302 (5650), p.1540-1543 |
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creator | Mairesse, Y. de Bohan, A. Frasinski, L. J. Merdji, H. Dinu, L. C. Monchicourt, P. Breger, P. Kovačev, M. Taïeb, R. Carré, B. Muller, H. G. Agostini, P. Salières, P. |
description | Subfemtosecond light pulses can be obtained by superposing several high harmonics of an intense laser pulse. Provided that the harmonics are emitted simultaneously, increasing their number should result in shorter pulses. However, we found that the high harmonics were not synchronized on an attosecond time scale, thus setting a lower limit to the achievable x-ray pulse duration. We showed that the synchronization could be improved considerably by controlling the underlying ultrafast electron dynamics, to provide pulses of 130 attoseconds in duration. We discuss the possibility of achieving even shorter pulses, which would allow us to track fast electron processes in matter. |
doi_str_mv | 10.1126/science.1090277 |
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We discuss the possibility of achieving even shorter pulses, which would allow us to track fast electron processes in matter.</description><identifier>ISSN: 0036-8075</identifier><identifier>EISSN: 1095-9203</identifier><identifier>DOI: 10.1126/science.1090277</identifier><identifier>PMID: 14645841</identifier><identifier>CODEN: SCIEAS</identifier><language>eng</language><publisher>Washington, DC: American Association for the Advancement of Science</publisher><subject>Design and construction ; Electric fields ; Electrons ; Emission spectra ; Exact sciences and technology ; Fundamental areas of phenomenology (including applications) ; Harmonics ; Laser beams ; Laser pulses, Ultrashort ; Lasers ; Light ; Nonlinear optics ; Optical measuring instruments ; Optics ; Overtone series ; Physics ; Pulse duration ; Sidebands ; Spectrum analysis ; Time ; Trajectories ; Ultrafast processes; optical pulse generation and pulse compression ; Ultrashort laser pulses ; X-rays</subject><ispartof>Science (American Association for the Advancement of Science), 2003-11, Vol.302 (5650), p.1540-1543</ispartof><rights>Copyright 2003 American Association for the Advancement of Science</rights><rights>2004 INIST-CNRS</rights><rights>COPYRIGHT 2003 American Association for the Advancement of Science</rights><rights>COPYRIGHT 2003 American Association for the Advancement of Science</rights><rights>Copyright American Association for the Advancement of Science Nov 28, 2003</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c782t-80229462929692de1cbdcc358a3788ea6d0be8b3e2bcde30c5699b40f7a435a43</citedby><cites>FETCH-LOGICAL-c782t-80229462929692de1cbdcc358a3788ea6d0be8b3e2bcde30c5699b40f7a435a43</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.jstor.org/stable/pdf/3835779$$EPDF$$P50$$Gjstor$$H</linktopdf><linktohtml>$$Uhttps://www.jstor.org/stable/3835779$$EHTML$$P50$$Gjstor$$H</linktohtml><link.rule.ids>314,776,780,799,2871,2872,27901,27902,57992,58225</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=15971461$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/14645841$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Mairesse, Y.</creatorcontrib><creatorcontrib>de Bohan, A.</creatorcontrib><creatorcontrib>Frasinski, L. 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However, we found that the high harmonics were not synchronized on an attosecond time scale, thus setting a lower limit to the achievable x-ray pulse duration. We showed that the synchronization could be improved considerably by controlling the underlying ultrafast electron dynamics, to provide pulses of 130 attoseconds in duration. We discuss the possibility of achieving even shorter pulses, which would allow us to track fast electron processes in matter.</abstract><cop>Washington, DC</cop><pub>American Association for the Advancement of Science</pub><pmid>14645841</pmid><doi>10.1126/science.1090277</doi><tpages>4</tpages></addata></record> |
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source | American Association for the Advancement of Science; Jstor Complete Legacy |
subjects | Design and construction Electric fields Electrons Emission spectra Exact sciences and technology Fundamental areas of phenomenology (including applications) Harmonics Laser beams Laser pulses, Ultrashort Lasers Light Nonlinear optics Optical measuring instruments Optics Overtone series Physics Pulse duration Sidebands Spectrum analysis Time Trajectories Ultrafast processes optical pulse generation and pulse compression Ultrashort laser pulses X-rays |
title | Attosecond Synchronization of High-Harmonic Soft X-rays |
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