Rheological microscopy: local mechanical properties from microrheology
We demonstrate how tracer microrheology methods can be extended to study submicron scale variations in the viscoelastic response of soft materials; in particular, a semidilute solution of lambda-DNA. The polymer concentration is depleted near the surfaces of the tracer particles, within a distance c...
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Veröffentlicht in: | Physical review letters 2003-03, Vol.90 (10), p.108301-108301 |
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creator | Chen, D T Weeks, E R Crocker, J C Islam, M F Verma, R Gruber, J Levine, A J Lubensky, T C Yodh, A G |
description | We demonstrate how tracer microrheology methods can be extended to study submicron scale variations in the viscoelastic response of soft materials; in particular, a semidilute solution of lambda-DNA. The polymer concentration is depleted near the surfaces of the tracer particles, within a distance comparable to the polymer correlation length. The rheology of this microscopic layer alters the tracers' motion and can be precisely quantified using one- and two-point microrheology. Interestingly, we found this mechanically distinct layer to be twice as thick as the layer of depleted concentration, likely due to solvent drainage through the locally perturbed polymer structure. |
doi_str_mv | 10.1103/PhysRevLett.90.108301 |
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Interestingly, we found this mechanically distinct layer to be twice as thick as the layer of depleted concentration, likely due to solvent drainage through the locally perturbed polymer structure.</description><subject>Bacteriophage lambda - genetics</subject><subject>DNA, Viral - chemistry</subject><subject>Elasticity</subject><subject>Fluorescent Dyes - chemistry</subject><subject>Microscopy - methods</subject><subject>Models, Chemical</subject><subject>Polystyrenes - chemistry</subject><subject>Rheology - methods</subject><subject>Rhodamines - chemistry</subject><subject>Viscosity</subject><issn>0031-9007</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2003</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNo1j8FOwzAQRH0A0VL4BFBP3FJ2aze2uaGKAlIlUAXnyLE3JCipg50i5e8b2nKa1czb1SxjNwgzROD372UfN_S7pq6b6cEDxQHP2BiAY6IB5IhdxvgNADhP1QUb_YkGrsdstSnJ1_6rsqaeNpUNPlrf9g_T2h8csqXZHsI2-JZCV1GcFsE3Rzgct_srdl6YOtL1SSfsc_X0sXxJ1m_Pr8vHddIi112SK7FAIbSDNJcpalQOQXIiaeZY5Kkj49RCpVYJoeRQcRgIHcmUHAmyfMLujneHNj87il3WVNFSXZst-V3MJEc1l1wM4O0J3OUNuawNVWNCn_1_zvfvUFyp</recordid><startdate>20030314</startdate><enddate>20030314</enddate><creator>Chen, D T</creator><creator>Weeks, E R</creator><creator>Crocker, J C</creator><creator>Islam, M F</creator><creator>Verma, R</creator><creator>Gruber, J</creator><creator>Levine, A J</creator><creator>Lubensky, T C</creator><creator>Yodh, A G</creator><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>7X8</scope></search><sort><creationdate>20030314</creationdate><title>Rheological microscopy: local mechanical properties from microrheology</title><author>Chen, D T ; Weeks, E R ; Crocker, J C ; Islam, M F ; Verma, R ; Gruber, J ; Levine, A J ; Lubensky, T C ; Yodh, A G</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-p139t-b8451449d06b761918d1073ee7a21fb6dead8586c84487890c84e1de76ede4ec3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2003</creationdate><topic>Bacteriophage lambda - genetics</topic><topic>DNA, Viral - chemistry</topic><topic>Elasticity</topic><topic>Fluorescent Dyes - chemistry</topic><topic>Microscopy - methods</topic><topic>Models, Chemical</topic><topic>Polystyrenes - chemistry</topic><topic>Rheology - methods</topic><topic>Rhodamines - chemistry</topic><topic>Viscosity</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chen, D T</creatorcontrib><creatorcontrib>Weeks, E R</creatorcontrib><creatorcontrib>Crocker, J C</creatorcontrib><creatorcontrib>Islam, M F</creatorcontrib><creatorcontrib>Verma, R</creatorcontrib><creatorcontrib>Gruber, J</creatorcontrib><creatorcontrib>Levine, A J</creatorcontrib><creatorcontrib>Lubensky, T C</creatorcontrib><creatorcontrib>Yodh, A G</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>MEDLINE - Academic</collection><jtitle>Physical review letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Chen, D T</au><au>Weeks, E R</au><au>Crocker, J C</au><au>Islam, M F</au><au>Verma, R</au><au>Gruber, J</au><au>Levine, A J</au><au>Lubensky, T C</au><au>Yodh, A G</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Rheological microscopy: local mechanical properties from microrheology</atitle><jtitle>Physical review letters</jtitle><addtitle>Phys Rev Lett</addtitle><date>2003-03-14</date><risdate>2003</risdate><volume>90</volume><issue>10</issue><spage>108301</spage><epage>108301</epage><pages>108301-108301</pages><issn>0031-9007</issn><abstract>We demonstrate how tracer microrheology methods can be extended to study submicron scale variations in the viscoelastic response of soft materials; in particular, a semidilute solution of lambda-DNA. 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subjects | Bacteriophage lambda - genetics DNA, Viral - chemistry Elasticity Fluorescent Dyes - chemistry Microscopy - methods Models, Chemical Polystyrenes - chemistry Rheology - methods Rhodamines - chemistry Viscosity |
title | Rheological microscopy: local mechanical properties from microrheology |
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