Design and Synthesis of 3d−4f Metal-Based Zeolite-type Materials with a 3D Nanotubular Structure Encapsulated “Water” Pipe
A nanotubular 3D heterometallic zeolitic polymer, {[Yb(PDA)3Mn1.5(H2O)3]·1.5H2O} n (2), was designed and synthesized by simply tuning the amount of coordinated water on the Mn ion in the molecular ladder polymer {[Yb(PDA)3Mn1.5(H2O)6]·6H2O} n (1). 1 and 2 were structurally and magnetically character...
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| Veröffentlicht in: | Journal of the American Chemical Society 2004-03, Vol.126 (10), p.3012-3013 |
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| container_issue | 10 |
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| container_title | Journal of the American Chemical Society |
| container_volume | 126 |
| creator | Zhao, Bin Cheng, Peng Chen, Xiaoyan Cheng, Cai Shi, Wei Liao, Daizheng Yan, Shiping Jiang, Zonghui |
| description | A nanotubular 3D heterometallic zeolitic polymer, {[Yb(PDA)3Mn1.5(H2O)3]·1.5H2O} n (2), was designed and synthesized by simply tuning the amount of coordinated water on the Mn ion in the molecular ladder polymer {[Yb(PDA)3Mn1.5(H2O)6]·6H2O} n (1). 1 and 2 were structurally and magnetically characterized. The water molecules capsulated within the nanotube were arrayed into an unprecedented “water” pipe. The robust 2 retained intact networks after the removal of guest water trapped in the nanotubes and even after methanol replaced guest water. |
| doi_str_mv | 10.1021/ja038784e |
| format | Article |
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The water molecules capsulated within the nanotube were arrayed into an unprecedented “water” pipe. 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Am. Chem. Soc</addtitle><description>A nanotubular 3D heterometallic zeolitic polymer, {[Yb(PDA)3Mn1.5(H2O)3]·1.5H2O} n (2), was designed and synthesized by simply tuning the amount of coordinated water on the Mn ion in the molecular ladder polymer {[Yb(PDA)3Mn1.5(H2O)6]·6H2O} n (1). 1 and 2 were structurally and magnetically characterized. The water molecules capsulated within the nanotube were arrayed into an unprecedented “water” pipe. The robust 2 retained intact networks after the removal of guest water trapped in the nanotubes and even after methanol replaced guest water.</description><subject>Chemistry</subject><subject>Condensed matter: structure, mechanical and thermal properties</subject><subject>Exact sciences and technology</subject><subject>General and physical chemistry</subject><subject>Inorganic compounds</subject><subject>Ion-exchange</subject><subject>Metal complexes</subject><subject>Physics</subject><subject>Structure of solids and liquids; crystallography</subject><subject>Structure of specific crystalline solids</subject><subject>Surface physical chemistry</subject><subject>Zeolites: preparations and properties</subject><issn>0002-7863</issn><issn>1520-5126</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2004</creationdate><recordtype>article</recordtype><recordid>eNptkMFu1DAQhi0EokvhwAsgX0DiELBjJ06OtNulSN1SsUVIXKyJM6ZZskmwHbV72yNnzvBy-yS42lXLgZM1nm8-zfyEPOfsDWcpf7sEJgpVSHxAJjxLWZLxNH9IJoyxNFFFLg7IE--XsZRpwR-TA54xnnKWT8hmir751lHoarpYd-Eqlp72lop6-_OXtHSOAdrkCDzW9Cv2bRMwCesB6RwCugZaT6-bcEWBiik9h64PYzW24OgiuNGE0SE96QwMPn6G6Nhufn-5ndxu_tCLZsCn5JGNEny2fw_J59nJ5fFpcvbx_Yfjd2cJCFWGRKLMbSlSLlJTGplntbFFxeqKK1mUGWelzU1a5WizeGVZlygKiL1K2lLVuRCH5NXOO7j-x4g-6FXjDbYtdNiPXiuuhJJMRfD1DjSu996h1YNrVuDWmjN9G7e-izuyL_bSsVphfU_u843Ayz0A3kBrHXSm8f9wmVJCyMglO67xAW_u-uC-6zzulenLi4Wen7JPanY-1bN7Lxivl_3oupjdfxb8C-a6pNU</recordid><startdate>20040317</startdate><enddate>20040317</enddate><creator>Zhao, Bin</creator><creator>Cheng, Peng</creator><creator>Chen, Xiaoyan</creator><creator>Cheng, Cai</creator><creator>Shi, Wei</creator><creator>Liao, Daizheng</creator><creator>Yan, Shiping</creator><creator>Jiang, Zonghui</creator><general>American Chemical Society</general><scope>BSCLL</scope><scope>IQODW</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope></search><sort><creationdate>20040317</creationdate><title>Design and Synthesis of 3d−4f Metal-Based Zeolite-type Materials with a 3D Nanotubular Structure Encapsulated “Water” Pipe</title><author>Zhao, Bin ; Cheng, Peng ; Chen, Xiaoyan ; Cheng, Cai ; Shi, Wei ; Liao, Daizheng ; Yan, Shiping ; Jiang, Zonghui</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a379t-4e46f932132c9c465dcf8b0db174895109f6c2b6ef50049d9e38a174b4f97d633</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2004</creationdate><topic>Chemistry</topic><topic>Condensed matter: structure, mechanical and thermal properties</topic><topic>Exact sciences and technology</topic><topic>General and physical chemistry</topic><topic>Inorganic compounds</topic><topic>Ion-exchange</topic><topic>Metal complexes</topic><topic>Physics</topic><topic>Structure of solids and liquids; crystallography</topic><topic>Structure of specific crystalline solids</topic><topic>Surface physical chemistry</topic><topic>Zeolites: preparations and properties</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhao, Bin</creatorcontrib><creatorcontrib>Cheng, Peng</creatorcontrib><creatorcontrib>Chen, Xiaoyan</creatorcontrib><creatorcontrib>Cheng, Cai</creatorcontrib><creatorcontrib>Shi, Wei</creatorcontrib><creatorcontrib>Liao, Daizheng</creatorcontrib><creatorcontrib>Yan, Shiping</creatorcontrib><creatorcontrib>Jiang, Zonghui</creatorcontrib><collection>Istex</collection><collection>Pascal-Francis</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>Journal of the American Chemical Society</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhao, Bin</au><au>Cheng, Peng</au><au>Chen, Xiaoyan</au><au>Cheng, Cai</au><au>Shi, Wei</au><au>Liao, Daizheng</au><au>Yan, Shiping</au><au>Jiang, Zonghui</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Design and Synthesis of 3d−4f Metal-Based Zeolite-type Materials with a 3D Nanotubular Structure Encapsulated “Water” Pipe</atitle><jtitle>Journal of the American Chemical Society</jtitle><addtitle>J. Am. Chem. Soc</addtitle><date>2004-03-17</date><risdate>2004</risdate><volume>126</volume><issue>10</issue><spage>3012</spage><epage>3013</epage><pages>3012-3013</pages><issn>0002-7863</issn><eissn>1520-5126</eissn><coden>JACSAT</coden><abstract>A nanotubular 3D heterometallic zeolitic polymer, {[Yb(PDA)3Mn1.5(H2O)3]·1.5H2O} n (2), was designed and synthesized by simply tuning the amount of coordinated water on the Mn ion in the molecular ladder polymer {[Yb(PDA)3Mn1.5(H2O)6]·6H2O} n (1). 1 and 2 were structurally and magnetically characterized. The water molecules capsulated within the nanotube were arrayed into an unprecedented “water” pipe. The robust 2 retained intact networks after the removal of guest water trapped in the nanotubes and even after methanol replaced guest water.</abstract><cop>Washington, DC</cop><pub>American Chemical Society</pub><pmid>15012106</pmid><doi>10.1021/ja038784e</doi><tpages>2</tpages></addata></record> |
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| subjects | Chemistry Condensed matter: structure, mechanical and thermal properties Exact sciences and technology General and physical chemistry Inorganic compounds Ion-exchange Metal complexes Physics Structure of solids and liquids crystallography Structure of specific crystalline solids Surface physical chemistry Zeolites: preparations and properties |
| title | Design and Synthesis of 3d−4f Metal-Based Zeolite-type Materials with a 3D Nanotubular Structure Encapsulated “Water” Pipe |
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