Attosecond Synchronization of High-Harmonic Soft X-rays

Subfemtosecond light pulses can be obtained by superposing several high harmonics of an intense laser pulse. Provided that the harmonics are emitted simultaneously, increasing their number should result in shorter pulses. However, we found that the high harmonics were not synchronized on an attoseco...

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Veröffentlicht in:Science (American Association for the Advancement of Science) 2003-11, Vol.302 (5650), p.1540-1543
Hauptverfasser: Mairesse, Y., de Bohan, A., Frasinski, L. J., Merdji, H., Dinu, L. C., Monchicourt, P., Breger, P., Kovačev, M., Taïeb, R., Carré, B., Muller, H. G., Agostini, P., Salières, P.
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container_end_page 1543
container_issue 5650
container_start_page 1540
container_title Science (American Association for the Advancement of Science)
container_volume 302
creator Mairesse, Y.
de Bohan, A.
Frasinski, L. J.
Merdji, H.
Dinu, L. C.
Monchicourt, P.
Breger, P.
Kovačev, M.
Taïeb, R.
Carré, B.
Muller, H. G.
Agostini, P.
Salières, P.
description Subfemtosecond light pulses can be obtained by superposing several high harmonics of an intense laser pulse. Provided that the harmonics are emitted simultaneously, increasing their number should result in shorter pulses. However, we found that the high harmonics were not synchronized on an attosecond time scale, thus setting a lower limit to the achievable x-ray pulse duration. We showed that the synchronization could be improved considerably by controlling the underlying ultrafast electron dynamics, to provide pulses of 130 attoseconds in duration. We discuss the possibility of achieving even shorter pulses, which would allow us to track fast electron processes in matter.
doi_str_mv 10.1126/science.1090277
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subjects Design and construction
Electric fields
Electrons
Emission spectra
Exact sciences and technology
Fundamental areas of phenomenology (including applications)
Harmonics
Laser beams
Laser pulses, Ultrashort
Lasers
Light
Nonlinear optics
Optical measuring instruments
Optics
Overtone series
Physics
Pulse duration
Sidebands
Spectrum analysis
Time
Trajectories
Ultrafast processes
optical pulse generation and pulse compression
Ultrashort laser pulses
X-rays
title Attosecond Synchronization of High-Harmonic Soft X-rays
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