MOCVD-Loading of Mesoporous Siliceous Matrices with Cu/ZnO: Supported Catalysts for Methanol Synthesis

Consecutive vaporization cycles for the preparation of heterogeneous catalysts: Active Cu‐ and ZnO‐containing methanol‐synthesis catalysts were obtained by vaporizing suitable organometallic precursors into mesoporous silicates, followed by thermal treatment (see scheme). The catalytically active co...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Angewandte Chemie International Edition 2004-05, Vol.43 (21), p.2839-2842
Hauptverfasser: Becker, Ralf, Parala, Harish, Hipler, Frank, Tkachenko, Olga P., Klementiev, Konstantin V., Grünert, Wolfgang, Wilmer, Hagen, Hinrichsen, Olaf, Muhler, Martin, Birkner, Alexander, Wöll, Christof, Schäfer, Sven, Fischer, Roland A.
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 2842
container_issue 21
container_start_page 2839
container_title Angewandte Chemie International Edition
container_volume 43
creator Becker, Ralf
Parala, Harish
Hipler, Frank
Tkachenko, Olga P.
Klementiev, Konstantin V.
Grünert, Wolfgang
Wilmer, Hagen
Hinrichsen, Olaf
Muhler, Martin
Birkner, Alexander
Wöll, Christof
Schäfer, Sven
Fischer, Roland A.
description Consecutive vaporization cycles for the preparation of heterogeneous catalysts: Active Cu‐ and ZnO‐containing methanol‐synthesis catalysts were obtained by vaporizing suitable organometallic precursors into mesoporous silicates, followed by thermal treatment (see scheme). The catalytically active components in the final material have nanoscopic dimensions. The methanol production by the catalysts is similar to that of systems synthesized by the classical route.
doi_str_mv 10.1002/anie.200351166
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_71936451</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>71936451</sourcerecordid><originalsourceid>FETCH-LOGICAL-c3796-e07758b8eb2e76f5b5883c0c2c12badce137ced6de8361d3420d5bf6c4bb0ba03</originalsourceid><addsrcrecordid>eNqFkDtv2zAUhYmiQd5rx4JTNzmkaJJytkCN87LjwWkLZCFI6ipmK4suSSHxv48MG0m2TPcM3_mAexD6RsmAEpKf6dbBICeEcUqF-IIOKc9pxqRkX_s8ZCyTBacH6CjGvz1fFETsowPKKSdSsENUT2fl75_ZxOvKtU_Y13gK0a988F3Ec9c4C5s01Sn0MeJnlxa47M4e29k5nnernkxQ4VIn3axjirj2oVekhW59g-frNi0guniC9mrdRDjd3WP0a3z5UF5nk9nVTXkxySyTI5EBkZIXpgCTgxQ1N7womCU2tzQ3urJAmbRQiQoKJmjFhjmpuKmFHRpDjCbsGP3YelfB_-8gJrV00ULT6Hbzh5J0xMSQ0x4cbEEbfIwBarUKbqnDWlGiNsuqzbLqbdm-8H1n7swSqnd8N2UPjLbAs2tg_YlOXdzfXH6UZ9uuiwle3ro6_FNCMsnVn_sr9fhwN55f01s1Zq9T0ZWh</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>71936451</pqid></control><display><type>article</type><title>MOCVD-Loading of Mesoporous Siliceous Matrices with Cu/ZnO: Supported Catalysts for Methanol Synthesis</title><source>Access via Wiley Online Library</source><creator>Becker, Ralf ; Parala, Harish ; Hipler, Frank ; Tkachenko, Olga P. ; Klementiev, Konstantin V. ; Grünert, Wolfgang ; Wilmer, Hagen ; Hinrichsen, Olaf ; Muhler, Martin ; Birkner, Alexander ; Wöll, Christof ; Schäfer, Sven ; Fischer, Roland A.</creator><creatorcontrib>Becker, Ralf ; Parala, Harish ; Hipler, Frank ; Tkachenko, Olga P. ; Klementiev, Konstantin V. ; Grünert, Wolfgang ; Wilmer, Hagen ; Hinrichsen, Olaf ; Muhler, Martin ; Birkner, Alexander ; Wöll, Christof ; Schäfer, Sven ; Fischer, Roland A.</creatorcontrib><description>Consecutive vaporization cycles for the preparation of heterogeneous catalysts: Active Cu‐ and ZnO‐containing methanol‐synthesis catalysts were obtained by vaporizing suitable organometallic precursors into mesoporous silicates, followed by thermal treatment (see scheme). The catalytically active components in the final material have nanoscopic dimensions. The methanol production by the catalysts is similar to that of systems synthesized by the classical route.</description><identifier>ISSN: 1433-7851</identifier><identifier>EISSN: 1521-3773</identifier><identifier>DOI: 10.1002/anie.200351166</identifier><identifier>PMID: 15150763</identifier><language>eng</language><publisher>Weinheim: WILEY-VCH Verlag</publisher><subject>copper ; CVD (chemical vapor deposition) ; heterogeneous catalysis ; mesoporous materials ; methanol synthesis ; zinc oxide</subject><ispartof>Angewandte Chemie International Edition, 2004-05, Vol.43 (21), p.2839-2842</ispartof><rights>Copyright © 2004 WILEY‐VCH Verlag GmbH &amp; Co. KGaA, Weinheim</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c3796-e07758b8eb2e76f5b5883c0c2c12badce137ced6de8361d3420d5bf6c4bb0ba03</citedby><cites>FETCH-LOGICAL-c3796-e07758b8eb2e76f5b5883c0c2c12badce137ced6de8361d3420d5bf6c4bb0ba03</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fanie.200351166$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fanie.200351166$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>315,781,785,1418,27929,27930,45579,45580</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/15150763$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Becker, Ralf</creatorcontrib><creatorcontrib>Parala, Harish</creatorcontrib><creatorcontrib>Hipler, Frank</creatorcontrib><creatorcontrib>Tkachenko, Olga P.</creatorcontrib><creatorcontrib>Klementiev, Konstantin V.</creatorcontrib><creatorcontrib>Grünert, Wolfgang</creatorcontrib><creatorcontrib>Wilmer, Hagen</creatorcontrib><creatorcontrib>Hinrichsen, Olaf</creatorcontrib><creatorcontrib>Muhler, Martin</creatorcontrib><creatorcontrib>Birkner, Alexander</creatorcontrib><creatorcontrib>Wöll, Christof</creatorcontrib><creatorcontrib>Schäfer, Sven</creatorcontrib><creatorcontrib>Fischer, Roland A.</creatorcontrib><title>MOCVD-Loading of Mesoporous Siliceous Matrices with Cu/ZnO: Supported Catalysts for Methanol Synthesis</title><title>Angewandte Chemie International Edition</title><addtitle>Angewandte Chemie International Edition</addtitle><description>Consecutive vaporization cycles for the preparation of heterogeneous catalysts: Active Cu‐ and ZnO‐containing methanol‐synthesis catalysts were obtained by vaporizing suitable organometallic precursors into mesoporous silicates, followed by thermal treatment (see scheme). The catalytically active components in the final material have nanoscopic dimensions. The methanol production by the catalysts is similar to that of systems synthesized by the classical route.</description><subject>copper</subject><subject>CVD (chemical vapor deposition)</subject><subject>heterogeneous catalysis</subject><subject>mesoporous materials</subject><subject>methanol synthesis</subject><subject>zinc oxide</subject><issn>1433-7851</issn><issn>1521-3773</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2004</creationdate><recordtype>article</recordtype><recordid>eNqFkDtv2zAUhYmiQd5rx4JTNzmkaJJytkCN87LjwWkLZCFI6ipmK4suSSHxv48MG0m2TPcM3_mAexD6RsmAEpKf6dbBICeEcUqF-IIOKc9pxqRkX_s8ZCyTBacH6CjGvz1fFETsowPKKSdSsENUT2fl75_ZxOvKtU_Y13gK0a988F3Ec9c4C5s01Sn0MeJnlxa47M4e29k5nnernkxQ4VIn3axjirj2oVekhW59g-frNi0guniC9mrdRDjd3WP0a3z5UF5nk9nVTXkxySyTI5EBkZIXpgCTgxQ1N7womCU2tzQ3urJAmbRQiQoKJmjFhjmpuKmFHRpDjCbsGP3YelfB_-8gJrV00ULT6Hbzh5J0xMSQ0x4cbEEbfIwBarUKbqnDWlGiNsuqzbLqbdm-8H1n7swSqnd8N2UPjLbAs2tg_YlOXdzfXH6UZ9uuiwle3ro6_FNCMsnVn_sr9fhwN55f01s1Zq9T0ZWh</recordid><startdate>20040517</startdate><enddate>20040517</enddate><creator>Becker, Ralf</creator><creator>Parala, Harish</creator><creator>Hipler, Frank</creator><creator>Tkachenko, Olga P.</creator><creator>Klementiev, Konstantin V.</creator><creator>Grünert, Wolfgang</creator><creator>Wilmer, Hagen</creator><creator>Hinrichsen, Olaf</creator><creator>Muhler, Martin</creator><creator>Birkner, Alexander</creator><creator>Wöll, Christof</creator><creator>Schäfer, Sven</creator><creator>Fischer, Roland A.</creator><general>WILEY-VCH Verlag</general><general>WILEY‐VCH Verlag</general><scope>BSCLL</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope></search><sort><creationdate>20040517</creationdate><title>MOCVD-Loading of Mesoporous Siliceous Matrices with Cu/ZnO: Supported Catalysts for Methanol Synthesis</title><author>Becker, Ralf ; Parala, Harish ; Hipler, Frank ; Tkachenko, Olga P. ; Klementiev, Konstantin V. ; Grünert, Wolfgang ; Wilmer, Hagen ; Hinrichsen, Olaf ; Muhler, Martin ; Birkner, Alexander ; Wöll, Christof ; Schäfer, Sven ; Fischer, Roland A.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c3796-e07758b8eb2e76f5b5883c0c2c12badce137ced6de8361d3420d5bf6c4bb0ba03</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2004</creationdate><topic>copper</topic><topic>CVD (chemical vapor deposition)</topic><topic>heterogeneous catalysis</topic><topic>mesoporous materials</topic><topic>methanol synthesis</topic><topic>zinc oxide</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Becker, Ralf</creatorcontrib><creatorcontrib>Parala, Harish</creatorcontrib><creatorcontrib>Hipler, Frank</creatorcontrib><creatorcontrib>Tkachenko, Olga P.</creatorcontrib><creatorcontrib>Klementiev, Konstantin V.</creatorcontrib><creatorcontrib>Grünert, Wolfgang</creatorcontrib><creatorcontrib>Wilmer, Hagen</creatorcontrib><creatorcontrib>Hinrichsen, Olaf</creatorcontrib><creatorcontrib>Muhler, Martin</creatorcontrib><creatorcontrib>Birkner, Alexander</creatorcontrib><creatorcontrib>Wöll, Christof</creatorcontrib><creatorcontrib>Schäfer, Sven</creatorcontrib><creatorcontrib>Fischer, Roland A.</creatorcontrib><collection>Istex</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>Angewandte Chemie International Edition</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Becker, Ralf</au><au>Parala, Harish</au><au>Hipler, Frank</au><au>Tkachenko, Olga P.</au><au>Klementiev, Konstantin V.</au><au>Grünert, Wolfgang</au><au>Wilmer, Hagen</au><au>Hinrichsen, Olaf</au><au>Muhler, Martin</au><au>Birkner, Alexander</au><au>Wöll, Christof</au><au>Schäfer, Sven</au><au>Fischer, Roland A.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>MOCVD-Loading of Mesoporous Siliceous Matrices with Cu/ZnO: Supported Catalysts for Methanol Synthesis</atitle><jtitle>Angewandte Chemie International Edition</jtitle><addtitle>Angewandte Chemie International Edition</addtitle><date>2004-05-17</date><risdate>2004</risdate><volume>43</volume><issue>21</issue><spage>2839</spage><epage>2842</epage><pages>2839-2842</pages><issn>1433-7851</issn><eissn>1521-3773</eissn><abstract>Consecutive vaporization cycles for the preparation of heterogeneous catalysts: Active Cu‐ and ZnO‐containing methanol‐synthesis catalysts were obtained by vaporizing suitable organometallic precursors into mesoporous silicates, followed by thermal treatment (see scheme). The catalytically active components in the final material have nanoscopic dimensions. The methanol production by the catalysts is similar to that of systems synthesized by the classical route.</abstract><cop>Weinheim</cop><pub>WILEY-VCH Verlag</pub><pmid>15150763</pmid><doi>10.1002/anie.200351166</doi><tpages>4</tpages></addata></record>
fulltext fulltext
identifier ISSN: 1433-7851
ispartof Angewandte Chemie International Edition, 2004-05, Vol.43 (21), p.2839-2842
issn 1433-7851
1521-3773
language eng
recordid cdi_proquest_miscellaneous_71936451
source Access via Wiley Online Library
subjects copper
CVD (chemical vapor deposition)
heterogeneous catalysis
mesoporous materials
methanol synthesis
zinc oxide
title MOCVD-Loading of Mesoporous Siliceous Matrices with Cu/ZnO: Supported Catalysts for Methanol Synthesis
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-16T10%3A28%3A37IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=MOCVD-Loading%20of%20Mesoporous%20Siliceous%20Matrices%20with%20Cu/ZnO:%20Supported%20Catalysts%20for%20Methanol%20Synthesis&rft.jtitle=Angewandte%20Chemie%20International%20Edition&rft.au=Becker,%20Ralf&rft.date=2004-05-17&rft.volume=43&rft.issue=21&rft.spage=2839&rft.epage=2842&rft.pages=2839-2842&rft.issn=1433-7851&rft.eissn=1521-3773&rft_id=info:doi/10.1002/anie.200351166&rft_dat=%3Cproquest_cross%3E71936451%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=71936451&rft_id=info:pmid/15150763&rfr_iscdi=true