Conductance Switching in Single Molecules through Conformational Changes
We tracked over time the conductance switching of single and bundled phenylene ethynylene oligomers isolated in matrices of alkanethiolate monolayers. The persistence times for isolated and bundled molecules in either the ON or OFF switch state range from seconds to tens of hours. When the surroundi...
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| Veröffentlicht in: | Science (American Association for the Advancement of Science) 2001-06, Vol.292 (5525), p.2303-2307 |
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| container_title | Science (American Association for the Advancement of Science) |
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| creator | Donhauser, Z. J. Mantooth, B. A. Kelly, K. F. Bumm, L. A. Monnell, J. D. Stapleton, J. J. Price, D. W. Rawlett, A. M. Allara, D. L. Tour, J. M. Weiss, P. S. |
| description | We tracked over time the conductance switching of single and bundled phenylene ethynylene oligomers isolated in matrices of alkanethiolate monolayers. The persistence times for isolated and bundled molecules in either the ON or OFF switch state range from seconds to tens of hours. When the surrounding matrix is well ordered, the rate at which the inserted molecules switch is low. Conversely, when the surrounding matrix is poorly ordered, the inserted molecules switch more often. We conclude that the switching is a result of conformational changes in the molecules or bundles, rather than electrostatic effects of charge transfer. |
| doi_str_mv | 10.1126/science.1060294 |
| format | Article |
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J. ; Mantooth, B. A. ; Kelly, K. F. ; Bumm, L. A. ; Monnell, J. D. ; Stapleton, J. J. ; Price, D. W. ; Rawlett, A. M. ; Allara, D. L. ; Tour, J. M. ; Weiss, P. S.</creator><creatorcontrib>Donhauser, Z. J. ; Mantooth, B. A. ; Kelly, K. F. ; Bumm, L. A. ; Monnell, J. D. ; Stapleton, J. J. ; Price, D. W. ; Rawlett, A. M. ; Allara, D. L. ; Tour, J. M. ; Weiss, P. S.</creatorcontrib><description>We tracked over time the conductance switching of single and bundled phenylene ethynylene oligomers isolated in matrices of alkanethiolate monolayers. The persistence times for isolated and bundled molecules in either the ON or OFF switch state range from seconds to tens of hours. When the surrounding matrix is well ordered, the rate at which the inserted molecules switch is low. Conversely, when the surrounding matrix is poorly ordered, the inserted molecules switch more often. We conclude that the switching is a result of conformational changes in the molecules or bundles, rather than electrostatic effects of charge transfer.</description><identifier>ISSN: 0036-8075</identifier><identifier>EISSN: 1095-9203</identifier><identifier>DOI: 10.1126/science.1060294</identifier><identifier>PMID: 11423655</identifier><identifier>CODEN: SCIEAS</identifier><language>eng</language><publisher>Washington, DC: American Society for the Advancement of Science</publisher><subject>Algorithms ; Atomic and molecular physics ; Chemistry ; Cosmic microwave background radiation ; Electric fields ; Electric potential ; Exact sciences and technology ; Galaxies ; Glacial lakes ; Imaging ; Logic ; Material films ; Memory ; Molecular properties and interactions with photons ; Molecules ; Movies ; Oligomers ; Other topics in molecular properties and interactions with photons ; Persistence ; Physics ; Physiological aspects ; Spectral energy distribution ; Statistical Analysis ; Surface Structure ; Topography</subject><ispartof>Science (American Association for the Advancement of Science), 2001-06, Vol.292 (5525), p.2303-2307</ispartof><rights>Copyright 2001 American Association for the Advancement of Science</rights><rights>2001 INIST-CNRS</rights><rights>COPYRIGHT 2001 American Association for the Advancement of Science</rights><rights>COPYRIGHT 2001 American Association for the Advancement of Science</rights><rights>Copyright American Association for the Advancement of Science Jun 22, 2001</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c774t-c281b480d4850cb9ebf666be547aaa7d509a0d13369bbd52a3d916f6877834cc3</citedby><cites>FETCH-LOGICAL-c774t-c281b480d4850cb9ebf666be547aaa7d509a0d13369bbd52a3d916f6877834cc3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.jstor.org/stable/pdf/3083880$$EPDF$$P50$$Gjstor$$H</linktopdf><linktohtml>$$Uhttps://www.jstor.org/stable/3083880$$EHTML$$P50$$Gjstor$$H</linktohtml><link.rule.ids>314,776,780,799,2871,2872,27901,27902,57992,58225</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=1062646$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/11423655$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Donhauser, Z. 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When the surrounding matrix is well ordered, the rate at which the inserted molecules switch is low. Conversely, when the surrounding matrix is poorly ordered, the inserted molecules switch more often. We conclude that the switching is a result of conformational changes in the molecules or bundles, rather than electrostatic effects of charge transfer.</description><subject>Algorithms</subject><subject>Atomic and molecular physics</subject><subject>Chemistry</subject><subject>Cosmic microwave background radiation</subject><subject>Electric fields</subject><subject>Electric potential</subject><subject>Exact sciences and technology</subject><subject>Galaxies</subject><subject>Glacial lakes</subject><subject>Imaging</subject><subject>Logic</subject><subject>Material films</subject><subject>Memory</subject><subject>Molecular properties and interactions with photons</subject><subject>Molecules</subject><subject>Movies</subject><subject>Oligomers</subject><subject>Other topics in molecular properties and interactions with photons</subject><subject>Persistence</subject><subject>Physics</subject><subject>Physiological aspects</subject><subject>Spectral energy distribution</subject><subject>Statistical Analysis</subject><subject>Surface Structure</subject><subject>Topography</subject><issn>0036-8075</issn><issn>1095-9203</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2001</creationdate><recordtype>article</recordtype><sourceid>8G5</sourceid><sourceid>BEC</sourceid><sourceid>BENPR</sourceid><sourceid>GUQSH</sourceid><sourceid>M2O</sourceid><recordid>eNqN0kFv0zAUB3ALgVgpnLkgFCEEHJbNjh3bOY4IukmFHgpcI8d5SV258bATAd8eT42AogoqH55k_947PP8RekrwBSEZvwzaQK_hgmCOs4LdQzOCizwtMkzvoxnGlKcSi_wMPQphi3F8K-hDdEYIyyjP8xm6Ll3fjHpQcUqy_mYGvTF9l5g-WcdqIfngLOjRQkiGjXdjt0liR-v8Tg3G9com5Ub1HYTH6EGrbIAnU52jz-_ffSqv0-VqcVNeLVMtBBtSnUlSM4kbJnOs6wLqlnNeQ86EUko0OS4UbgilvKjrJs8UbQrCWy6FkJRpTefo9X7urXdfRwhDtTNBg7WqBzeGSjBKYrPAUb76t4zbkJLS_8KMcyEZu5v44i-4daOPS4iG0FxiFsscne9RpyxUJu5q8Ep30INX1vXQmnh9JeL2cYGLyNMjPJ4GdkYf828OfCQDfB86NYZQ3aw_nkxXX06mbxenUrlYHtDzY1Q7a6GDKuaiXB3wyz3X3oXgoa1uvdkp_6MiuLqLezXFvZriHjueTx8y1jtofvsp3xG8nIAKWtnWx5yb8MdcnnHGI3u2Z9swOP_rmWJJpcT0J-7VDDI</recordid><startdate>20010622</startdate><enddate>20010622</enddate><creator>Donhauser, Z. 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When the surrounding matrix is well ordered, the rate at which the inserted molecules switch is low. Conversely, when the surrounding matrix is poorly ordered, the inserted molecules switch more often. We conclude that the switching is a result of conformational changes in the molecules or bundles, rather than electrostatic effects of charge transfer.</abstract><cop>Washington, DC</cop><pub>American Society for the Advancement of Science</pub><pmid>11423655</pmid><doi>10.1126/science.1060294</doi><tpages>5</tpages></addata></record> |
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| source | American Association for the Advancement of Science; Jstor Complete Legacy |
| subjects | Algorithms Atomic and molecular physics Chemistry Cosmic microwave background radiation Electric fields Electric potential Exact sciences and technology Galaxies Glacial lakes Imaging Logic Material films Memory Molecular properties and interactions with photons Molecules Movies Oligomers Other topics in molecular properties and interactions with photons Persistence Physics Physiological aspects Spectral energy distribution Statistical Analysis Surface Structure Topography |
| title | Conductance Switching in Single Molecules through Conformational Changes |
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