Catalytic Motors for Transport of Colloidal Cargo
Autonomous micro- and nanomotors should, in principle, deliver materials in a site-directed fashion, powering the assembly of dynamic, nonequilibrium superstructures. Here we demonstrate that catalytic Pt−Au nanomotors can transport a prototypical cargo: polystyrene microspheres. In addition, motors...
Gespeichert in:
| Veröffentlicht in: | Nano letters 2008-05, Vol.8 (5), p.1271-1276 |
|---|---|
| Hauptverfasser: | , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 1276 |
|---|---|
| container_issue | 5 |
| container_start_page | 1271 |
| container_title | Nano letters |
| container_volume | 8 |
| creator | Sundararajan, Shakuntala Lammert, Paul E Zudans, Andrew W Crespi, Vincent H Sen, Ayusman |
| description | Autonomous micro- and nanomotors should, in principle, deliver materials in a site-directed fashion, powering the assembly of dynamic, nonequilibrium superstructures. Here we demonstrate that catalytic Pt−Au nanomotors can transport a prototypical cargo: polystyrene microspheres. In addition, motors with Ni segments can overcome both Brownian orientational fluctuations and biased rotation of the rod−sphere doublet to enable persistent steerable uniaxial motion in an external magnetic field. Assuming a cargo-independent motive force, the speeds are inversely proportional to the Stokes resistance, which we compute using a completed double-layer boundary integral equation. In addition, we demonstrate motors transporting cargo via chemotaxis toward a H2O2 fuel source. |
| doi_str_mv | 10.1021/nl072275j |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_70724539</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>70724539</sourcerecordid><originalsourceid>FETCH-LOGICAL-a409t-bb9732589237054d2d6958b6cdcc46a1481f544e7581a3164d587028c9a1dfb53</originalsourceid><addsrcrecordid>eNpt0LtOwzAUgGELgWgpDLwAygISQ8DX2B5RxE0qYimzdWInKJUbFzsZ-vYENWoXJp_h0znyj9A1wQ8EU_LYeSwplWJ9guZEMJwXWtPTw6z4DF2ktMYYaybwOZoRxUkhOJ4jUkIPfte3NvsIfYgpa0LMVhG6tA2xz0KTlcH70DrwWQnxO1yiswZ8qq-md4G-Xp5X5Vu-_Hx9L5-WOXCs-7yqtGRUKE2ZxII76gotVFVYZy0vgHBFGsF5LYUiwEjBnVASU2U1ENdUgi3Q3X7vNoafoU692bTJ1t5DV4chGTn-mQumR3i_hzaGlGLdmG1sNxB3hmDz18cc-oz2Zlo6VJvaHeUUZAS3E4BkwTdjCNumg6OYCSl5cXRgk1mHIXZji38O_gJyr3am</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>70724539</pqid></control><display><type>article</type><title>Catalytic Motors for Transport of Colloidal Cargo</title><source>MEDLINE</source><source>ACS Publications</source><creator>Sundararajan, Shakuntala ; Lammert, Paul E ; Zudans, Andrew W ; Crespi, Vincent H ; Sen, Ayusman</creator><creatorcontrib>Sundararajan, Shakuntala ; Lammert, Paul E ; Zudans, Andrew W ; Crespi, Vincent H ; Sen, Ayusman</creatorcontrib><description>Autonomous micro- and nanomotors should, in principle, deliver materials in a site-directed fashion, powering the assembly of dynamic, nonequilibrium superstructures. Here we demonstrate that catalytic Pt−Au nanomotors can transport a prototypical cargo: polystyrene microspheres. In addition, motors with Ni segments can overcome both Brownian orientational fluctuations and biased rotation of the rod−sphere doublet to enable persistent steerable uniaxial motion in an external magnetic field. Assuming a cargo-independent motive force, the speeds are inversely proportional to the Stokes resistance, which we compute using a completed double-layer boundary integral equation. In addition, we demonstrate motors transporting cargo via chemotaxis toward a H2O2 fuel source.</description><identifier>ISSN: 1530-6984</identifier><identifier>EISSN: 1530-6992</identifier><identifier>DOI: 10.1021/nl072275j</identifier><identifier>PMID: 18416540</identifier><language>eng</language><publisher>Washington, DC: American Chemical Society</publisher><subject>Applied sciences ; Colloids - chemistry ; Computer Simulation ; Electromagnetic Fields ; Electronics ; Exact sciences and technology ; Gold - chemistry ; Gold - radiation effects ; Materials Testing ; Micro- and nanoelectromechanical devices (mems/nems) ; Models, Chemical ; Models, Molecular ; Motion ; Nanostructures - chemistry ; Nanostructures - radiation effects ; Nanostructures - ultrastructure ; Nanotechnology - instrumentation ; Nanotechnology - methods ; Particle Size ; Platinum - chemistry ; Platinum - radiation effects ; Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices</subject><ispartof>Nano letters, 2008-05, Vol.8 (5), p.1271-1276</ispartof><rights>Copyright © 2008 American Chemical Society</rights><rights>2008 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a409t-bb9732589237054d2d6958b6cdcc46a1481f544e7581a3164d587028c9a1dfb53</citedby><cites>FETCH-LOGICAL-a409t-bb9732589237054d2d6958b6cdcc46a1481f544e7581a3164d587028c9a1dfb53</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/nl072275j$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/nl072275j$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,778,782,2754,27059,27907,27908,56721,56771</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=20357746$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/18416540$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Sundararajan, Shakuntala</creatorcontrib><creatorcontrib>Lammert, Paul E</creatorcontrib><creatorcontrib>Zudans, Andrew W</creatorcontrib><creatorcontrib>Crespi, Vincent H</creatorcontrib><creatorcontrib>Sen, Ayusman</creatorcontrib><title>Catalytic Motors for Transport of Colloidal Cargo</title><title>Nano letters</title><addtitle>Nano Lett</addtitle><description>Autonomous micro- and nanomotors should, in principle, deliver materials in a site-directed fashion, powering the assembly of dynamic, nonequilibrium superstructures. Here we demonstrate that catalytic Pt−Au nanomotors can transport a prototypical cargo: polystyrene microspheres. In addition, motors with Ni segments can overcome both Brownian orientational fluctuations and biased rotation of the rod−sphere doublet to enable persistent steerable uniaxial motion in an external magnetic field. Assuming a cargo-independent motive force, the speeds are inversely proportional to the Stokes resistance, which we compute using a completed double-layer boundary integral equation. In addition, we demonstrate motors transporting cargo via chemotaxis toward a H2O2 fuel source.</description><subject>Applied sciences</subject><subject>Colloids - chemistry</subject><subject>Computer Simulation</subject><subject>Electromagnetic Fields</subject><subject>Electronics</subject><subject>Exact sciences and technology</subject><subject>Gold - chemistry</subject><subject>Gold - radiation effects</subject><subject>Materials Testing</subject><subject>Micro- and nanoelectromechanical devices (mems/nems)</subject><subject>Models, Chemical</subject><subject>Models, Molecular</subject><subject>Motion</subject><subject>Nanostructures - chemistry</subject><subject>Nanostructures - radiation effects</subject><subject>Nanostructures - ultrastructure</subject><subject>Nanotechnology - instrumentation</subject><subject>Nanotechnology - methods</subject><subject>Particle Size</subject><subject>Platinum - chemistry</subject><subject>Platinum - radiation effects</subject><subject>Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices</subject><issn>1530-6984</issn><issn>1530-6992</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2008</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNpt0LtOwzAUgGELgWgpDLwAygISQ8DX2B5RxE0qYimzdWInKJUbFzsZ-vYENWoXJp_h0znyj9A1wQ8EU_LYeSwplWJ9guZEMJwXWtPTw6z4DF2ktMYYaybwOZoRxUkhOJ4jUkIPfte3NvsIfYgpa0LMVhG6tA2xz0KTlcH70DrwWQnxO1yiswZ8qq-md4G-Xp5X5Vu-_Hx9L5-WOXCs-7yqtGRUKE2ZxII76gotVFVYZy0vgHBFGsF5LYUiwEjBnVASU2U1ENdUgi3Q3X7vNoafoU692bTJ1t5DV4chGTn-mQumR3i_hzaGlGLdmG1sNxB3hmDz18cc-oz2Zlo6VJvaHeUUZAS3E4BkwTdjCNumg6OYCSl5cXRgk1mHIXZji38O_gJyr3am</recordid><startdate>20080501</startdate><enddate>20080501</enddate><creator>Sundararajan, Shakuntala</creator><creator>Lammert, Paul E</creator><creator>Zudans, Andrew W</creator><creator>Crespi, Vincent H</creator><creator>Sen, Ayusman</creator><general>American Chemical Society</general><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope></search><sort><creationdate>20080501</creationdate><title>Catalytic Motors for Transport of Colloidal Cargo</title><author>Sundararajan, Shakuntala ; Lammert, Paul E ; Zudans, Andrew W ; Crespi, Vincent H ; Sen, Ayusman</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a409t-bb9732589237054d2d6958b6cdcc46a1481f544e7581a3164d587028c9a1dfb53</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2008</creationdate><topic>Applied sciences</topic><topic>Colloids - chemistry</topic><topic>Computer Simulation</topic><topic>Electromagnetic Fields</topic><topic>Electronics</topic><topic>Exact sciences and technology</topic><topic>Gold - chemistry</topic><topic>Gold - radiation effects</topic><topic>Materials Testing</topic><topic>Micro- and nanoelectromechanical devices (mems/nems)</topic><topic>Models, Chemical</topic><topic>Models, Molecular</topic><topic>Motion</topic><topic>Nanostructures - chemistry</topic><topic>Nanostructures - radiation effects</topic><topic>Nanostructures - ultrastructure</topic><topic>Nanotechnology - instrumentation</topic><topic>Nanotechnology - methods</topic><topic>Particle Size</topic><topic>Platinum - chemistry</topic><topic>Platinum - radiation effects</topic><topic>Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Sundararajan, Shakuntala</creatorcontrib><creatorcontrib>Lammert, Paul E</creatorcontrib><creatorcontrib>Zudans, Andrew W</creatorcontrib><creatorcontrib>Crespi, Vincent H</creatorcontrib><creatorcontrib>Sen, Ayusman</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>Nano letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Sundararajan, Shakuntala</au><au>Lammert, Paul E</au><au>Zudans, Andrew W</au><au>Crespi, Vincent H</au><au>Sen, Ayusman</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Catalytic Motors for Transport of Colloidal Cargo</atitle><jtitle>Nano letters</jtitle><addtitle>Nano Lett</addtitle><date>2008-05-01</date><risdate>2008</risdate><volume>8</volume><issue>5</issue><spage>1271</spage><epage>1276</epage><pages>1271-1276</pages><issn>1530-6984</issn><eissn>1530-6992</eissn><abstract>Autonomous micro- and nanomotors should, in principle, deliver materials in a site-directed fashion, powering the assembly of dynamic, nonequilibrium superstructures. Here we demonstrate that catalytic Pt−Au nanomotors can transport a prototypical cargo: polystyrene microspheres. In addition, motors with Ni segments can overcome both Brownian orientational fluctuations and biased rotation of the rod−sphere doublet to enable persistent steerable uniaxial motion in an external magnetic field. Assuming a cargo-independent motive force, the speeds are inversely proportional to the Stokes resistance, which we compute using a completed double-layer boundary integral equation. In addition, we demonstrate motors transporting cargo via chemotaxis toward a H2O2 fuel source.</abstract><cop>Washington, DC</cop><pub>American Chemical Society</pub><pmid>18416540</pmid><doi>10.1021/nl072275j</doi><tpages>6</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1530-6984 |
| ispartof | Nano letters, 2008-05, Vol.8 (5), p.1271-1276 |
| issn | 1530-6984 1530-6992 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_70724539 |
| source | MEDLINE; ACS Publications |
| subjects | Applied sciences Colloids - chemistry Computer Simulation Electromagnetic Fields Electronics Exact sciences and technology Gold - chemistry Gold - radiation effects Materials Testing Micro- and nanoelectromechanical devices (mems/nems) Models, Chemical Models, Molecular Motion Nanostructures - chemistry Nanostructures - radiation effects Nanostructures - ultrastructure Nanotechnology - instrumentation Nanotechnology - methods Particle Size Platinum - chemistry Platinum - radiation effects Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices |
| title | Catalytic Motors for Transport of Colloidal Cargo |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-17T04%3A54%3A51IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Catalytic%20Motors%20for%20Transport%20of%20Colloidal%20Cargo&rft.jtitle=Nano%20letters&rft.au=Sundararajan,%20Shakuntala&rft.date=2008-05-01&rft.volume=8&rft.issue=5&rft.spage=1271&rft.epage=1276&rft.pages=1271-1276&rft.issn=1530-6984&rft.eissn=1530-6992&rft_id=info:doi/10.1021/nl072275j&rft_dat=%3Cproquest_cross%3E70724539%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=70724539&rft_id=info:pmid/18416540&rfr_iscdi=true |