Laser Absorption Scanning Tunneling Microscopy of Carbon Nanotubes

We report single molecule laser absorption by carbon nanotubes stamped under ultrahigh vacuum onto Si(100)2×1:H surfaces. Absorption is detected by scanning tunneling microscopy. Images are obtained with and without modulated laser excitation using lock-in amplification and a rear-illumination geome...

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Veröffentlicht in:Nano letters 2006-01, Vol.6 (1), p.45-49
Hauptverfasser: Ballard, Joshua B, Carmichael, Erin S, Shi, Dongxia, Lyding, Joseph W, Gruebele, Martin
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container_issue 1
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container_title Nano letters
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creator Ballard, Joshua B
Carmichael, Erin S
Shi, Dongxia
Lyding, Joseph W
Gruebele, Martin
description We report single molecule laser absorption by carbon nanotubes stamped under ultrahigh vacuum onto Si(100)2×1:H surfaces. Absorption is detected by scanning tunneling microscopy. Images are obtained with and without modulated laser excitation using lock-in amplification and a rear-illumination geometry to reduce thermal effects. Noise appears at topographic edges and is analyzed by a quantitative model in terms of scan speed, mechanical instabilities, and feedback current fluctuations at the edge of the nanotubes. Noise due to mechanical instabilities is shown to persist even in the limit of slow scan speed.
doi_str_mv 10.1021/nl0519231
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subjects Condensed matter: structure, mechanical and thermal properties
Cross-disciplinary physics: materials science
rheology
Electron, ion, and scanning probe microscopy
Exact sciences and technology
Materials science
Nanoscale materials and structures: fabrication and characterization
Nanotubes
Physics
Scanning probe microscopy: scanning tunneling, atomic force, scanning optical, magnetic force, etc
Structure of solids and liquids
crystallography
title Laser Absorption Scanning Tunneling Microscopy of Carbon Nanotubes
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