Diaryl Ethers Using Fischer Chromium Carbene Mediated Benzannulation

Diaryl Ethers Using Fischer Chromium Carbene Mediated Benzannulation

The biological relevance and irresistible synthetic challenge of compounds containing the diaryl ether linkage encourages the development of new methodologies targeted toward this structural subunit. The syntheses of diaryl ethers 2 using a benzannulation strategy that formally involves a [3 + 2 + 1...

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Veröffentlicht in:Organic letters 1999-12, Vol.1 (11), p.1721-1723
Hauptverfasser: Pulley, Shon R, Sen, Subhabrata, Vorogushin, Andrei, Swanson, Erika
Format: Artikel
Sprache:eng
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Alkynes - chemistry
Chromium - chemistry
Cyclization
Organometallic Compounds - chemistry
Phenyl Ethers - chemical synthesis
Ultrasonics
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container_end_page 1723
container_issue 11
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container_title Organic letters
container_volume 1
creator Pulley, Shon R
Sen, Subhabrata
Vorogushin, Andrei
Swanson, Erika
description The biological relevance and irresistible synthetic challenge of compounds containing the diaryl ether linkage encourages the development of new methodologies targeted toward this structural subunit. The syntheses of diaryl ethers 2 using a benzannulation strategy that formally involves a [3 + 2 + 1] cycloaddition between aryloxy-substituted Fischer carbenes 1 and alkynes are described. This methodology provides a neutral near ambient temperature formation of diaryl ethers.
doi_str_mv 10.1021/ol990949u
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subjects Alkynes - chemistry
Chromium - chemistry
Cyclization
Organometallic Compounds - chemistry
Phenyl Ethers - chemical synthesis
Ultrasonics
title Diaryl Ethers Using Fischer Chromium Carbene Mediated Benzannulation
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