Conducting Layered Organic-Inorganic Halides Containing -Oriented Perovskite Sheets
Single crystals of the layered organic-inorganic perovskites, [NH$_2$C(I)=NH$_2$]$_2$(CH$_3$NH$_3$)$_m$Sn$_m$I$_{3m+2}$, were prepared by an aqueous solution growth technique. In contrast to the recently discovered family,(C$_4$H$_9$NH$_3$)$_2$ (CH$_3$NH$_3$)$_{n-1}$Sn$_n $I$_{3n+1}$, which consists...
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| Veröffentlicht in: | Science (American Association for the Advancement of Science) 1995-03, Vol.267 (5203), p.1473-1476 |
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| creator | Mitzi, D. B. Wang, S. Feild, C. A. Chess, C. A. Guloy, A. M. |
| description | Single crystals of the layered organic-inorganic perovskites, [NH$_2$C(I)=NH$_2$]$_2$(CH$_3$NH$_3$)$_m$Sn$_m$I$_{3m+2}$, were prepared by an aqueous solution growth technique. In contrast to the recently discovered family,(C$_4$H$_9$NH$_3$)$_2$ (CH$_3$NH$_3$)$_{n-1}$Sn$_n $I$_{3n+1}$, which consists of -terminated perovskite layers, structure determination reveals an unusual structural class with sets of m -oriented CH$_3$NH$_3$SnI$_3$ perovskite sheets separated by iodoformamidinium cations. Whereas the m = 2 compound is semiconducting with a band gap of 0.33 ± 0.05 electron volt, increasing m leads to more metallic character. The ability to control perovskite sheet orientation through the choice of organic cation demonstrates the flexibility provided by organic-inorganic perovskites and adds an important handle for tailoring and understanding lower dimensional transport in layered perovskites. |
| doi_str_mv | 10.1126/science.267.5203.1473 |
| format | Article |
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B. ; Wang, S. ; Feild, C. A. ; Chess, C. A. ; Guloy, A. M.</creator><creatorcontrib>Mitzi, D. B. ; Wang, S. ; Feild, C. A. ; Chess, C. A. ; Guloy, A. M.</creatorcontrib><description>Single crystals of the layered organic-inorganic perovskites, [NH$_2$C(I)=NH$_2$]$_2$(CH$_3$NH$_3$)$_m$Sn$_m$I$_{3m+2}$, were prepared by an aqueous solution growth technique. In contrast to the recently discovered family,(C$_4$H$_9$NH$_3$)$_2$ (CH$_3$NH$_3$)$_{n-1}$Sn$_n $I$_{3n+1}$, which consists of -terminated perovskite layers, structure determination reveals an unusual structural class with sets of m -oriented CH$_3$NH$_3$SnI$_3$ perovskite sheets separated by iodoformamidinium cations. Whereas the m = 2 compound is semiconducting with a band gap of 0.33 ± 0.05 electron volt, increasing m leads to more metallic character. The ability to control perovskite sheet orientation through the choice of organic cation demonstrates the flexibility provided by organic-inorganic perovskites and adds an important handle for tailoring and understanding lower dimensional transport in layered perovskites.</description><identifier>ISSN: 0036-8075</identifier><identifier>EISSN: 1095-9203</identifier><identifier>DOI: 10.1126/science.267.5203.1473</identifier><identifier>PMID: 17743545</identifier><identifier>CODEN: SCIEAS</identifier><language>eng</language><publisher>Washington, DC: American Society for the Advancement of Science</publisher><subject>Atoms ; Biochemistry ; Cations ; Chemistry ; Condensed matter: structure, mechanical and thermal properties ; Coordination ; Coordination compounds ; Crystallography ; Cubic crystals ; Electrical resistivity ; Exact sciences and technology ; Halides ; Inorganic chemistry and origins of life ; Inorganic compounds ; Iodine ; Lead ; Metal complexes ; Organic Chemistry ; Perovskite ; Perovskites ; Physics ; Preparations and properties ; Single crystals ; Structure of solids and liquids; crystallography ; Structure of specific crystalline solids ; Superconductors ; Transport phenomena</subject><ispartof>Science (American Association for the Advancement of Science), 1995-03, Vol.267 (5203), p.1473-1476</ispartof><rights>Copyright 1995 American Association for the Advancement of Science</rights><rights>1995 INIST-CNRS</rights><rights>COPYRIGHT 1995 American Association for the Advancement of Science</rights><rights>COPYRIGHT 1995 American Association for the Advancement of Science</rights><rights>Copyright American Association for the Advancement of Science Mar 10, 1995</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.jstor.org/stable/pdf/2886541$$EPDF$$P50$$Gjstor$$H</linktopdf><linktohtml>$$Uhttps://www.jstor.org/stable/2886541$$EHTML$$P50$$Gjstor$$H</linktohtml><link.rule.ids>314,776,780,799,27901,27902,57992,58225</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=3456897$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/17743545$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Mitzi, D. B.</creatorcontrib><creatorcontrib>Wang, S.</creatorcontrib><creatorcontrib>Feild, C. A.</creatorcontrib><creatorcontrib>Chess, C. A.</creatorcontrib><creatorcontrib>Guloy, A. M.</creatorcontrib><title>Conducting Layered Organic-Inorganic Halides Containing -Oriented Perovskite Sheets</title><title>Science (American Association for the Advancement of Science)</title><addtitle>Science</addtitle><description>Single crystals of the layered organic-inorganic perovskites, [NH$_2$C(I)=NH$_2$]$_2$(CH$_3$NH$_3$)$_m$Sn$_m$I$_{3m+2}$, were prepared by an aqueous solution growth technique. In contrast to the recently discovered family,(C$_4$H$_9$NH$_3$)$_2$ (CH$_3$NH$_3$)$_{n-1}$Sn$_n $I$_{3n+1}$, which consists of -terminated perovskite layers, structure determination reveals an unusual structural class with sets of m -oriented CH$_3$NH$_3$SnI$_3$ perovskite sheets separated by iodoformamidinium cations. Whereas the m = 2 compound is semiconducting with a band gap of 0.33 ± 0.05 electron volt, increasing m leads to more metallic character. 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B.</au><au>Wang, S.</au><au>Feild, C. A.</au><au>Chess, C. A.</au><au>Guloy, A. M.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Conducting Layered Organic-Inorganic Halides Containing -Oriented Perovskite Sheets</atitle><jtitle>Science (American Association for the Advancement of Science)</jtitle><addtitle>Science</addtitle><date>1995-03-10</date><risdate>1995</risdate><volume>267</volume><issue>5203</issue><spage>1473</spage><epage>1476</epage><pages>1473-1476</pages><issn>0036-8075</issn><eissn>1095-9203</eissn><coden>SCIEAS</coden><abstract>Single crystals of the layered organic-inorganic perovskites, [NH$_2$C(I)=NH$_2$]$_2$(CH$_3$NH$_3$)$_m$Sn$_m$I$_{3m+2}$, were prepared by an aqueous solution growth technique. In contrast to the recently discovered family,(C$_4$H$_9$NH$_3$)$_2$ (CH$_3$NH$_3$)$_{n-1}$Sn$_n $I$_{3n+1}$, which consists of -terminated perovskite layers, structure determination reveals an unusual structural class with sets of m -oriented CH$_3$NH$_3$SnI$_3$ perovskite sheets separated by iodoformamidinium cations. Whereas the m = 2 compound is semiconducting with a band gap of 0.33 ± 0.05 electron volt, increasing m leads to more metallic character. The ability to control perovskite sheet orientation through the choice of organic cation demonstrates the flexibility provided by organic-inorganic perovskites and adds an important handle for tailoring and understanding lower dimensional transport in layered perovskites.</abstract><cop>Washington, DC</cop><pub>American Society for the Advancement of Science</pub><pmid>17743545</pmid><doi>10.1126/science.267.5203.1473</doi><tpages>4</tpages></addata></record> |
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| source | American Association for the Advancement of Science; Jstor Complete Legacy |
| subjects | Atoms Biochemistry Cations Chemistry Condensed matter: structure, mechanical and thermal properties Coordination Coordination compounds Crystallography Cubic crystals Electrical resistivity Exact sciences and technology Halides Inorganic chemistry and origins of life Inorganic compounds Iodine Lead Metal complexes Organic Chemistry Perovskite Perovskites Physics Preparations and properties Single crystals Structure of solids and liquids crystallography Structure of specific crystalline solids Superconductors Transport phenomena |
| title | Conducting Layered Organic-Inorganic Halides Containing -Oriented Perovskite Sheets |
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