Femtosecond coincidence imaging of multichannel multiphoton dynamics

Femtosecond coincidence imaging of multichannel multiphoton dynamics

The novel technique of femtosecond time-resolved photoelectron-photoion coincidence imaging is applied to unravel dissociative ionization processes in a polyatomic molecule. Femtosecond coincidence imaging of CF3I photodynamics illustrates how competing multiphoton dissociation pathways can be disti...

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Veröffentlicht in:Physical review letters 2004-03, Vol.92 (12), p.123002-123002, Article 123002
Hauptverfasser: Rijs, Anouk M, Janssen, Maurice H M, Chrysostom, Engelene T H, Hayden, Carl C
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container_title Physical review letters
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creator Rijs, Anouk M
Janssen, Maurice H M
Chrysostom, Engelene T H
Hayden, Carl C
description The novel technique of femtosecond time-resolved photoelectron-photoion coincidence imaging is applied to unravel dissociative ionization processes in a polyatomic molecule. Femtosecond coincidence imaging of CF3I photodynamics illustrates how competing multiphoton dissociation pathways can be distinguished, which would be impossible using photoelectron or ion imaging alone. Ion-electron energy correlations and photoelectron angular distributions reveal competing processes for the channel producing (e(-)+CF+3+I). The molecular-frame photoelectron angular distributions of the two major pathways are strikingly different.
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title Femtosecond coincidence imaging of multichannel multiphoton dynamics
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