Connection between Adam-Gibbs theory and spatially heterogeneous dynamics

We investigate the spatially heterogeneous dynamics in the extended simple point charge model of water using molecular dynamics simulations. We relate the average mass n* of mobile particle clusters to the diffusion constant and the configurational entropy. Hence, n* can be interpreted as the mass o...

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Veröffentlicht in:	Physical review letters 2003-02, Vol.90 (8), p.085506-085506, Article 085506
Hauptverfasser:	Giovambattista, Nicolas, Buldyrev, Sergey V, Starr, Francis W, Stanley, H Eugene
Format:	Artikel
Sprache:	eng
Online-Zugang:	Volltext
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