Rheological microscopy: local mechanical properties from microrheology

We demonstrate how tracer microrheology methods can be extended to study submicron scale variations in the viscoelastic response of soft materials; in particular, a semidilute solution of lambda-DNA. The polymer concentration is depleted near the surfaces of the tracer particles, within a distance c...

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Veröffentlicht in:Physical review letters 2003-03, Vol.90 (10), p.108301-108301
Hauptverfasser: Chen, D T, Weeks, E R, Crocker, J C, Islam, M F, Verma, R, Gruber, J, Levine, A J, Lubensky, T C, Yodh, A G
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container_end_page 108301
container_issue 10
container_start_page 108301
container_title Physical review letters
container_volume 90
creator Chen, D T
Weeks, E R
Crocker, J C
Islam, M F
Verma, R
Gruber, J
Levine, A J
Lubensky, T C
Yodh, A G
description We demonstrate how tracer microrheology methods can be extended to study submicron scale variations in the viscoelastic response of soft materials; in particular, a semidilute solution of lambda-DNA. The polymer concentration is depleted near the surfaces of the tracer particles, within a distance comparable to the polymer correlation length. The rheology of this microscopic layer alters the tracers' motion and can be precisely quantified using one- and two-point microrheology. Interestingly, we found this mechanically distinct layer to be twice as thick as the layer of depleted concentration, likely due to solvent drainage through the locally perturbed polymer structure.
doi_str_mv 10.1103/PhysRevLett.90.108301
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subjects Bacteriophage lambda - genetics
DNA, Viral - chemistry
Elasticity
Fluorescent Dyes - chemistry
Microscopy - methods
Models, Chemical
Polystyrenes - chemistry
Rheology - methods
Rhodamines - chemistry
Viscosity
title Rheological microscopy: local mechanical properties from microrheology
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