Shear ordering in polymer photonic crystals

Shear ordering in polymer photonic crystals

Optical scattering spectra are recorded in situ on flowing colloidal polymeric nanocomposites which are sheared into photonic crystals at 150 degrees C using a high-pressure quartz-cell multipass rheometer. Broadband spectroscopy of the resonant Bragg scattering peak allows the direct observation of...

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Veröffentlicht in:Physical review. E, Statistical, nonlinear, and soft matter physics Statistical, nonlinear, and soft matter physics, 2010-02, Vol.81 (2 Pt 1), p.020401-020401, Article 020401
Hauptverfasser: Snoswell, D R E, Kontogeorgos, A, Baumberg, J J, Lord, T D, Mackley, M R, Spahn, P, Hellmann, G P
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Sprache:eng
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Mechanical Phenomena
Nanocomposites - chemistry
Optical Phenomena
Photons
Polymers - chemistry
Temperature
Viscosity
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container_end_page 020401
container_issue 2 Pt 1
container_start_page 020401
container_title Physical review. E, Statistical, nonlinear, and soft matter physics
container_volume 81
creator Snoswell, D R E
Kontogeorgos, A
Baumberg, J J
Lord, T D
Mackley, M R
Spahn, P
Hellmann, G P
description Optical scattering spectra are recorded in situ on flowing colloidal polymeric nanocomposites which are sheared into photonic crystals at 150 degrees C using a high-pressure quartz-cell multipass rheometer. Broadband spectroscopy of the resonant Bragg scattering peak allows the direct observation of crystal formation and melting of monodisperse core-shell particles. A range of flow conditions of this solventless, highly viscous melt reveals four distinct regimes of crystal growth and decay which match a simple rheological model. Extraction of crystal thickness, order and lattice spacing are validated by one-dimensional electromagnetic simulations.
doi_str_mv 10.1103/PhysRevE.81.020401
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subjects Mechanical Phenomena
Nanocomposites - chemistry
Optical Phenomena
Photons
Polymers - chemistry
Temperature
Viscosity
title Shear ordering in polymer photonic crystals
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