Mean-field nucleation theory with nonlocal interactions

Mean-field nucleation theory has for a long time been successfully used to extract microscopic parameters from island density data in growth experiments. However, it produces grossly incorrect results when used to analyze weakly corrugated systems, where adsorbate interactions cannot be neglected. H...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Physical review letters 2002-03, Vol.88 (11), p.116102-116102, Article 116102
1. Verfasser: Ovesson, Staffan
Format: Artikel
Sprache:eng
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 116102
container_issue 11
container_start_page 116102
container_title Physical review letters
container_volume 88
creator Ovesson, Staffan
description Mean-field nucleation theory has for a long time been successfully used to extract microscopic parameters from island density data in growth experiments. However, it produces grossly incorrect results when used to analyze weakly corrugated systems, where adsorbate interactions cannot be neglected. Here, a mean-field theory that includes nonlocal adsorbate interactions is developed and successfully tested against kinetic Monte Carlo growth simulations for a realistic adsorbate system.
doi_str_mv 10.1103/PhysRevLett.88.116102
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_71534318</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>71534318</sourcerecordid><originalsourceid>FETCH-LOGICAL-c307t-2284014b9cf75a7c135386a2c21a7065124acadbcf673777536170131260a7b03</originalsourceid><addsrcrecordid>eNpNkE1Lw0AQhhdRbK3-BCUnb6kzu0lmc5TiF1QU0fOy2W5oJN3U3Y2Sf29KC3oaGJ73neFh7BJhjgji5nU9hDf7vbQxzqUcdwUCP2JTBCpTQsyO2RRAYFoC0ISdhfAJAMgLecomiCWUGWZTRs9Wu7RubLtKXG9aq2PTuSSubeeH5KeJ68R1ru2MbpPGReu12QHhnJ3Uug324jBn7OP-7n3xmC5fHp4Wt8vUCKCYci4zwKwqTU25JoMiF7LQ3HDUBEWOPNNGrypTFySIKBcFEqAY_wRNFYgZu973bn331dsQ1aYJxratdrbrgyLMRSZQjmC-B43vQvC2VlvfbLQfFILaGVP_jCkp1d7YmLs6HOirjV39pQ6KxC9z52jO</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>71534318</pqid></control><display><type>article</type><title>Mean-field nucleation theory with nonlocal interactions</title><source>American Physical Society Journals</source><creator>Ovesson, Staffan</creator><creatorcontrib>Ovesson, Staffan</creatorcontrib><description>Mean-field nucleation theory has for a long time been successfully used to extract microscopic parameters from island density data in growth experiments. However, it produces grossly incorrect results when used to analyze weakly corrugated systems, where adsorbate interactions cannot be neglected. Here, a mean-field theory that includes nonlocal adsorbate interactions is developed and successfully tested against kinetic Monte Carlo growth simulations for a realistic adsorbate system.</description><identifier>ISSN: 0031-9007</identifier><identifier>EISSN: 1079-7114</identifier><identifier>DOI: 10.1103/PhysRevLett.88.116102</identifier><identifier>PMID: 11909414</identifier><language>eng</language><publisher>United States</publisher><ispartof>Physical review letters, 2002-03, Vol.88 (11), p.116102-116102, Article 116102</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c307t-2284014b9cf75a7c135386a2c21a7065124acadbcf673777536170131260a7b03</citedby><cites>FETCH-LOGICAL-c307t-2284014b9cf75a7c135386a2c21a7065124acadbcf673777536170131260a7b03</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>315,781,785,2877,2878,27929,27930</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/11909414$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Ovesson, Staffan</creatorcontrib><title>Mean-field nucleation theory with nonlocal interactions</title><title>Physical review letters</title><addtitle>Phys Rev Lett</addtitle><description>Mean-field nucleation theory has for a long time been successfully used to extract microscopic parameters from island density data in growth experiments. However, it produces grossly incorrect results when used to analyze weakly corrugated systems, where adsorbate interactions cannot be neglected. Here, a mean-field theory that includes nonlocal adsorbate interactions is developed and successfully tested against kinetic Monte Carlo growth simulations for a realistic adsorbate system.</description><issn>0031-9007</issn><issn>1079-7114</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2002</creationdate><recordtype>article</recordtype><recordid>eNpNkE1Lw0AQhhdRbK3-BCUnb6kzu0lmc5TiF1QU0fOy2W5oJN3U3Y2Sf29KC3oaGJ73neFh7BJhjgji5nU9hDf7vbQxzqUcdwUCP2JTBCpTQsyO2RRAYFoC0ISdhfAJAMgLecomiCWUGWZTRs9Wu7RubLtKXG9aq2PTuSSubeeH5KeJ68R1ru2MbpPGReu12QHhnJ3Uug324jBn7OP-7n3xmC5fHp4Wt8vUCKCYci4zwKwqTU25JoMiF7LQ3HDUBEWOPNNGrypTFySIKBcFEqAY_wRNFYgZu973bn331dsQ1aYJxratdrbrgyLMRSZQjmC-B43vQvC2VlvfbLQfFILaGVP_jCkp1d7YmLs6HOirjV39pQ6KxC9z52jO</recordid><startdate>20020318</startdate><enddate>20020318</enddate><creator>Ovesson, Staffan</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope></search><sort><creationdate>20020318</creationdate><title>Mean-field nucleation theory with nonlocal interactions</title><author>Ovesson, Staffan</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c307t-2284014b9cf75a7c135386a2c21a7065124acadbcf673777536170131260a7b03</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2002</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ovesson, Staffan</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>Physical review letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ovesson, Staffan</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Mean-field nucleation theory with nonlocal interactions</atitle><jtitle>Physical review letters</jtitle><addtitle>Phys Rev Lett</addtitle><date>2002-03-18</date><risdate>2002</risdate><volume>88</volume><issue>11</issue><spage>116102</spage><epage>116102</epage><pages>116102-116102</pages><artnum>116102</artnum><issn>0031-9007</issn><eissn>1079-7114</eissn><abstract>Mean-field nucleation theory has for a long time been successfully used to extract microscopic parameters from island density data in growth experiments. However, it produces grossly incorrect results when used to analyze weakly corrugated systems, where adsorbate interactions cannot be neglected. Here, a mean-field theory that includes nonlocal adsorbate interactions is developed and successfully tested against kinetic Monte Carlo growth simulations for a realistic adsorbate system.</abstract><cop>United States</cop><pmid>11909414</pmid><doi>10.1103/PhysRevLett.88.116102</doi><tpages>1</tpages></addata></record>
fulltext fulltext
identifier ISSN: 0031-9007
ispartof Physical review letters, 2002-03, Vol.88 (11), p.116102-116102, Article 116102
issn 0031-9007
1079-7114
language eng
recordid cdi_proquest_miscellaneous_71534318
source American Physical Society Journals
title Mean-field nucleation theory with nonlocal interactions
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-14T07%3A50%3A56IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Mean-field%20nucleation%20theory%20with%20nonlocal%20interactions&rft.jtitle=Physical%20review%20letters&rft.au=Ovesson,%20Staffan&rft.date=2002-03-18&rft.volume=88&rft.issue=11&rft.spage=116102&rft.epage=116102&rft.pages=116102-116102&rft.artnum=116102&rft.issn=0031-9007&rft.eissn=1079-7114&rft_id=info:doi/10.1103/PhysRevLett.88.116102&rft_dat=%3Cproquest_cross%3E71534318%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=71534318&rft_id=info:pmid/11909414&rfr_iscdi=true