Broadband near-field interference spectroscopy of metal nanoparticles using a femtosecond white-light continuum
We demonstrate a new nanoscale spectroscopic technique that combines subwavelength near-field imaging with broadband interference spectroscopy. We apply this technique to study phase spectra of surface plasmons in individual gold nanoparticles and nanoparticle dimers. Collective plasmon oscillations...
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Veröffentlicht in: | Optics letters 2003-09, Vol.28 (18), p.1686-1688 |
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creator | Mikhailovsky, A A Petruska, M A Stockman, M I Klimov, V I |
description | We demonstrate a new nanoscale spectroscopic technique that combines subwavelength near-field imaging with broadband interference spectroscopy. We apply this technique to study phase spectra of surface plasmons in individual gold nanoparticles and nanoparticle dimers. Collective plasmon oscillations in selected nanostructures are excited by a femtosecond white-light continuum transmitted through a subwavelength aperture. The interference spectra detected in the far field result from the coherent superposition of the aperture field and the secondary field re-emitted by the nanostructure. The analysis of these spectra allows us to accurately measure the positions and damping constants of single-nanostructure plasmon resonances. |
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The analysis of these spectra allows us to accurately measure the positions and damping constants of single-nanostructure plasmon resonances.</description><identifier>ISSN: 0146-9592</identifier><identifier>EISSN: 1539-4794</identifier><identifier>DOI: 10.1364/OL.28.001686</identifier><identifier>PMID: 13677537</identifier><language>eng</language><publisher>United States</publisher><ispartof>Optics letters, 2003-09, Vol.28 (18), p.1686-1688</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c330t-62aa7c452bed8430186e248ee8085aa9ae4355431269ecc067ff6b173c6a5e923</citedby><cites>FETCH-LOGICAL-c330t-62aa7c452bed8430186e248ee8085aa9ae4355431269ecc067ff6b173c6a5e923</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>315,781,785,3259,27929,27930</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/13677537$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Mikhailovsky, A A</creatorcontrib><creatorcontrib>Petruska, M A</creatorcontrib><creatorcontrib>Stockman, M I</creatorcontrib><creatorcontrib>Klimov, V I</creatorcontrib><title>Broadband near-field interference spectroscopy of metal nanoparticles using a femtosecond white-light continuum</title><title>Optics letters</title><addtitle>Opt Lett</addtitle><description>We demonstrate a new nanoscale spectroscopic technique that combines subwavelength near-field imaging with broadband interference spectroscopy. We apply this technique to study phase spectra of surface plasmons in individual gold nanoparticles and nanoparticle dimers. Collective plasmon oscillations in selected nanostructures are excited by a femtosecond white-light continuum transmitted through a subwavelength aperture. The interference spectra detected in the far field result from the coherent superposition of the aperture field and the secondary field re-emitted by the nanostructure. 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We apply this technique to study phase spectra of surface plasmons in individual gold nanoparticles and nanoparticle dimers. Collective plasmon oscillations in selected nanostructures are excited by a femtosecond white-light continuum transmitted through a subwavelength aperture. The interference spectra detected in the far field result from the coherent superposition of the aperture field and the secondary field re-emitted by the nanostructure. The analysis of these spectra allows us to accurately measure the positions and damping constants of single-nanostructure plasmon resonances.</abstract><cop>United States</cop><pmid>13677537</pmid><doi>10.1364/OL.28.001686</doi><tpages>3</tpages></addata></record> |
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title | Broadband near-field interference spectroscopy of metal nanoparticles using a femtosecond white-light continuum |
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